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Dual-comb spectroscopy has emerged as an indispensable analytical technique in applications that require high resolution and broadband coverage within short acquisition times. Its experimental realization, however, remains hampered by…

Instrumentation and Detectors · Physics 2019-12-02 Łukasz A. Sterczewski , Aleksandra Przewłoka , Wawrzyniec Kaszub , Jarosław Sotor

We show how two frequency combs $\mathcal{E}_1$, $\mathcal{E}_2$ can be used to measure single-photon, two-photon absorption (TPA), and Raman resonances in a molecule with three electronic bands, by detecting the radio frequency modulation…

Chemical Physics · Physics 2014-08-12 Rachel Glenn , Shaul Mukamel

Chemical imaging enabled by Raman processes is crucial to investigating biological and chemical samples in a label-free manner. Stimulated Raman spectroscopy (SRS) overcomes the key limitation associated with low signal levels in…

Optics · Physics 2026-03-25 Florian M. Schweizer , Hannah Terrasa , Manish Garg

In this paper, we describe two complementary non-linear spectroscopy methods which both allow to achieve Doppler-free spectra of atomic gases. First, saturated absorption spectroscopy is used to investigate the structure of the $5{\rm…

Physics Education · Physics 2015-05-13 V. Jacques , B. Hingant , A. Allafort , M. Pigeard , J. -F. Roch

Broadband precision spectroscopy is indispensable for providing high fidelity molecular parameters for spectroscopic databases. We have recently shown that mechanical Fourier transform spectrometers based on optical frequency combs can…

Instrumentation and Detectors · Physics 2018-05-09 Lucile Rutkowski , Piotr Maslowski , Alexandra C. Johansson , Amir Khodabakhsh , Aleksandra Foltynowicz

Electromagnetic scattering in accelerating reference frames inspires a variety of phenomena, requiring employment of general relativity for their description. While the quasi-stationary field analysis could be applied to slowly-accelerating…

Classical Physics · Physics 2017-02-21 Vitali Kozlov , Dmitrii Filonov , Yefim Yankelevich , Pavel Ginzburg

In this paper, we introduce an all-fibered dual-comb spectrometer based on a new design of highly nonlinear fiber to efficiently convert frequency combs from 1.55 micron to 2 micron We show that our spectrometer can be used to measure…

Dual-comb spectroscopy has demonstrated remarkable capabilities for rapid and sensitive measurements; however, significant challenges still exist in generating high-power, mutually coherent mid-infrared combs. Here we demonstrate that a…

Dual-comb spectroscopy utilizes two sets of comb lines with slightly different comb-tooth-spacings, and optical spectral information is acquired by measuring the radio-frequency beat notes between the sets of comb lines. It holds the…

Optics · Physics 2016-09-13 Xin Zhao , Guoqing Hu , Bofeng Zhao , Cui Li , Yingling Pan , Ya Liu , Takeshi Yasui , Zheng Zheng

Two-photon resonance transition technology has been proven to have a wide range of applications,it's limited by the available wavelength of commercial lasers.The application of optical comb technology with direct two-photon transition…

Atomic Physics · Physics 2022-04-27 Lin Dan , Hao Xu , Ping Guo , Jianye Zhao

Frequency combs have revolutionized the field of optical spectroscopy, enabling researchers to probe molecular systems with a multitude of accurate and precise optical frequencies. While there have been tremendous strides in direct…

I review the method of Doppler tomography which translates binary-star line profiles taken at a series of orbital phases into a distribution of emission over the binary. I begin with a discussion of the basic principles behind Doppler…

Astrophysics · Physics 2007-05-23 T. R. Marsh

With transfer matrix theory, we study the transmission of a distributed Bragg reflector (DBR) with two dielectric gratings on top and on the bottom. Owing to the diffraction of the two gratings, the transmission shows a comb-like spectrum…

Optics · Physics 2015-05-22 Xiaobo Zhao , Bingsuo Zou , Yongyou Zhang

Dual-comb spectroscopy in the ultraviolet (UV) and visible would enable broad bandwidth electronic spectroscopy with unprecedented frequency resolution. However, there are significant challenges in generation, detection and processing of…

Specific features of nonlinear interference processes at quantum transitions in near- and fully-resonant optically-dense Doppler-broadened medium are studied. The feasibility of overcoming of the fundamental limitation on a…

Quantum Physics · Physics 2009-11-11 A. K. Popov , S. A. Myslivets , Thomas F. George

Dual-comb spectroscopy enables broadband analysis of key molecules with unparalleled frequency resolution and exceptional signal-to-noise ratios across various spectral regions. However, fully harnessing its potential for broadband…

Dual-comb interferometry is a measurement technique that uses two laser frequency combs to retrieve complex spectra in a line-by-line basis. This technique can be implemented with electro-optic frequency combs, offering intrinsic mutual…

Optics · Physics 2016-09-21 Vicente Duran , Peter A. Andrekson , Victor Torres-Company

Ultrabroadband electro-optic sampling with few-cycle optical pulses is known to be an extremely sensitive technique to detect electric field amplitudes. By combining this method with dual-comb spectroscopy and with a new class of ultrafast…

Improvements to dual-comb interferometers will benefit precision spectroscopy and sensing, distance metrology, tomography, telecommunications etc. A specific requirement of such interferometers is to enforce mutual coherence between the two…

Optics · Physics 2018-08-10 Zaijun Chen , Ming Yan , Theodor W. Hänsch , Nathalie Picqué

The frequency correlation properties of the radiation from an atom in a strong field in resonance with neighboring transitions are considered. It is shown that the difference in frequency correlation in two-photon and stepwise processes…

Quantum Physics · Physics 2007-05-23 T. Ya. Popova , A. K. Popov , S. G. Rautian , A. A. Feoktistov