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We present a new theory that the molecular high order harmonic generation in an intense laser field is determined by molecular internal symmetry and momentum distribution of the tunneling-ionized electron. The molecular internal symmetry…

Atomic Physics · Physics 2008-01-30 J. Chen , Y. J. Chen , J. Fan , J. Liu , S. G. Chen , X. T. He

We predict high-order harmonics in which the polarization within the spectral bandwidth of each harmonic varies continuously and significantly. For example, the interaction of counter-rotating circularly-polarized bichromatic drivers having…

Optics · Physics 2014-10-24 Avner Fleischer , Ofer Kfir , Pavel Sidorenko , Oren Cohen

We present a theoretical analysis of high-order harmonic generation from ion-atom collisions in the presence of linearly polarized intense laser pulses. Photons with frequencies significantly higher than in standard atomic high-harmonic…

Atomic Physics · Physics 2009-11-10 Manfred Lein , Jan M. Rost

We study high-order harmonic generation (HHG) from aligned molecules in strong elliptically polarized laser fields numerically and analytically. Our simulations show that the spectra and polarization of HHG depend strongly on the molecular…

Atomic Physics · Physics 2021-05-19 F. J. Sun , C. Chen , W. Y. Li , X. Liu , W. Li , Y. J. Chen

We show that two-particle interferences can be used to probe the nuclear motion in a doubly-excited hydrogen molecule. The dissociation of molecular hydrogen by electron impact involves several decay channels, associated to different…

Asymmetric molecules look different when viewed from one side or the other. This difference influences the electronic structure of the valence electrons, thereby giving stereo sensitivity to chemistry and biology. We show that attosecond…

We present a complete theory of bicircular high-order-harmonic emission from N-fold rotationally symmetric molecules. Using a rotating frame of reference we predict the complete structure of the high-order-harmonic spectra for arbitrary…

Atomic Physics · Physics 2016-09-26 Daniel M. Reich , Lars Bojer Madsen

The generation of high harmonics is a strongly nonlinear effect that allows to probe properties of the target and to study electron dynamics in matter. It has been investigated in many different kinds of targets, including molecular gases,…

Quantum Physics · Physics 2026-05-06 Lina Bielke , Samuel Schöpa , Falk-Erik Wiechmann , Franziska Fennel , Dieter Bauer

High-order harmonics are ubiquitous in nature and present in electromagnetic, acoustic, and gravitational waves. They are generated by periodic nonlinear processes or periodic high-frequency pulses. However, this periodicity is often…

Head-on collision of laser-induced plasma wakefields with differing profiles of electrostatic potential has been recently found to be an efficient mechanism for generating high-power electromagnetic emission at the second harmonic of the…

Plasma Physics · Physics 2021-02-24 E. Volchok , V. Annenkov , I. Timofeev

Spontaneous emission of quantum emitters can be modified by engineering their optical environment. This allows a resonant nanoantenna to significantly modify the radiative properties of a quantum emitter. In this article, we go beyond the…

In this Letter, it is experimentally and theoretically shown that weak odd harmonics generated during the propagation of an infrared ultrashort ultra-intense pulse unexpectedly modify the nonlinear properties of the medium and lead to a…

Optics · Physics 2015-06-18 P. Béjot , G. Karras , F. Billard , E. Hertz , B. Lavorel , E. Cormier , O. Faucher

We investigate the contributions from the $3\sigma_{g}$ and $1\pi_{u}$ and molecular orbitals in high-order harmonic generation in $N_{2}$, with particular emphasis on quantum-interference effects. We consider both the physical processes in…

Atomic Physics · Physics 2009-09-08 C. Figueira de Morisson Faria , B. B. Augstein

We investigate the spatial characteristics of high-order harmonic radiation generated in argon, and observe cross-like patterns in the far field. An analytical model describing harmonics from an astigmatic driving beam reveals that these…

The double-slit experiment is the most direct demonstration of interference between individual quantum objects. Since similar experiments with single particles and more slits produce interference fringes reducible to a combination of…

Quantum Physics · Physics 2021-05-11 Lee A. Rozema , Zhao Zhuo , Tomasz Paterek , Borivoje Dakić

A theory of ultra-fast pump-probe experiments proposed by us earlier [F.H.M. Faisal et al., Phys. Rev. Lett. 98, 143001 (2007) and F.H.M. Faisal and A. Abdurrouf, Phys. Rev. Lett. 100, 123005 (2008)] is developed here fully and applied to…

Atomic and Molecular Clusters · Physics 2009-11-13 A. Abdurrouf , F. H. M. Faisal

The contribution of interference effects to the radiation of a charged particle moving in a medium of randomly spaced plates is considered. In the angular dependent radiation intensity a peak appears at angles $\theta\sim\pi-\gamma^{-1}$,…

Disordered Systems and Neural Networks · Physics 2007-05-23 Zh. S. Gevorkian , Th. M. Nieuwenhuizen

We utilize few-level model systems to analyze the polarization and phase properties of below-threshold harmonics generated from aligned molecules. In a two-level system, we find that the phase of emitted harmonics undergoes a distinct…

Quantum Physics · Physics 2026-05-06 Samuel Schöpa , Falk-Erik Wiechmann , Franziska Fennel , Dieter Bauer

Recent technological advances allowed the coherent optical manipulation of high-energy electron wavepackets with attosecond precision. Here we theoretically investigate the collision of optically-modulated pulsed electron beams with atomic…

Atomic Physics · Physics 2021-04-21 Yuya Morimoto , Peter Hommelhoff , Lars Bojer Madsen

Control and manipulation of electric current and, especially, its degree of spin polarization (spin filtering) across single molecules are currently of great interest in the field of molecular spintronics. We explore one possible strategy…

Mesoscale and Nanoscale Physics · Physics 2019-08-20 Dongzhe Li , Rajdeep Banerjee , Sourav Mondal , Ivan Maliyov , Mariya Romanova , Yannick J. Dappe , Alexander Smogunov