Related papers: Coherent Control of Bond Making
We propose to control the retinal photoisomerization yield through the back-action dynamics imparted by a nonselective optical measurement of the molecular electronic state. This incoherent effect is easier to implement than comparable…
The coherent control of optical phonons has been experimentally demonstrated in various physical systems. While the transient dynamics for optical phonons can be explained by phenomenological models, the coherent control experiment cannot…
Coherent control of the atomic two-photon absorption with shaped single-cycle pulses is examined theoretically in the weak-field regime. The control over the stabilized carrier-envelope phase (CEP) of the pulses is determined as a key…
We theoretically examine photoassociation of a two-component Fermi degenerate gas, focusing on light-induced atom-atom interactions as a means to raise the critical temperature of the BCS transition to a superfluid state. As it stands,…
We experimentally demonstrate coherent control of the nonlinear response of optical second harmonic generation in resonant nanostructures beyond the weak-field regime. Contrary to common perception, we show that maximizing the intensity of…
Photoassociation of ultracold atoms is shown to lead to alignment of the product molecules along the excitation laser polarization axis. We theoretically investigate pulsed photoassociation of $^{87}Rb$ atoms into a specific weakly-bound…
The generation of the narrowband strong-correlated biphotons via spontaneous four-wave mixing can be effectively controlled and enhanced by an additional driving field which drives a transition with its upper level being a Rydberg state. We…
Two-photon photoassociation of hot magnesium atoms by femtosecond laser pulses, creating electronically excited magnesium dimer molecules, is studied from first principles, combining \textit{ab initio} quantum chemistry and molecular…
Coherent control over photoelectron wavepackets, via the use of polarization-shaped laser pulses, can be understood as a time and polarization-multiplexed process. In this work, we investigate this multiplexing via computation of the…
We consider the simultaneous propagation of a pair of Raman-resonant, frequency-modulated (chirped) laser pulses in an optically thick medium, modeled by an ensemble of $\Lambda$-atoms. A self-organization ('matching`) effect is shown for…
We describe optimized coherent control methods for two-photon transitions in atoms of a ladder-type three-state energy configuration. Our approach is based on the spatial coherent control scheme which utilizes counter-propagating ultrashort…
We demonstrate the use of the ultrafast spatial coherent-control method to resolve the fine-structure two-photon transitions of atomic rubidium. Counter-propagating ultrafast optical pulses with spectral phase and amplitude programmed with…
We propose and demonstrate a robust control scheme by ultrafast nonadiabatic chirped laser pulse, designed for targeting coherent superpositions of two-level systems. Robustness against power fluctuation is proved by our numerical study and…
We describe experiments and associated quantum simulations involving the production of ultracold $^{87}$Rb$_{2}$ molecules with nanosecond pulses of frequency-chirped light. With appropriate chirp parameters, the formation is dominated by…
The coherent superposition of two-atomic levels induced by coherent population trapping is employed in a standard $\Lambda$ type scheme to form a tripod-like system. A weak probe pulse scanning across the system is shown to experience a…
We demonstrate coherent control of multiphoton and above-threshold photoemission from a single solid-state nanoemitter driven by a fundamental and a weak second harmonic laser pulse. Depending on the relative phase of the two pulses,…
Coherent control of femtosecond two-photon absorption in the intermediate-field regime is analyzed in detail in the powerful frequency domain using an extended 4th-order perturbative description. The corresponding absorption is coherently…
We describe a new method of coherent optical control of internal dynamics of atomic collisions by means of two correlated light beams having entangled polarizations. We show that if excitation of a colliding pair of atoms is by two photons…
A chirped-pulse quantum control scheme applicable to Coherent Anti-Stokes Raman Scattering spectroscopy, named as C-CARS, is presented aimed at maximizing the vibrational coherence in molecules. It implies chirping of three incoming pulses…
We address a scheme to enhance the quantum correlations in cavity opto-magnomechanical system by using the coherent feedback loop in the presence of magnon squeezing. The proposed coherent feedback-control allows a significant enhancement…