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The ionization of H2 in intense laser pulses is studied by numerical integration of the time-dependent Schr\"odinger equation for a single-active-electron model including the vibrational motion. The electron kinetic-energy spectra in…

Atomic Physics · Physics 2009-11-13 Stefan Pieper , Manfred Lein

We propose a new scenario to apply IR-pump-XUV-probe schemes to resolving strong field ionization induced and attosecond pulse driven electron-hole dynamics and coherence in real time. The coherent driving of both the infrared laser and the…

Atomic Physics · Physics 2016-02-26 Jing Zhao , Jianmin Yuan , Zengxiu Zhao

We analyze, quantum mechanically, the dynamics of ionization with a strong, circularly polarized, laser field. We show that the main source for non-adiabatic effects is connected to an effective barrier lowering due to the laser frequency.…

Atomic Physics · Physics 2014-09-26 Francois Mauger , A. D. Bandrauk

The angular distribution of the emitted electrons, following the two--photon ionization of the hydrogen--like ions, is studied within the framework of second order perturbation theory \textit{and} the Dirac equation. Using a density matrix…

Atomic Physics · Physics 2007-05-23 Peter Koval , Stephan Fritzsche , Andrey Surzhykov

We employ the exact factorization of a multi-component wavefunction to analyze the dynamics of interacting photons, electrons and nuclei. We consider physical situations emerging in the regime of strong coupling between light excitations…

Chemical Physics · Physics 2026-04-24 Claudia Magi , Peter Schuerger , David Lauvergnat , Federica Agostini

We investigate the dynamics of an ion sympathetically cooled by another laser-cooled ion or small ion crystal. To this end, we develop simple models of the cooling dynamics in the limit of weak Coulomb interactions. Experimentally, we…

Quantum Physics · Physics 2015-10-02 M. Guggemos , D. Heinrich , O. A. Herrera-Sancho , R. Blatt , C. F. Roos

We study the role of electron-electron correlation in the ground-state of Ne, as well as in photoionization dynamics induced by an attosecond XUV pulse. For a selection of central photon energies around 100 eV, we find that while the…

Atomic Physics · Physics 2018-01-31 Juan J. Omiste , Lars Bojer Madsen

The degree of elliptical polarization of intense short laser pulses is shown to be related to the timing of strong-field non-sequential double ionization. Higher ellipticity is predicted to force the initiation of double ionization into a…

Atomic Physics · Physics 2010-08-20 Xu Wang , J. H. Eberly

We describe an ab initio and non-perturbative $R$-matrix with time-dependence theory for ultrafast atomic processes in light fields of arbitrary polarization. The theory is applicable to complex, multielectron atoms and atomic ions subject…

Atomic Physics · Physics 2018-12-04 D. D. A. Clarke , G. S. J. Armstrong , A. C. Brown , H. W. van der Hart

A new electronic structure model is developed in which the ground state energy of a molecular system is given by a Hartree-Fock-like expression with parametrized one- and two-electron integrals over an extended (minimal + polarization) set…

Chemical Physics · Physics 2014-02-11 Dimitri N. Laikov

We study a novel regime of the Rydberg excitation blockade using highly Stark-shifted, yet long-living, states of Rb atoms subject to electric fields above the classical ionization limit. Such states allow tuning the dipole-dipole…

It has recently been suggested that two counter-propagating, circularly polarized, ultra-intense lasers can induce a strong electron spin polarization at the magnetic node of the electromagnetic field that they setup. We confirm these…

Plasma Physics · Physics 2018-04-16 Dario Del Sorbo , Daniel Seipt , Alexander G. R. Thomas , Christopher P. Ridgres

We study excitation and ionization in the 1.5 MeV/amu O$^{8+}$-Li collision system, which was the subject of a recent reaction-microscope-type experiment [Fischer \textit{et al.}, Phys. Rev. Lett. \textbf{109}, 113202 (2012)]. Starting from…

Atomic Physics · Physics 2015-01-19 T. Kirchner , N. Khazai , L. Gulyás

Coulomb interactions that occur in electronic structure calculations are correlated by allowing basis function components of the interacting densities to polarize, thereby reducing the magnitude of the interaction. Exchange integrals of…

Chemical Physics · Physics 2022-05-16 Jerry L. Whitten

We investigate dynamics of atomic and molecular systems exposed to intense, shaped chaotic fields and a weak femtosecond laser pulse theoretically. As a prototype example, the photoionization of a hydrogen atom is considered in detail. The…

Quantum Physics · Physics 2015-05-18 Kamal P Singh , Jan M Rost

The polarisation conversion of a linear polarised electromagnetic wave incident onto a two-dimensional (2D) electron system at an angle is theoretically studied. We consider the 2D system located at the interface between two dielectric…

Condensed Matter · Physics 2009-11-07 V. V. Popov , T. V. Teperik

A theory for the many-electron multi-photon process is presented. It is shown that after single-electron excitation into some level in the continuum (ATI) an inelastic collision of the excited electron with the parent atomic particle can…

atom-ph · Physics 2009-10-28 M. Yu. Kuchiev

When a strong laser pulse induces the ionization of an atom, momentum conservation dictates that the absorbed photons transfer their momentum $p_{\gamma}=E_{\gamma}/c$ to the electron and its parent ion. Even after 30 years of studying…

Double ionization processes triggered by intense linearly polarized laser fields have revealed the paramount role of electron-electron collisions. It has been shown that the correlated dynamics of such electronic collisions can be modeled…

Atomic Physics · Physics 2011-05-03 Francois Mauger , Cristel Chandre , Turgay Uzer

Electron heating and ionization dynamics in capacitively coupled radio frequency (RF) atmospheric pressure microplasmas operated in helium are investigated by Particle in Cell simulations and semi-analytical modeling. A strong heating of…

Plasma Physics · Physics 2013-06-03 T. Hemke , D. Eremin , T. Mussenbrock , A. Derzsi , Z. Donkó , K. Dittmann , J. Meichsner , J. Schulze