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The spectrum of higher harmonics in atoms calculated with a uniformized semiclassical propagator is presented and it is shown that higher harmonic generation is an interference phenomenon which can be described semiclassically. This can be…

Atomic Physics · Physics 2009-10-31 Gerd van de Sand , Jan M Rost

The interference phenomenon of light is a common but most important effect in physics. In this article, we compare and analyse the interference effects of both coherent and incoherent light; in particular, the interference of spatially…

Quantum Physics · Physics 2023-03-28 Kaige Wang

We present a theoretical model of high-harmonic generation from diatomic molecules. The theory includes effects of alignment as well as nuclear motion and is used to predict results for N$_2$, O$_2$, H$_2$ and D$_2$. The results show that…

Atomic Physics · Physics 2007-05-23 Christian Bruun Madsen , Lars Bojer Madsen

We investigate the effect on high-order harmonic generation of the distortion of molecular orbitals by the driving laser field. Calculations for high-order harmonic generation including orbital distortion are performed for N2. Our results…

Atomic Physics · Physics 2015-06-15 Maciej Dominik Śpiewanowski , Adam Etches , Lars Bojer Madsen

We address the influence of the orbital symmetry and of the molecular alignment with respect to the laser-field polarization on laser-induced nonsequential double ionization of diatomic molecules, in the length and velocity gauges. We work…

Atomic Physics · Physics 2009-11-13 C. Figueira de Morisson Faria , T. Shaaran , X. Liu , W. Yang

We investigate how short and long electron trajectory contributions to high harmonic emission and their interferences give access to intra-molecular dynamics. In the case of unaligned molecules, we show experimental evidences that the long…

Nonlinear effects in emission and absorption spectra of gaseous systems are considered. It is shown that level splitting can be detected spectroscopically even if it is below the Doppler width. Conditions for distinguishing interference…

Quantum Physics · Physics 2007-05-23 T. Ya. Popova , A. K. Popov , S. G. Rautian , R. I. Sokolovskii

Recent reports on intense-field pump-probe experiments for high harmonic generation from coherently rotating linear molecules, have revealed remarkable characteristic effects of the simultaneous variation of the polarization geometry and…

Atomic and Molecular Clusters · Physics 2009-11-13 F. H. M. Faisal , A. Abdurrouf

The alternative to dynamic alignment explanation of experimental results on spatial-asymmetric dissociation of molecules in a laser field is proposed. The concept of geometrical alignment is sufficient for explanation of these results. In…

Optics · Physics 2007-05-23 V. A. Kuz'menko

The spectral line polarization produced by optically pumped atoms contains a wealth of information on the thermal and magnetic structure of a variety of astrophysical plasmas, including that of the solar atmosphere. A correct decoding of…

Solar and Stellar Astrophysics · Physics 2015-05-30 Luca Belluzzi , Javier Trujillo Bueno

We report results from a series of PIC simulations carried out to investigate the interaction of intense laser light with overdense plasma and in particular, aspects of the harmonic emission spectrum generated in these interactions. Recent…

Plasma Physics · Physics 2007-05-23 Tim James Morrow Boyd , Ricardo Ondarza-Rovira

We calculate angle-resolved above-threshold ionization spectra for diatomic molecules in linearly polarized laser fields, employing the strong-field approximation. The interference structure resulting from the individual contributions of…

Atomic Physics · Physics 2009-11-13 H. Hetzheim , C. Figueira de Morisson Faria , W. Becker

High-order harmonic generation via single-slit diffraction of relativistic laser pulses is investigated. Using fully kinetic 2D and 3D particle-in-cell simulations, we show that interesting optical phenomena emerge, including the generation…

Plasma Physics · Physics 2025-05-07 Longqing Yi

We study the ellipticity of high-order harmonics emitted from CO$_2$ molecule driven by linearly polarized laser fields using numerical simulations within the time-dependent density functional theory. We find that the overall ellipticity of…

Atomic and Molecular Clusters · Physics 2024-09-17 Andres Mora , Lauren Bauerle , Yuqing Xia , Agnieszka Jaron

We investigate the alignment-dependent high-order harmonic spectrum generated from nonadiabatically aligned molecules around the first half rotational revival. It is found that the evolution of the molecular alignment is encoded in the…

Atomic Physics · Physics 2014-03-13 Meiyan Qin , Xiaosong Zhu , Yang Li , Qingbin Zhang , Pengfei Lan , Peixiang Lu

We investigate high-order harmonic generation (HHG) in graphene with a quantum master equation approach. The simulations reproduce the observed enhancement in HHG in graphene under elliptically polarized light [N. Yoshikawa et al, Science…

Materials Science · Physics 2021-02-03 Shunsuke A. Sato , Hideki Hirori , Yasuyuki Sanari , Yoshihiko Kanemitsu , Angel Rubio

We study first-order interference in spontaneous parametric down-conversion generated by two pump pulses that do not overlap in time. The observed modulation in the angular distribution of the signal detector counting rate can only be…

Quantum Physics · Physics 2009-10-31 Yoon-Ho Kim , Maria V. Chekhova , Sergei P. Kulik , Yanhua Shih , Morton H. Rubin

We consider several aspects of high-order harmonic generation in solids: the effects of elastic and inelastic scattering; varying pulse characteristics; and inclusion of material-specific parameters through a realistic band structure. We…

Other Condensed Matter · Physics 2013-02-07 A. F. Kemper , B. Moritz , J. K. Freericks , T. P. Devereaux

We introduce and demonstrate a new approach to measuring coherent electron wave packets using high-harmonic spectroscopy. By preparing a molecule in a coherent superposition of electronic states, we show that electronic coherence opens…

Chemical Physics · Physics 2014-07-09 P. M. Kraus , S. B. Zhang , A. Gijsbertsen , R. R. Lucchese , N. Rohringer , H. J. Wörner

Reradiation of a spatially non-uniform ultrashort electromagnetic pulse interacting with the linear chain of multielectron atoms is studied in the framework of sudden perturbation approximation. Angular distributions of the reradiation…

Atomic Physics · Physics 2018-10-16 V. I. Matveev , D. U. Matrasulov