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Quantum spin liquids (QSLs), in which spins are highly entangled, have been considered a groundwork for generating exotic superconductivity.Despite numerous efforts, superconductivity emerging from QSLs has been unrealized in actual…

We present a detailed structural investigation of the organic superconductor $\kappa$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Br at temperatures $T$ from 9 to 300 K. Anomalies in the $T$ dependence of the lattice parameters are associated with a…

Materials Science · Physics 2016-08-16 A. U. B. Wolter , R. Feyerherm , E. Dudzik , S. Süllow , Ch. Strack , M. Lang , D. Schweitzer

CeTa$_7$O$_{19}$ is a recently found two-dimensional triangular lattice antiferromagnet without showing magnetic order. We grew high-quality CeTa$_7$O$_{19}$ single crystals and studied the low-temperature magnetic susceptibility, specific…

Strongly Correlated Electrons · Physics 2025-03-06 N. Li , A. Rutherford , Y. Y. Wang , H. Liang , Y. Zhou , Y. Sun , D. D. Wu , P. F. Chen , Q. J. Li , H. Wang , W. Xie , E. S. Choi , S. Z. Zhang , M. Lee , H. D. Zhou , X. F. Sun

We have developed a novel BEDT-TTF-based organic conductor, $\kappa$-(BEDT-TTF)$_2 m$-HOOCC$_6$H$_4$SO$_3$ ($\kappa$-$m$-SBA), and propose it as a candidate for altermagnet. Tight-binding band calculations of $\kappa$-$m$-SBA provide a…

Materials Science · Physics 2026-05-01 Kohei Tokura , Takato Masuta , Kazushi Aoyama , Hiroki Akutsu , Yasuhiro Nakazawa , Scott S. Turner

The conducting state of the quasi-two-dimensional organic conductor, $\alpha$-(BEDT-TTF)$_2$I$_3$, at ambient pressure is investigated with $^{13}$C NMR measurements, which separate the local electronic states at three nonequivalent…

Materials Science · Physics 2011-10-04 Michihiro Hirata , Kyohei Ishikawa , Kazuya Miyagawa , Kazushi Kanoda

A quantum spin liquid (QSL) would be an exotic stage for superconductivity. A promising candidate for a doped QSL is the organic triangular-lattice system, kappa-(BEDT-TTF)4Hg2:89Br8, which hosts a non-Fermi liquid and magnetism of a QSL…

Superconductivity · Physics 2022-06-16 K. Wakamatsu , Y. Ueno , K. Miyagawa , H. Taniguchi , K. Kanoda

We show that the anisotropy of the effective spin model for the dimer Mott insulator phase of $\kappa$-(BEDT-TTF)$_2X$ salts is dramatically different from that of the underlying tight-binding model. Intra-dimer quantum interference results…

Strongly Correlated Electrons · Physics 2018-07-11 B. J. Powell , E. P. Kenny , J. Merino

We performed $^{13}$C-NMR experiment and measured spin-lattice relaxation rate divided by temperature $1/T_{1}T$ near the superconducting (SC) transition temperature $T_{c}$ in $\kappa$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]Br ($\kappa$-Br salt),…

Superconductivity · Physics 2015-06-19 T. Kobayashi , Y. Ihara , Y. Saito , A. Kawamoto

We have in detail characterized the anisotropic charge response of the dimer Mott insulator $\kappa$-(BEDT-TTF)$_2$\-Cu$_2$(CN)$_3$ by dc conductivity, Hall effect and dielectric spectroscopy. At room temperature the Hall coefficient is…

We study the response of a two-channel Kondo quantum dot device proposed by Y. Oreg and D. Goldhaber-Gordon [Phys. Rev. Lett. {\bf 90}, 136602 (2003)] to a spin-bias applied across one of its channels formed by Fermi liquid reservoirs…

Mesoscale and Nanoscale Physics · Physics 2009-09-29 Prashant Sharma

The thermal conductivity $\kappa$ of the quasi-2D organic spin-liquid candidate EtMe$_3$Sb[Pd(dmit)$_2$]$_2$ (dmit-131) was measured at low temperatures, down to 0.07 K. We observe a vanishingly small residual linear term $\kappa_0/T$, in…

We investigated the local magnetism of the organic conductor, $\kappa$-(ET)$_{2}$Hg(SCN)$_{2}$Cl, with a quasi-triangular lattice of weakly dimerized molecules through $^{13}$C NMR spectroscopy. The NMR spectra and nuclear relaxation show…

Strongly Correlated Electrons · Physics 2026-03-31 M. Urai , K. Miyagawa , S. A. Torunova , N. Drichko , E. I. Zhilyaeva , K. Kanoda

EtMe$_3$Sb[Pd(dmit)$_2$]$_2$, an organic Mott insulator with nearly isotropic triangular lattice, is a candidate material for a quantum spin liquid, in which the zero-point fluctuations do not allow the spins to order. The itinerant gapless…

Strongly Correlated Electrons · Physics 2020-04-29 M. Yamashita , Y. Sato , T. Tominaga , Y. Kasahara , S. Kasahara , H. Cui , R. Kato , T. Shibauchi , Y. Matsuda

Measurements of the low-temperature thermal conductivity collected on insulators with geometrical frustration produce important experimental facts shedding light on the nature of quantum spin liquid composed of spinons. We employ a model of…

Strongly Correlated Electrons · Physics 2013-10-09 V. R. Shaginyan , A. Z. Msezane , K. G. Popov , G. S. Japaridze , V. A. Khodel

Resonant inelastic x-ray scattering at the N K edge reveals clearly resolved harmonics of the anion plane vibrations in the kappa-(BEDT-TTF)2Cu2(CN)3 spin-liquid insulator. Tuning the incoming light energy at the K edge of two distinct N…

The ground state of the quantum spin system kappa-(BEDT-TTF)2Cu2(CN)3 in which antiferromagnetically-interacting S=1/2 spins are located on a nearly equilateral triangular lattice attracts considerable interest both from experimental and…

We report the magnetic, magnetodielectric, and electric polarization properties of single crystals of the Co-based Kitaev Spin Liquid (KSL) candidate Na$_2$Co$_2$TeO$_6$ (NCTO). The sample shows magnetic transitions at 26 K, 16 K, and 5 K,…

We compare theoretical results for electron spin resonance (ESR) properties of the Heisenberg-Ising Hamiltonian with ESR experiments on the quasi-one-dimensional magnet Cu(py)$_2$Br$_2$ (CPB). Our measurements were performed over a wide…

Resistivity measurements have been performed on a low (LR)- and high (HR)-resistance variant of the kappa-(BEDT-TTF)_2Cu[N(CN)_2]Br superconductor. While the HR sample was synthesized following the standard procedure, the LR crystal is a…

Strongly Correlated Electrons · Physics 2009-11-10 C. Strack , C. Akinci , B. Wolf , M. Lang , J. A. Schlueter , J. Wosnitza , D. Schweitzer , J. Mueller

Identifying the elusive spinon excitations in quantum spin liquid (QSL) materials is what scientists have long sought for. Recently, thermal conductivity ($\kappa$) has emerged to be a decisive probe because the fermionic nature of spinons…

Strongly Correlated Electrons · Physics 2024-05-24 N. Li , A. Brassington , M. F. Shu , Y. Y. Wang , H. Liang , Q. J. Li , X. Zhao , P. J. Baker , H. Kikuchi , T. Masuda , G. Duan , C. Liu , H. Wang , W. Xie , R. Zhong , J. Ma , R. Yu , H. D. Zhou , X. F. Sun