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Dual-comb spectroscopy has been proven a powerful tool in molecular characterization, which remains challenging to implement in the mid-infrared region due to difficulties in the realization of two mutually locked comb sources and efficient…

Frequency comb based multidimensional coherent spectroscopy is a novel optical method that enables high resolution measurement in a short acquisition time. The method's resolution makes multidimensional coherent spectroscopy relevant for…

Atomic Physics · Physics 2018-06-13 Bachana Lomsadze , Steven T. Cundiff

Detector nonlinearity is an important factor limiting the maximal power and hence the signal-to-noise ratio (SNR) in dual-comb interferometry. To increase the SNR without overwhelming averaging time, specific experimental conditions must be…

High resolution and fast detection of molecular vibrational absorption is important for organic synthesis, pharmaceutical process and environmental monitoring, and is enabled by mid-infrared (mid-IR) laser frequency combs via dual-comb…

Hyperspectral imaging is a technique that allows for the creation of multi-color images. At terahertz wavelengths, it has emerged as a prominent tool for a number of applications, ranging from non-ionizing cancer diagnosis and…

A multichannel dual-comb spectroscopy (DCS) approach for high-resolution, broadband spectral measurements is presented, demonstrating its effectiveness in studying complex atomic systems. By implementing a photodetector array, we enhance…

Atomic Physics · Physics 2025-03-14 R. Aramyan , O. Tretiak , S. S. Sahoo , D. Budker

We demonstrate a simple system for dual-comb spectroscopy based on two inherently coherent optical frequency combs generated via seeded parametric down-conversion. The inbuilt coherence is established by making the two combs share a common…

Optics · Physics 2024-08-13 Mikhail Roiz , Santeri Larnimaa , Touko Uotila , Mikko Narhi , Markku Vainio

We propose a scheme for realizing broadband and tunable transmission non-reciprocity by utilizing two-photon near-resonant transitions in thermal atoms as single-photon far-detuned transitions can be eliminated. Our basic idea is to largely…

Quantum Physics · Physics 2024-02-12 Hui-Min Zhao , Di-Di Zheng , Xiao-Jun Zhang , Jin-Hui Wu

Spectral analysis is one of the most powerful technologies for studying and understanding matter. As the devices for spectral analysis, spectrometers are widely used in material detection, isotope analysis, trace gas detection, and the…

It is proposed a few-atom Doppler-sensitive absorption spectroscopy scheme resolving the long-standing dilemma regarding the nature of an atomic quantum translational motion (superpositional or non-superpositional) and its measurement…

Quantum Physics · Physics 2025-06-17 A. Zh. Muradyan

We have carried out dual-comb spectroscopy and observed in a simultaneous acquisition a 140-THz-wide spectrum from 1.0 to 1.9 {\mu}m using two fiber-based frequency combs phase-locked to each other. This ultra-broad wavelength bandwidth is…

Fourier-transform spectroscopy is an indispensable tool for analyzing chemical samples in scientific research as well as chemical and pharmaceutical industries. Recently, its measurement speed, sensitivity, and precision have been shown to…

Optics · Physics 2025-05-06 Takuro Ideguchi , Tasuku Nakamura , Yohei Kobayashi , Keisuke Goda

Doppler tomography is a method to compute the emissivity distribution within the co-rotating frames of binary stars from observations of their emission line profiles at multiple orbital phases. A key assumption of the method as it is…

Solar and Stellar Astrophysics · Physics 2021-12-08 T. R. Marsh

Continuous wave (CW) lasers are the enabling technology for producing ultracold atoms and molecules through laser cooling and trapping. The resulting pristine samples of slow moving particles are the de facto starting point for both…

Atomic Physics · Physics 2016-10-19 A. M. Jayich , X. Long , W. C. Campbell

A phase-stabilized femtosecond laser comb is directly used for high-resolution spectroscopy and absolute optical frequency measurements of one- and two-photon transitions in laser-cooled \rb atoms. Absolute atomic transition frequencies,…

Atomic Physics · Physics 2009-11-11 Adela Marian , Matthew C. Stowe , Daniel Felinto , Jun Ye

A chirped-pulse interleaving method is reported for generation of dual optical frequency combs based on electro-optic phase modulators (EOM) in a free-running all-fiber based system. Methods are discussed to easily modify the linear chirp…

Dual-comb interferometry utilizes two optical frequency combs to map the optical field's spectrum to a radio-frequency signal without using moving parts, allowing improved speed and accuracy. However, the method is compounded by the…

Frequency comb-referenced measurements of sub-Doppler laser saturation dip absorption lines in the $v_1+v_3$ band of acetylene near $1.5\,\mu \mathrm{m}$ are reported. These measurements include transitions involving higher rotational…

Chemical Physics · Physics 2020-03-10 Sylvestre Twagirayezu , Gregory E. Hall , Trevor J. Sears

Dual-comb spectroscopy allows for the rapid, multiplexed acquisition of high-resolution spectra without the need for moving parts or low-resolution dispersive optics. This method of broadband spectroscopy is most often accomplished via…

Dual-frequency comb spectroscopy permits broadband precision spectroscopic measurements with short acquisition time. A dramatic improvement of the maximal spectral bandwidth and the minimal measurement time can be expected when the lasers'…