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Unveiling unconventional magnetism at the surface of Sr$_2$RuO$_4$

Strongly Correlated Electrons 2024-03-02 v1 Materials Science

Abstract

Materials with strongly correlated electrons exhibit physical properties that are often difficult to predict as they result from the interactions of large numbers of electrons combined with several quantum degrees of freedom. The layered oxide perovskite Sr2_2RuO4_4 is a strongly correlated electron material that has been intensively investigated since its discovery due to its unusual physical properties. Whilst recent experiments have reopened the debate on the exact symmetry of the superconducting state in Sr2_2RuO4_4, a deeper understanding of the Sr2_2RuO4_4 normal state appears crucial as this is the background in which electron pairing occurs. Here, by using low-energy muon spin spectroscopy we discover the existence of magnetism at the surface of Sr2_2RuO4_4 in its normal state. We detect static weak dipolar fields yet manifesting below a relatively high onset temperature larger than 50 K, which reveals the unconventional nature of the observed magnetism. We relate the origin of this phase breaking time reversal symmetry to electronic ordering in the form of orbital loop currents that originate at the reconstructed Sr2_2RuO4_4 surface. Our observations set a reference for the discovery of the same magnetic phase in other materials and unveil an electronic ordering mechanism that can influence unconventional electron pairing with broken time reversal symmetry in those materials where the observed magnetic phase coexists with superconductivity.

Keywords

Cite

@article{arxiv.2402.18359,
  title  = {Unveiling unconventional magnetism at the surface of Sr$_2$RuO$_4$},
  author = {Rosalba Fittipaldi and Roman Hartmann and Maria Teresa Mercaldo and Sachio Komori and Anders Bjørlig and Wonshik Kyung and Yuuki Yasui and Takuto Miyoshi and Linde Olde-Olthof and Carla Palomares-Garcia and Veronica Granata and Itai Keren and Wataru Higemoto and Andreas Suter and Thomas Prokscha and Alfonso Romano and Canio Noce and Changyoung Kim and Yoshiteru Maeno and Elke Scheer and Beena Kalisky and Jason W. A. Robinson and Mario Cuoco and Zaher Salman and Antonio Vecchione and Angelo Di Bernardo},
  journal= {arXiv preprint arXiv:2402.18359},
  year   = {2024}
}

Comments

20 pages, 5 figures