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A few organic conductors show a diversity of exciting properties like Mott insulating behaviour, spin liquid, antiferromagnetism, bad metal or unconventional superconductivity controlled by small changes in temperature, pressure or chemical…

Strongly Correlated Electrons · Physics 2014-02-05 Johannes Ferber , Kateryna Foyevtsova , Harald O. Jeschke , Roser Valenti

We present high-resolution measurements of the coefficient of thermal expansion $\alpha (T)=\partial \ln l(T)/\partial T$ of the quasi-twodimensional (quasi-2D) salts $\kappa$-(BEDT-TTF)$_2$X with X = Cu(NCS)$_2$, Cu[N(CN)$_2$]Br and…

Superconductivity · Physics 2009-11-07 J. Müller , M. Lang , F. Steglich , J. A. Schlueter , A. M. Kini , T. Sasaki

The static and dynamic local spin susceptibility of the organic Mott insulator $\kappa$-(ET)$_2$Cu$_2$(CN)$_3$, a model material of the spin- 1/2 triangular lattice, is studied by $^{13}$C NMR spectroscopy from room temperature down to 20…

Strongly Correlated Electrons · Physics 2007-05-23 Yasuhiro Shimizu , Kazuya Miyagawa , Kazushi Kanoda , Maesato Mitsuhiko , Gunzi Saito

We explore orbital dynamics in the spin liquid candidate Ba3CuSb2O9 using multi-frequency electron spin resonance. We prepared two high quality single crystals. The crystal with a slight copper deficiency shows a structural phase transition…

Strongly Correlated Electrons · Physics 2015-12-09 Yibo Han , Masayuki Hagiwara , Takehito Nakano , Yasuo Nozue , Kenta Kimura , Mario Halim , Satoru Nakatsuji

Quantum spin liquids attract great interest due to their exceptional magnetic properties characterized by the absence of long-range order down to low temperatures despite the strong magnetic interaction. Commonly, these compounds are…

Strongly Correlated Electrons · Physics 2018-05-01 Martin Dressel , Andrej Pustogow

We present the results of our $^{13}$C NMR study of the quasi-two-dimensional organic conductor $\theta$-(BEDT-TTF)$_2$I$_{3}$ under pressure, which is suggested to be a zero-gap conductor by transport measurements. We found that NMR spin…

Mesoscale and Nanoscale Physics · Physics 2010-05-27 K. Miyagawa , M. Hirayama , M. Tamura , K. Kanoda

A high frequency (111.2-420 GHz) electron spin resonance study of the inter-layer (perpendicular) spin diffusion as a function of pressure and temperature is presented in the conducting phases of the layered organic compounds,…

Strongly Correlated Electrons · Physics 2013-09-24 Á. Antal , T. Fehér , E. Tátrai-Szekeres , F. Fülöp , B. Náfrádi , L. Forró , A. Jánossy

The thermal conductivity of organic superconductor kappa-(BEDT-TTF)2Cu(NCS)2 (Tc =10.4 K) has been studied in a magnetic field rotating within the 2D superconducting planes with high alignment precision. At low temperatures (T < 0.5 K), a…

Superconductivity · Physics 2009-11-07 Koichi Izawa , Hidemasa Yamaguchi , Takahiko Sasaki , Yuji Matsuda

Recent studies of organic molecular solids are highlighted by their complex phase diagram and light-induced phenomena, such as Mott insulator, spin liquid phase, and superconductivity. However, a discrepancy between experimental observation…

Strongly Correlated Electrons · Physics 2024-12-25 Dongbin Shin , Fabijan Pavošević , Nicolas Tancogne-Dejean , Michele Buzzi , Emil Viñas Boström , Angel Rubio

The polarized optical reflectance spectra of the quasi two dimensional organic correlated electron system $\kappa$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]$Y$, $Y =$ Br and Cl are measured in the infrared region. The former shows the…

Superconductivity · Physics 2007-05-23 T. Sasaki , I. Ito , N. Yoneyama , N. Kobayashi , N. Hanasaki , H. Tajima , T. Ito , Y. Iwasa

We have studied the interlayer resistivity of the prototypical quasi-two-dimensional organic superconductor $\kappa$-(BEDT-TTF)$_2$Cu(NCS)$_2$ as a function of temperature, current and magnetic field, within the superconducting state. We…

Since the first observation of weak ferromagnetism in the charge-transfer salt kappa-(BEDT-TTF)2-Cu[N(CN)2]Cl [U. Welp et al., Phys. Rev. Lett. 69, 840 (1992)], no further evidence of ferromagnetism in this class of organic materials has…

We present microscopic magnetic properties of a two dimensional triangular lattice Sc2Ga2CuO7, consisting of single and double triangular Cu planes. A Curie-Weiss temperature theta_CW = --44 K and an antiferromagnetic (AFM) exchange…

Strongly Correlated Electrons · Physics 2017-12-06 P. Khuntia , R. Kumar , A. V. Mahajan , M. Baenitz , Y. Furukawa

It has been more than 40 years since superconductivity was discovered in organic conductors, and the way scientists view organic superconductors has changed over time. At first, the fact that organic conductors exhibit superconductivity was…

Superconductivity · Physics 2023-07-20 Hiroshi Oike , Hiromi Taniguchi , Kazuya Miyagawa , Kazushi Kanoda

The Mott insulator $\kappa$-(BEDT-TTF)$_2$Ag$_2$(CN)$_3$ forms a highly-frustrated triangular lattice of $S=1/2$ dimers with a possible quantum-spin-liquid state. Our experimental and numerical studies reveal the emergence of a slight…

Nuclear spin-lattice (1/T1) and spin-spin (1/T2) relaxation rates of the cation sites of a quantum spin-liquid candidate b'-EtMe3Sb[Pd(dmit)2]2 and its deuterated sample are presented. The enhanced 1/T1 of 1H and 2D are well analyzed…

Strongly Correlated Electrons · Physics 2018-01-18 S. Fujiyama , R. Kato

The layered triangular lattice owing to $1:2$ order of $B$ and $B'$ sites in the triple perovskite $A_3 B B'_2$O$_9$ family provides an enticing domain for exploring the complex phenomena of quantum spin liquids (QSLs). We report a…

Strongly Correlated Electrons · Physics 2024-08-07 K. Bhattacharya , S. Mohanty , A. D. Hillier , M. T. F. Telling , R. Nath , M. Majumder

Low-dimensional organic conductors show a rich phase diagram, which has, despite all efforts, still some unexploed regions. Charge ordered phases present in many compounds of the (TMTTF)$_2 X$ family are typically studied with their unique…

A Hubbard model at half-filling on an anisotropic triangular lattice has been proposed as the minimal model to describe conducting layers of $\kappa-(BEDT-TTF)_2X$ organic materials. The model interpolates between the square lattice and…

Superconductivity · Physics 2016-04-20 Shan-Wen Tsai , J. B. Marston

The metal-organic-framework (MOF) compound Cu$_3$(HOTP)$_2$, a.k.a. Cu$_3$(HHTP)$_2$, is a small-gap semiconductor containing a kagome lattice of antiferromagnetically coupled $S$=1/2 Cu$^\mathrm{II}$ spins with intra-layer nearest-neighbor…

Strongly Correlated Electrons · Physics 2024-11-28 F. L. Pratt , D. Lopez-Alcala , V. Garcia-Lopez , M. Clemente-Leon , J. J. Baldovi , E. Coronado