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Related papers: Complex oxide growth using simultaneous in situ RH…

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Pulsed Laser Deposition in molecular-beam epitaxy environment (Laser-MBE) has been used to grow high quality BaCuOx/CaCuO2 superlattices. In situ Reflection High Energy Electron Diffraction (RHEED) shows that the growth mechanism is…

Transition metal oxide heterostructures and interfaces host a variety of exciting quantum phases and can be grown with atomic-scale precision by utilising the intensity oscillations of $in$ $situ$ reflection high-energy electron diffraction…

Materials Science · Physics 2017-08-02 T. W. Zhang , Z. W. Mao , Z. B. Gu , Y. F. Nie , X. Q. Pan

We show that reflection high-energy electron diffraction (RHEED) can be used as a highly sensitive tool to track surface and resulting film stoichiometry in adsorption-limited molecular beam epitaxy of (001) SrTiO3 thin films. Even under…

Materials Science · Physics 2015-03-17 Adam P. Kajdos , Susanne Stemmer

The use of oxide materials in oxide electronics requires their controlled epitaxial growth. Recently, it was shown that Reflection High Energy Electron Diffraction (RHEED) allows to monitor the growth of oxide thin films even at high oxygen…

Materials Science · Physics 2009-11-07 D. Reisinger , B. Blass , J. Klein , J. B. Philipp , M. Schonecke , A. Erb , L. Alff , R. Gross

Reflection high-energy electron diffraction (RHEED) is a ubiquitous in situ molecular beam epitaxial (MBE) characterization tool. Although RHEED can be a powerful means for crystal surface structure determination, it is often used as a…

We present a pulsed laser deposition (PLD) system that can monitor growth by simultaneously using in situ optical spectroscopic ellipsometry (SE) and reflection high-energy electron diffraction (RHEED). The RHEED precisely monitors the…

Materials Science · Physics 2013-09-09 J. H. Gruenewald , J. Nichols , S. S. A. Seo

We have studied the growth dynamics and electronic properties of SrTiO3-d homoepitaxial films by pulsed laser deposition. We find the two dominant factors determining the growth mode are the kinetics of surface crystallization and…

Materials Science · Physics 2009-11-11 Akira Ohtomo , Harold Y. Hwang

We report on growth-mode transitions in the growth of SrRuO3 thin films on atomically flat Ti4+ single-terminated SrTiO3 (111) substrates, investigated by reflection high-energy electron diffraction and atomic force microscopy. Over the…

Materials Science · Physics 2010-02-03 Jaewan Chang , Yoon-Seok Park , Jong-Woo Lee , Sang-Koog Kim

Pulsed laser epitaxial growth is characterized by high instantaneous deposition rates that leads to the nucleation of transient islands, both on surface terraces, and on top of stable islands formed during previous deposition pulses. We…

Materials Science · Physics 2025-09-24 Jeffrey G. Ulbrandt , Xiaozhi Zhang , Randall L. Headrick

The homoepitaxial growth of initially flat surfaces has so far always led to surfaces which become rougher and rougher as the number of layers increases: even in systems exhibiting ``layer by layer'' growth the registry of the layers is…

Materials Science · Physics 2009-10-30 Joachim Jacobsen , James P. Sethna

Pulsed Laser Deposition (PLD) is widely used to grow epitaxial thin films of quantum materials such as complex oxides. Here, we use in-situ X-ray scattering to study homoepitaxy of SrTiO$_3$ by energetic (e-) and thermalized (th-) PLD. We…

The electrical conductance and RHEED intensities as a function of the coverage have been measured during Pb depositions at 105 K on Si(111)-(6x6)Au with up to 4.2 ML of annealed Pb. The experiments show the strong influence of used…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Z. Korczak , T. Kwapinski

Pulsed Laser Deposition (PLD) of homoepitaxial SrTiO3 <001> was studied with in-situ x-ray specular reflectivity and surface diffuse x-ray scattering. Unlike prior reflectivity-based studies, these measurements access both the time- and the…

Materials Science · Physics 2015-05-14 J. D. Ferguson , G. Arikan , D. S. Dale , A. R. Woll , J. D. Brock

Perovskite oxides such as LaFeO$_3$ are a well-studied family of materials that possess a wide range of useful and novel properties. Successfully synthesizing perovskite oxide samples usually requires a significant number of growth attempts…

Materials Science · Physics 2025-04-09 Patrick T. Gemperline , Rajendra Paudel , Rama K. Vasudevan , Ryan B. Comes

The subtle balance of electronic correlations, crystal field splitting and spin--orbit coupling in layered Ir$^{4+}$ oxides can give rise to novel electronic and magnetic phases. Experimental progress in this field relies on the synthesis…

Materials Science · Physics 2018-08-20 A. Gutiérrez-Llorente , L. Iglesias , B. Rodríguez-González , F. Rivadulla

Temperature dependent structural phase transitions of SrRuO3 thin films epitaxially grown on SrTiO3(001) single crystal substrates have been studied using high-resolution x-ray diffraction. In contrast to bulk SrRuO3, coherently strained…

Materials Science · Physics 2009-11-13 Arturas Vailionis , Wolter Siemons , Gertjan Koster

Understanding surface dynamics during epitaxial film growth is key to growing high quality materials with controllable properties. X-ray photon correlation spectroscopy (XPCS) using coherent x-rays opens new opportunities for in situ…

High quality epitaxial thin-films of EuTiO3 have been grown on the (001) surface of SrTiO3 using pulsed laser deposition. In situ x-ray reflectivity measurements reveal that the growth is two-dimensional and enable real-time monitoring of…

Materials Science · Physics 2007-05-23 Huan-Hua Wang , Aaron Fleet , Darren Dale , Yuri Suzuki , J. D. Brock

In situ reflective high-energy electron diffraction (RHEED) is widely used to monitor the surface crystalline state during thin-film growth by molecular beam epitaxy (MBE) and pulsed laser deposition. With the recent development of machine…

We present a systematic growth study of epitaxial RuO$_2$(110) and IrO$_2$(110) on TiO$_2$(110) substrates by pulsed laser deposition. We describe the main challenges encountered in the growth process, such as a deteriorating material flux…

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