English

Structural anomalies and short-range magnetic correlations in the orbitally degenerated system Sr$_2$VO$_4$

Strongly Correlated Electrons 2015-09-02 v1

Abstract

We report on the electronic ground state of a layered perovskite vanadium oxide Sr2_2VO4_4 studied by the combined use of synchrotron radiation x-ray diffraction (SR-XRD) and muon spin rotation/relaxation (μ\muSR) techniques, where μ\muSR measurements were extended down to 30 mK. We found an intermediate orthorhombic phase between Tc2T_{\rm c2} \sim~130 K and Tc1T_{\rm c1} \sim~100 K, whereas a tetragonal phase appears for T>Tc2T > T_{\rm c2} and T<Tc1T < T_{\rm c1}. The absence of long-range magnetic order was confirmed by μ\muSR at the reentrant tetragonal phase below Tc1T_{\rm c1}, where the relative enhancement in the cc-axis length versus that of the aa-axis length was observed. However, no clear indication of the lowering of the tetragonal lattice symmetry with superlattice modulation, which is expected in the orbital order state with superstructure of dyzd_{yz} and dzxd_{zx} orbitals, was observed by SR-XRD below Tc1T_{\rm c1}. Instead, it was inferred from μ\muSR that a magnetic state developed below Tc0T_{\rm c0} \sim~10 K, which was characterized by the highly inhomogeneous and fluctuating local magnetic fields down to 30 mK. We argue that the anomalous magnetic ground state below Tc0T_{\rm c0} originates from the coexistence of ferromagnetic and antiferromagnetic correlations.

Keywords

Cite

@article{arxiv.1507.04139,
  title  = {Structural anomalies and short-range magnetic correlations in the orbitally degenerated system Sr$_2$VO$_4$},
  author = {Ichihiro Yamauchi and Kazuhiro Nawa and Masatoshi Hiraishi and Masanori Miyazaki and Akihiro Koda and Kenji M. Kojima and Ryosuke Kadono and Hironori Nakao and Reiji Kumai and Youichi Murakami and Hiroaki Ueda and Kazuyoshi Yoshimura and Masashi Takigawa},
  journal= {arXiv preprint arXiv:1507.04139},
  year   = {2015}
}

Comments

8 pages, 8 figures, accepted for publication in Physical Review B