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Marcasite-type compounds have been proposed as promising hosts of exotic magnetic quantum states, yet experimental realizations in stoichiometric, disorder-free systems remain limited. Here, we report the high-pressure stabilization and…

We show by means of density functional calculations that CaMn$_{2}$Sb$_{2}$ is very close to a mean-field critical point known for the classical Heisenberg model on the honeycomb lattice. Three entirely different long range ordered magnetic…

Strongly Correlated Electrons · Physics 2013-09-17 I. I. Mazin

Lanthanide (Ln) based LnSbTe materials have garnered significant attention due to rich interplay of long range magnetic ordering and topological properties, driven by unique crystalline symmetry, 4f electron interactions, and pronounced…

A new crystal chemical method was used to calculate the sign and strength not only of the nearest-neighbor (NN)interactions, but also of the next-nearest-neighbor (NNN) ones in tetragonal compounds Zn2(VO)(PO4)2 (I),(VO)(H2PO4)2 (II),…

Materials Science · Physics 2007-05-23 L. M. Volkova , S. A. Polyshchuk

The recent discoveries of proximate quantum spin-liquid compounds and their potential application in quantum computing informs the search for new candidate materials for quantum spin-ice and spin-liquid physics. While the majority of such…

Strongly Correlated Electrons · Physics 2019-01-16 K. M. Taddei , L. Sanjeewa , J. W. Kolis , A. S. Sefat , C. de la Cruz , D. M. Pajerowski

We present observations of highly frustrated quasi two-dimensional (2D) magnetic correlations in the honeycomb lattice layers of the S$_{eff}$ = 1/2 compound $\gamma$-BaCo$_2$(PO$_4$)$_2$ ($\gamma$-BCPO). Specific heat shows a broad peak…

Strongly Correlated Electrons · Physics 2018-04-18 H. S. Nair , J. M. Brown , E. Coldren , G. Hester , M. P. Gelfand , A. Podlesnyak , Q. Huang , K. A. Ross

Magnetic frustration and low dimensionality can prevent long range magnetic order and lead to exotic correlated ground states. SrDy$_2$O$_4$ consists of magnetic Dy$^{3+}$ ions forming magnetically frustrated zig-zag chains along the c-axis…

A non-technical introduction to the theory of magnets with strong geometric frustration is given, concentrating on magnets on corner-sharing (kagome, pyrochlore, SCGO and GGG) lattices. Their rich behaviour is traced back to a large…

Statistical Mechanics · Physics 2009-10-31 R. Moessner

For temperatures T well above the ordering temperature T*=3.0+-0.2K the magnetic properties of the metal-organic material Mn[C10H6(OH)(COO)]2x2H20 built from Mn^2+ ions and 3-hydroxy-2-naphthoic anions can be described by a S=5/2 quantum…

The structural and magnetic properties of the hexagonal four-layer form of SrMnO$_3$ have been investigated by combining magnetization measurements, electron diffraction and high-resolution synchrotron X-ray and neutron powder diffraction.…

Strongly Correlated Electrons · Physics 2007-05-23 A. Daoud-Aladine , C. Martin , L. C. Chapon , M. Hervieu , K. S. Knight , M. Brunelli , P. G. Radaelli

A series of polycrystalline samples of Sr2-xIrO4 have been synthesized by a solid-state reaction method. The crystal structure of this doped system can be explained on the basis of the extended nature of 5d electrons and strontium vacancies…

Strongly Correlated Electrons · Physics 2016-11-09 Jimei Kong , S. L. Liu , Jie Cheng , Haiyun Wang , Xing ao Li , Z. H. Wang

Materials with strongly correlated electrons exhibit physical properties that are often difficult to predict as they result from the interactions of large numbers of electrons combined with several quantum degrees of freedom. The layered…

Depending on the crystal growth conditions, an orthorhombic (O-type) or a tetragonal (T-type) structure can be found in the solid solution Cs2CuCl4-xBrx (0 < x < 4). Here we present measurements of the temperature-dependent magnetic…

Detailed studies of the magnetoresistance of alpha-(ET)2KHg(SCN)4 and alpha-(ET)2TlHg(SCN)4 as a function of temperature, magnetic field strength, and field orientation are reported. Below 15 K, the temperature dependence of the…

Condensed Matter · Physics 2007-05-23 J. S. Qualls , J. S. Brooks , S. Uji , T. Terashima , C. Terakura , H. Aoki , L. K. Montgomery

A frustrated system is one whose symmetry precludes the possibility that every pairwise interaction (``bond'') in the system can be satisfied at the same time. Such systems are common in all areas of physical and biological science. In the…

Disordered Systems and Neural Networks · Physics 2009-11-07 Steven T. Bramwell , Michel J. -P. Gingras

The results of dc magnetization, heat capacity, electrical resistivity (rho) and magnetoresistance measurements are reported in detail for the compounds, RCuAs2 for R= Pr, Nd, Sm, Gd, Tb, Dy, Ho, and Er, crystallizing in HfCuSi2-type…

Materials Science · Physics 2009-11-10 Kausik Sengupta , S. Rayaprol , E. V. Sampathkumaran , Th. Doert , J. P. F. Jemetio

Pyrochlores offer an ideal playground to investigate the magnetic ground state of frustrated magnetic systems. In this class of materials, competition between various magnetic interactions remains frustrated and prevents an ordered magnetic…

Strongly Correlated Electrons · Physics 2022-10-06 Karan Singh , Dheeraj Ranaut , G. Sharma , K. Mukherjee

We report the magnetic structure and properties of a thiocyanate-based honeycomb magnet [Na(OH$_2$)$_3$]Mn(NCS)$_3$ which crystallises in the unusual low-symmetry trigonal space group $P\overline{3}$. Magnetic measurements on powder samples…

We report the magnetic properties of compounds in the KBaRE(BO3)2 family (RE= Sm, Eu, Gd, Tb, Dy, Ho, Er, Tm, Yb), materials with a planar triangular lattice composed of rare earth ions. The samples were analyzed by x-ray diffraction and…

Strongly Correlated Electrons · Physics 2016-11-28 M. B. Sanders , F. A. Cevallos , R. J. Cava

Frustrated magnets are one class of fascinating materials that host many intriguing phases such as spin ice, spin liquid and complex long-range magnetic orderings at low temperatures. In this work we use first-principles calculations to…

Materials Science · Physics 2019-08-07 Yue-Wen Fang , Ruihan Yang , Hanghui Chen
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