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We use the lattice model of directed walks to investigate the conformational as well as the adsorption properties of a semiflexible homopolymer chain immersed in a good solvent in two and three dimensions. To account for the stiffness in…

Statistical Mechanics · Physics 2009-11-07 P. K. Mishra , S. Kumar , Y. Singh

Self-avoiding walks are studied on the 3-simplex fractal lattice as a model of linear polymer conformations in a dilute, non-homogeneous solution. A model is supplemented with bending energies and attractive-interaction energies between…

Statistical Mechanics · Physics 2023-02-21 Dušanka Marčetić

We study the entropic force due to a fluctuating semiflexible polymer that is grafted from one end and confined by a rigid and rough wall from the other end. We show how roughness of the wall modifies the entropic force. In addition to the…

Soft Condensed Matter · Physics 2021-11-17 Parvin Bayati , Leila Ghassab , Ali Najafi

Solutions of semiflexible polymers confined by repulsive planar walls are studied by density functional theory and Molecular Dynamics simulations, to clarify the competition between the chain alignment favored by the wall and the depletion…

Soft Condensed Matter · Physics 2016-05-25 Sergei A. Egorov , Andrey Milchev , Peter Virnau , Kurt Binder

We study a single flexible chain molecule grafted to a membrane which has pores of size slightly larger than the monomer size. On both sides of the membrane there is the same solvent. When this solvent is good, i.e. when the polymer is…

Soft Condensed Matter · Physics 2015-06-25 Hsiao-Ping Hsu , Peter Grassberger

The properties of a bundle of grafted semi-flexible living filaments in ideal solution facing an obstacle wall, under supercritical conditions, are explored. For this purpose, we make use of the discrete wormlike chain model characterized…

Soft Condensed Matter · Physics 2013-10-18 Jean-Paul Ryckaert , Sanoop Ramachandran

Polymers in confined spaces are compressed and have reduced conformational entropy, and will partially or fully escape from confinement if conditions are suitable. This is in particular the case for a polymer grafted in a pore. The escape…

Soft Condensed Matter · Physics 2024-08-05 CJ Bradly , EJ Janse van Rensburg

We consider a self-avoiding walk on the $d$-dimensional hypercubic lattice, terminally attached to an impenetrable hyperplane at which it can adsorb. When a force is applied the walk can be pulled off the surface and we consider the…

Statistical Mechanics · Physics 2017-02-01 EJ Janse van Rensburg , SG Whittington

We study a model of a semiflexible long chain polymer confined to a two-dimensional slit of width $w$, and interacting with the walls of the slit. The interactions with the walls are controlled by Boltzmann weights $a$ and $b$, and the…

Statistical Mechanics · Physics 2019-12-03 Nicholas R. Beaton , Leo Li , Jonathon Liu , Thomas Wong

We consider a self-avoiding walk model of polymer adsorption where the adsorbed polymer can be desorbed by the application of a force, concentrating on the case of the square lattice. Using series analysis methods we investigate the…

Statistical Mechanics · Physics 2015-06-17 Anthony J. Guttmann , Iwan Jensen , Stu G. Whittington

Lattice model of directed self avoiding walk has been solved analytically to investigate adsorption desorption phase transition behaviour of a semiflexible sequential copolymer chain on a two dimensional impenetrable surface perpendicular…

Statistical Mechanics · Physics 2010-02-23 Pramod Kumar Mishra

We present a Bethe approximation to study lattice models of linear polymers. The approach is variational in nature and based on the cluster variation method (CVM). We focus on a model with $(i)$ a nearest neighbor attractive energy…

Statistical Mechanics · Physics 2009-10-31 Stefano Lise , Amos Maritan , Alessandro Pelizzola

We study the directed polymer with fixed endpoints near an absorbing wall, in the continuum and in presence of disorder, equivalent to the KPZ equation on the half space with droplet initial conditions. From a Bethe Ansatz solution of the…

Disordered Systems and Neural Networks · Physics 2015-06-11 Thomas Gueudre , Pierre Le Doussal

The entropic pressure in the vicinity of a two dimensional square lattice polygon is examined as a model of the entropic pressure near a planar ring polymer. The scaling of the pressure as a function of distance from the polygon and length…

Statistical Mechanics · Physics 2015-06-16 F. Gassoumov , E. J. Janse van Rensburg

In this paper, we study the equilibrium properties of polymer chains end-tethered to a fluid membrane. The loss of conformational entropy of the polymer results in an inhomogeneous pressure field that we calculate for gaussian chains. We…

Soft Condensed Matter · Physics 2009-10-31 T. Bickel , C. Jeppesen , C. M. Marques

In order to study long chain polymers many lattice models accommodate a pulling force applied to a particular part of the chain, often a free endpoint. This is in addition to well-studied features such as energetic interaction between the…

Statistical Mechanics · Physics 2023-07-19 C. J. Bradly , A. L. Owczarek

Using molecular dynamic simulation, we study the stretching of an adsorbed homopolymer in a poor solvent with one end held at a distance $z_e$ from the substrate. We measure the vertical force $f$ on the end of the chain as a function of…

Soft Condensed Matter · Physics 2009-11-10 Franck Celestini , Thoma Frisch , Xabier Oyharcabal

We consider the entropy of polydisperse chains placed on a lattice. In particular, we study a model for equilibrium polymerization, where the polydispersivity is determined by two activities, for internal and endpoint monomers of a chain.…

Statistical Mechanics · Physics 2009-11-13 Minos A. Neto , Jürgen F. Stilck

We consider self-avoiding lattice polygons, in the hypercubic lattice, as a model of a ring polymer adsorbed at a surface and either being desorbed by the action of a force, or pushed towards the surface. We show that, when there is no…

Statistical Mechanics · Physics 2018-02-14 AJ Guttmann , EJ Janse van Rensburg , I Jensen , SG Whittington

The entropic force exerted by the Brownian fluctuations of a grafted semiflexible polymer upon a rigid smooth wall are calculated both analytically and by Monte Carlo simulations. Such forces are thought to play an important role for…

Soft Condensed Matter · Physics 2007-05-23 Azam Gholami , Jan Wilhelm , Erwin Frey