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We present the implementation of an electronic-structure approach dedicated to ionization dynamics of molecules interacting with x-ray free-electron laser (XFEL) pulses. In our scheme, molecular orbitals for molecular core-hole states are…

Chemical Physics · Physics 2015-05-18 Yajiang Hao , Ludger Inhester , Kota Hanasaki , Sang-Kil Son , Robin Santra

Although the interaction of a flat-foil with currently available laser intensities is now considered a routine process, during the last decade emphasis is given to targets with complex geometries aiming on increasing the ion energy. This…

Plasma Physics · Physics 2020-06-03 P. Hadjisolomou , S. V. Bulanov , G. Korn

Spin-dependent Kapitza-Dirac scattering of electron beams from counterpropagating bichromatic laser waves in various polarization geometries is studied. The corresponding scattering probabilities are obtained by analytical and numerical…

Atomic Physics · Physics 2017-05-23 Matthias M. Dellweg , Carsten Müller

The photoionization of a helium atom by short intense laser pulses is studied theoretically in the vicinity of the $2s2p\,^1P$ doubly-excited state with the intention to investigate the impact of the intensity and duration of the exciting…

Atomic Physics · Physics 2017-09-20 Anton N. Artemyev , Lorenz S. Cederbaum , Philipp V. Demekhin

We study double ionization in a one-dimensional model of a three-electron atom exposed to strong short laser fields. The corresponding ab initio simulations reveal a characteristic ``knee'' in the ionization yield at lower field intensities…

Atomic Physics · Physics 2025-06-30 Dmitry Efimov

We suggest a new spin orientation mechanism for localized electrons: $dynamic~electron~spin~polarization~provided~by~nuclear~spin~fluctuations$. The angular momentum for the electrons is gained from the nuclear spin system via the hyperfine…

Mesoscale and Nanoscale Physics · Physics 2020-10-14 D. S. Smirnov , T. S. Shamirzaev , D. R. Yakovlev , M. Bayer

We propose a scheme to overcome the great challenge of polarization loss in spin-polarized ion acceleration. When a petawatt laser pulse penetrates through a compound plasma target consisting of a double layer slab and prepolarized hydrogen…

Plasma Physics · Physics 2020-11-24 Zheng Gong , Yinren Shou , Yuhui Tang , Xueqing Yan

Relativistic Hartree-Fock and random phase approximation methods for open shells are used to calculate ionization potentials and static scalar polarizabilities of eight superheavy elements with open $6d$-shell, which include Db, Sg, Bh, Hs,…

Atomic Physics · Physics 2016-04-06 V. A. Dzuba

We identify that both the dynamic core polarization and dynamic orbital deformation are important in the orientation-dependent high-harmonic generation of CO molecules subjected to intense few cycle laser fields. These polarization dynamics…

Atomic Physics · Physics 2015-06-19 Bin Zhang , Jianmin Yuan , Zengxiu Zhao

The potential energy curves, permanent and transition dipole moments, and the static dipolar polarizability, of molecular ions composed of one alkali-metal atom and a Strontium ion are determined with a quantum chemistry approach. The…

Quantum Physics · Physics 2015-05-27 Mireille Aymar , Romain Guérout , Olivier Dulieu

In this work, we investigate the applicability of the core-polarization-corrected Dirac--Fock method, formulated within the framework of the local Dirac--Hartree--Fock (LDF) potential, for the accurate determination of static scalar and…

Theoretical study on H$_2^+$ in an intense infrared laser field on the attosecond time-scale reveals that the molecular ion shows multiple bursts of ionization within a half-cycle of the laser field oscillation, in contrast to the widely…

Chemical Physics · Physics 2010-12-10 Norio Takemoto , Andreas Becker

The fixed-nuclei full dimensional time-dependent Schr \"odinger equation is directly solved for H$_2^+$ in the linearly polarized laser field of $I \sim 1.0 \times 10^{14}$W cm$^{-2}$ and $\lambda \sim 1064 $nm Instantaneous ionization rate…

Atomic Physics · Physics 2007-05-23 Mohsen Vafaee , Hassan Sabzyan , Zahra Vafaee , Ali Katanforoush

Electron-electron correlation effects play an instrumental role in our understanding of sequential (SDI) and non-sequential double ionization (NSDI) mechanisms. Here, we present a theoretical study of NSDI driven by plasmonic-enhanced…

The laser excitation of an ion crystal to high lying and long-lived electronic states is a genuine many-body process even if in fact only a single ion is excited. This is a direct manifestation of the strong coupling between internal and…

Atomic Physics · Physics 2012-01-16 Weibin Li , Igor Lesanovsky

We formulate a three-dimensional semi-classical model to address triple and double ionization in three-electron atoms driven by intense infrared laser pulses. During time propagation, our model fully accounts for the Coulomb singularities,…

Atomic Physics · Physics 2022-04-20 M. B. Peters , G. P. Katsoulis , A. Emmanouilidou

Nonlinear relativistic ionization phenomena induced by a strong linearly polarized laser field are considered. The starting point is the classical relativistic action for a free electron moving in the electromagnetic field created by a…

Atomic Physics · Physics 2017-08-23 J. Ortner , V. M. Rylyuk

The phenomenon of polarization of nuclei in the process of stimulated recombination of atoms in the field of circularly polarized laser radiation is considered. This effect is considered for the case of the proton-electron beams used in the…

Atomic Physics · Physics 2017-07-11 M. A. Kutlan

We have studied the dynamics of one and two laser-cooled trapped $^{40}$Ca$^+$ ions by applying electric fields of different nature along the axial direction of the trap, namely, driving the motion with a harmonic dipolar field, or with…

Chirality causes symmetry breaks in a large variety of natural phenomena ranging from particle physics to biochemistry. We investigate one of the simplest conceivable chiral systems, a laser-excited, oriented, effective one-electron Li…