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Every realistic instance of a percolation problem is faced with some degree of polydispersity, e.g., the pore-size distribution of an inhomogeneous medium, the size distribution of filler particles in composite materials, or the vertex…

Statistical Mechanics · Physics 2025-06-16 Fabian Coupette , Tanja Schilling

We study the effect of physical confinement on the capillary infiltration of polymers into cylindrical nanopores using molecular dynamics simulations. In particular, we probe whether the critical contact angle above which capillary rise…

Soft Condensed Matter · Physics 2018-09-03 David J. Ring , Robert A. Riggleman , Daeyeon Lee

Configurations of a single semiflexible polymer is studied when it is pushed into a nanochannel in the case where the polymer persistence length $l_p$ is much longer than the channel diameter $D$, i.e. $l_p/D \gg 1$. Using numerical…

Statistical Mechanics · Physics 2017-06-28 Yumino Hayase , Takahiro Sakaue , Hiizu Nakanishi

We study the effect of volumetric constraints on the structure and electronic transport properties of distilled water in a nanopore with embedded electrodes. Combining classical molecular dynamics simulations with quantum scattering theory,…

Soft Condensed Matter · Physics 2014-01-30 P. Boynton , M. Di Ventra

We simulate entangled linear polymers in free-standing thin film geometries where the confining dimension is on the same scale or smaller than the bulk chain dimensions. We compare both film-averaged and layer-resolved, spatially…

Soft Condensed Matter · Physics 2016-08-24 Daniel M. Sussman

The structure of flexible polymers endgrafted in cylindrical pores of diameter D is studied as a function of chain length N and grafting density \sigma, assuming good solvent conditions. A phenomenological scaling theory, describing the…

Soft Condensed Matter · Physics 2009-11-11 D. I. Dimitrov , A. Milchev , K. Binder

The physics of diffusion phenomena in nano and micro channels has attracted a lot of attention in recent years, due to its close connection with many technological, medical and industrial applications. In the present paper we employ a…

Soft Condensed Matter · Physics 2015-09-30 Umberto Marini Bettolo Marconi , Paolo Malgaretti , Ignacio Pagonabarraga

We study the dynamics of a knot in a semiflexible polymer confined to a narrow channel of width comparable to the polymers' persistence length. Using a combination of Brownian dynamics simulations and a coarse-grained stochastic model, we…

Soft Condensed Matter · Physics 2008-08-14 Wolfram Mobius , Erwin Frey , Ulrich Gerland

The 1+1 dimensional directed polymers in a Poissonean random environment is studied. For two polymers of maximal length with the same origin and distinct end points we establish that the point of last branching is governed by the exponent…

Mathematical Physics · Physics 2007-05-23 Patrik L. Ferrari , Herbert Spohn

A number of recent experiments have provided detailed observations of the configurations of long DNA strands under nano-to-micrometer sized confinement. We therefore revisit the problem of an excluded volume polymer chain confined between…

Soft Condensed Matter · Physics 2011-03-23 Debasish Chaudhuri , Bela Mulder

By quantitative studies of statistics of polymer stretching in a random flow and of a flow field we demonstrate that the stretching of polymer molecules in a 3D random flow occurs rather sharply via the coil-stretch transition at the value…

Chaotic Dynamics · Physics 2009-11-10 S. Gerashchenko , C. Chevallard , V. Steinberg

Describing the diffusion of particles through crowded, confined environments with which they can interact is of considerable biological and technological interest. Under conditions where the confinement dimensions become comparable to the…

Soft Condensed Matter · Physics 2009-11-13 Mark L. Henle , Brian DiDonna , Christian D. Santangelo , Ajay Gopinathan

We characterize the motion of charged as well as neutral tracers, in an electrolyte embedded in a varying section channel. We exploit a set of systematic approximations that allows us to simplify the problem, yet capturing the essential of…

Soft Condensed Matter · Physics 2015-05-20 Paolo Malgaretti , Ignacio Pagonabarraga , J. Miguel Rubi

We study knotted polymers in equilibrium with an array of obstacles which models confinement in a gel or immersion in a melt. We find a crossover in both the geometrical and the topological behavior of the polymer. When the polymers' radius…

Soft Condensed Matter · Physics 2013-05-29 Enzo Orlandini , Attilio L. Stella , Carlo Vanderzande

Using analytical techniques and Langevin dynamics simulations, we investigate the dynamics of polymer translocation through a nanochannel embedded in two dimensions under an applied external field. We examine the translocation time for…

Soft Condensed Matter · Physics 2012-03-26 Huaisong Yong , Yilin Wang , Shichen Yuan , Bi Xu , Kaifu Luo

Macromolecular crowding can influence polymer shapes, which is important for understanding the thermodynamic stability of polymer solutions and the structure and function of biopolymers (proteins, RNA, DNA) under confinement. We explore the…

Soft Condensed Matter · Physics 2014-10-27 Wei Kang Lim , Alan R. Denton

The effect of a finite torque on semiflexible polymers in a confined environment is investigated. It is shown how a new lengthscale appears in the strongly confined limit. The influence of a torque on the extension of biopolymers in…

Soft Condensed Matter · Physics 2013-01-18 Marc Emanuel

We investigate the interplay of shape changes and localized surface plasmons in small metal particles with the potential of a large enhancement of the Raman signal from the particles own vibrations. The framework is a geometrical one where…

Optics · Physics 2016-01-26 S. P. Apell , G. Mukhopadhyay , Tomasz Antosiewicz , J Aizpurua

The conformational behavior of a polymer in a critical binary solvent confined in a porous medium is studied. The size of the polymer in bulk, which is mainly governed by the correlation length of the solvent density fluctuations, depends…

Soft Condensed Matter · Physics 2007-05-23 Amina Negadi , Arti Dua , Thomas A. Vigis

Mixtures of nanoparticles and polymer-like objects are encountered in many nanotechnological applications and biological systems. We study the behavior of grafted polymer layers decorated by nanoparticles that are attracted to the polymers…

Soft Condensed Matter · Physics 2011-10-31 Michael G. Opferman , Rob D. Coalson , David Jasnow , Anton Zilman