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The orientation-dependent strong-field ionization of CO molecules is investigated using the fully propagated three-dimensional time-dependent Hartree-Fock theory. The full ionization results are in good agreement with recent experiments.…

Atomic Physics · Physics 2013-10-30 Bin Zhang , Jianmin Yuan , Zengxiu Zhao

The influence of inner electrons on the ionization dynamics in strong laser fields is investigated in a wavelength regime where the inner electron dynamics is usually assumed to be negligible. The role of inner electrons is of particular…

Atomic Physics · Physics 2014-03-11 J. Rapp , D. Bauer

We develop an analytical model of correlated two-electron ionization in strong infrared laser fields. The model includes all relevant interactions between the electrons, the laser field, and the ionic core nonperturbatively. We focus on the…

Atomic Physics · Physics 2009-02-14 Denys I. Bondar , Wing-Ki Liu , Misha Yu. Ivanov

Two-color laser fields offer significantly enhanced control over electron excitation dynamics under ultrashort intense laser pulses compared to monochromatic fields. However, their strong nonlinearity necessitates computationally expensive…

Optics · Physics 2025-07-03 Mizuki Tani , Kenichi L. Ishikawa , Tomohito Otobe

The dynamics of molecular electron excitation and ionisation is studied in real-time for ultra-short IR laser pulses of intensity I>10^{13} W/cm^{2}. The multi-electron molecule is modeled by a system of two active electrons moving in a…

Optics · Physics 2015-06-26 A. I. Pegarkov

We present a novel approach to calculating strong field ionization dynamics of multielectron molecular targets. Adopting a multielectron wavefunction ansatz based on field-free ab initio neutral and ionic multielectron states, a set of…

Atomic Physics · Physics 2015-05-14 Michael Spanner , Serguei Patchkovskii

Owing to its numerical simplicity, a two-dimensional two-electron model atom, with each electron moving in one direction, is an ideal system to study non-perturbatively a fully correlated atom exposed to a laser field. Frequently made…

Atomic Physics · Physics 2009-10-30 D. Bauer

Molecules show a much increased multiple ionization rate in a strong laser field as compared to atoms of similar ionization energy. A widely accepted model attributes this to the action of the joint fields of the adjacent ionic core and the…

Atomic Physics · Physics 2013-05-16 J. Wu , M. Meckel , L. Ph. H. Schmidt , M. Kunitski , S. Voss , H. Sann , H. Kim , T. Jahnke , A. Czasch , R. Dörner

We study numerically stabilization against ionization of a fully correlated two-electron model atom in an intense laser pulse. We concentrate on two frequency regimes: very high frequency, where the photon energy exceeds both, the…

Atomic Physics · Physics 2009-10-31 D. Bauer , F. Ceccherini

With a semiclassical quasi-static model we achieve an insight into the complex dynamics of two correlated electrons under the combined influence of a two-center Coulomb potential and an intense laser field. The model calculation is able to…

Atomic and Molecular Clusters · Physics 2009-11-13 J. Liu , D. F. Ye , J. Chen , X. liu

We consider the classical dynamics of a two-electron system subjected to an intense bichromatic linearly polarized laser pulse. By varying the parameters of the field, such as the phase lag and the relative amplitude between the two colors…

Chaotic Dynamics · Physics 2011-04-04 Adam Kamor , Francois Mauger , Cristel Chandre , Turgay Uzer

We discuss the mechanism by which the inclusion of multielectron polarization improves the solution of the time-dependent Schr\"{o}dinger equation (TDSE) for the oriented CO molecule in a strong external laser pulse within the…

Atomic Physics · Physics 2020-02-05 Mahmoud Abu-samha , Lars B Madsen

Double electron ionisation process occurs when an intense laser pulse interacts with atoms or molecules. Exact {\it ab initio} numerical simulation of such a situation is extremely computer resources demanding, thus often one is forced to…

Photoionization of an atom $A$ by a strong laser field in the presence of a spatially well-separated neighboring atom $B$ is considered. The laser field frequency is assumed to lie below the ionization potential of atom $A$ and be resonant…

Atomic Physics · Physics 2018-10-03 J. Fedyk , A. B. Voitkiv , C. Müller

We develop a time-dependent theory to investigate electron dynamics and photoionization processes of diatomic molecules interacting with strong laser fields including electron-electron correlation effects. We combine the recently formulated…

Chemical Physics · Physics 2016-02-02 Henrik R. Larsson , Sebastian Bauch , Lasse Kragh Sørensen , Michael Bonitz

The time-dependent complete-active-space self-consistent-field (TD-CASSCF) method for the description of multielectron dynamics in intense laser fields is presented, and a comprehensive description of the method is given. It introduces the…

Atomic Physics · Physics 2015-06-15 Takeshi Sato , Kenichi L. Ishikawa

The ionization of an atom by a high-frequency intense laser pulse, where the energy of a single-photon is sufficient to ionize the system, is investigated from first principles. It is shown that as a consequence of an AC Stark effect in the…

Atomic Physics · Physics 2012-06-26 Philipp V Demekhin , Lorenz S Cederbaum

The spin polarization of photoelectrons induced by an intense linearly polarized laser field is investigated using numerical solutions of the time-dependent Schr\"odinger equation in companion with our analytic treatment via the…

Atomic Physics · Physics 2024-02-20 Pei-Lun He , Zhao-Han Zhang , Karen Z. Hatsagortsyan , Christoph H. Keitel

Here, we demonstrate the radiative polarization of high-energy electron beams in collisions with ultrashort pulsed bi-chromatic laser fields. Employing a Boltzmann kinetic approach for the electron distribution allows us to simulate the…

Plasma Physics · Physics 2019-12-06 Daniel Seipt , Dario Del Sorbo , Christopher P. Ridgers , Alec G. R. Thomas

We theoretically study multiphoton ionization of Mg in the circularly as well as the linearly polarized laser fields. Specifically two-, three-, and four-photon ionization cross sections from the ground and first excited states are…

Atomic Physics · Physics 2013-03-07 Gabriela Buica , Takashi Nakajima
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