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Frustrated three dimensional quantum magnets are notoriously impervious to theoretical analysis. Here we use a combination of three computational methods to investigate the three dimensional pyrochlore $S=1/2$ quantum antiferromagnet, an…

Strongly Correlated Electrons · Physics 2020-08-10 Robin Schäfer , Imre Hagymási , Roderich Moessner , David J. Luitz

Using 170-Yb and 155-Gd Mossbauer measurements down to 0.03K, we have examined the semiconducting pyrochlore Yb2Mo2O7 where the Mo intra-sublattice interaction is anti-ferromagnetic and the metallic pyrochlore Gd2Mo2O7 where this…

Condensed Matter · Physics 2009-11-10 J. A. Hodges , P. Bonville , A. Forget , J. P. Sanchez , P. Vulliet , M. Rams , K. Krolas

In this study, we performed powder neutron diffraction and inelastic scattering measurements of frustrated pyrochlore Nd$_2$Ir$_2$O$_7$, which exhibits a metal-insulator transition at a temperature $T_{\rm MI}$ of 33 K. The diffraction…

Strongly Correlated Electrons · Physics 2012-02-29 K. Tomiyasu , K. Matsuhira , K. Iwasa , M. Watahiki , S. Takagi , M. Wakeshima , Y. Hinatsu , M. Yokoyama , K. Ohoyama , K. Yamada

We report a single-crystal neutron diffraction study of the layered $\rm Sr_2IrO_4$. This work unambiguously determines the magnetic structure of the system and reveals that the spin orientation rigidly tracks the staggered rotation of the…

Strongly Correlated Electrons · Physics 2013-04-23 Feng Ye , Songxue Chi , Bryan C. Chakoumakos , Jaime A. Fernandez-Baca , Tongfei Qi , G. Cao

The crystal structures of the A2B2O7-x Niobium-based pyrochlores Y2(Nb0.86Y0.14)2O6.91, CaYNb2O7, and Y2NbTiO7 are reported, determined by powder neutron diffraction. These compounds represent the first observation of B-site displacements…

Strongly Correlated Electrons · Physics 2009-02-02 T. M. McQueen , B. Muegge , Q. Huang , K. Noble , H. W. Zandbergen , R. J. Cava

We present time-of-flight inelastic neutron scattering measurements at low temperature on powder samples of the magnetic pyrochlore oxides Tb2Ti2O7 and Tb2Sn2O7. These two materials possess related, but different ground states, with…

Strongly Correlated Electrons · Physics 2014-05-01 J. Zhang , K. Fritsch , Z. Hao , B. V. Bagheri , M. J. P. Gingras , G. E. Granroth , P. Jiramongkolchai , R. J. Cava , B. D. Gaulin

We report a study of the geometrically frustrated magnetic material Tb2Sn2O7 by the positive muon spin relaxation technique. No signature of a static magnetically ordered state is detected while neutron magnetic reflections are observed in…

Strongly Correlated Electrons · Physics 2009-11-11 P. Dalmas de Reotier , A. Yaouanc , L. Keller , A. Cervellino , B. Roessli , C. Baines , A. Forget , C. Vaju , P. C. M. Gubbens , A. Amato , P. J. C. King

We report the magneto-dielectric response of single crystals of the spin-ice compound Dy2Ti2O7 down to 0.26 K. The dielectric constant under zero magnetic field exhibits a clear decrease reflecting the development of the local two-spins-in,…

Strongly Correlated Electrons · Physics 2009-11-11 Masafumi Saito , Ryuji Higashinaka , Yoshiteru Maeno

Muon-spin rotation (muSR) experiments are often used to study the magnetic field distribution in type-II superconductors in the vortex state. Based on the determination of the magnetic penetration depth it is frequently speculated---also…

Superconductivity · Physics 2011-10-31 B. M. Wojek , S. Weyeneth , S. Bosma , E. Pomjakushina , R. Puzniak

Considering certain interesting features in the previously reported 166Er Moessbauer effect and neutron diffraction data on the polycrystalline form of ErPd2Si2 crystallizing in ThCr2Si2-type tetragonal structure, we have carried out…

Strongly Correlated Electrons · Physics 2009-11-13 E. V. Sampathkumaran , Niharika Mohapatra , Kartik K Iyer , C. D. Cao , W. Loeser , G. Behr

The low temperature magnetic properties of pyrochlore compound Dy2Ti2O7 in magnetic fields applied along the [111] direction are reported. Below 1 K, a clear plateau has been observed in the magnetization process in the field range 2~9 kOe,…

Materials Science · Physics 2009-11-07 Kazuyuki Matsuhira , Zenji Hiroi , Takashi Tayama , Seishi Takagi , Toshiro Sakakibara

The geometrically-frustrated spin glass Y2Mo2O7 has been considered widely to be crystallographically ordered with a unique nearest neighbor magnetic exchange interaction, J. To test this assertion, we present x-ray-absorption…

Statistical Mechanics · Physics 2009-10-31 C. H. Booth , J. S. Gardner , G. H. Kwei , R. H. Heffner , F. Bridges , M. A. Subramanian

A detailed investigation of Ba$_2$MnGe$_2$O$_7$ was performed in its low-temperature magnetoelectric state combining neutron diffraction with magnetization measurements on single crystals. In the paramagnetic state at 10 K, polarized…

Strongly Correlated Electrons · Physics 2023-03-07 A. Sazonov , H. Thoma , R. Dutta , M. Meven , A. Gukasov , R. Fittipaldi , V. Granata , T. Masuda , B. Náfrádi , V. Hutanu

We present muon spin relaxation ($\mu$SR) and specific-heat versus temperature $C(T)$ measurements on polycrystalline and single-crystal samples of the pyrochlore magnet Yb$_2$Ti$_2$O$_7$. $C(T)$ exhibits a sharp peak at a $T_\mathrm{C}$ of…

Strongly Correlated Electrons · Physics 2014-05-28 Lieh-Jeng Chang , Martin R. Lees , Isao Watanabe , Adrian D. Hillier , Yukio Yasui , Shigeki Onoda

The series of magnetic rare earth pyrochlore stannates R2Sn2O7 (R = rare earth, except Ce and Pm) have been investigated by powder susceptibility measurements down to T =1.8 K. The results are compared to results for the analogous titanate…

Materials Science · Physics 2009-11-07 V. Bondah-Jagalu , S. T. Bramwell

We report a resonant inelastic X-ray scattering study on a single crystal of a non-stoichiometric pyrochlore iridate Tb$_{2+x}$Ir$_{2-x}$O$_{7-y}$ ($x \simeq 0.25$) that magnetically orders at $T_{\rm{N}}\simeq 50$ K. We find that the…

Strongly Correlated Electrons · Physics 2024-09-18 Q. Faure , A. Toschi , J. R. Soh , E. Lhotel , B. Detlefs , D. Prabhakaran , D. F. McMorrow , C. J. Sahle

We document the coexistence of ferro- and anti-ferromagnetism in pyrochlore $\rm Yb_2Ti_2O_7$ using three neutron scattering techniques on stoichiometric crystals: elastic neutron scattering shows a canted ferromagnetic ground state,…

Strongly Correlated Electrons · Physics 2020-10-27 A. Scheie , J. Kindervater , S. Zhang , H. J. Changlani , G. Sala , G. Ehlers , A. Heinemann , G. S. Tucker , S. M. Koohpayeh , C. Broholm

Rare-earth pyrochlores are known to exhibit exotic magnetic phenomena. We report a study of crystal growth and characterizations of a new rare-earth compound Er$_2$AlSbO$_7$, in which Al$^{3+}$ and Sb$^{5+}$ ions share the same positions…

The low-temperature thermodynamic properties of the frustrated pyrochlore Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$ have been studied using the single crystal of $x=0.005$ sitting in a long range ordered phase in the $x$-$T$ phase diagram. We observed…

Strongly Correlated Electrons · Physics 2017-04-25 H. Takatsu , T. Taniguchi , S. Kittaka , T. Sakakibara , H. Kadowaki

The spin ice system Dy$_{2}$Ti$_{2}$O$_{7}$ exhibits strong frequency-dependent spin-freezing at $\sim$ 16 K temperature. Although it has been a matter of discussion for years, the origin of this unusual spin freezing is still unknown. The…

Strongly Correlated Electrons · Physics 2022-04-06 Sheetal , C. S. Yadav
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