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We study a large number of physically-plausible arrangements of chromophores, generated via a computational method involving stochastic real-space transformations of a naturally occurring `reference' structure, illustrating our methodology…

Chemical Physics · Physics 2017-05-23 George C. Knee , Patrick Rowe , Luke D. Smith , Alessandro Troisi , Animesh Datta

The performance enhancements observed in various models of continuous quantum thermal machines have been linked to the buildup of coherences in a preferred basis. But, is this connection always an evidence of `quantum-thermodynamic…

Quantum Physics · Physics 2019-07-04 J. Onam González , José P. Palao , Daniel Alonso , Luis A. Correa

We study the modification of the second law of thermodynamics for a quantum system interacting with a reservoir regarding quantum coherence. The whole system is isolated so that neither energy nor information is lost. It is discovered that…

Quantum Physics · Physics 2021-10-12 Yu-Han Ma , C. L. Liu , C. P. Sun

In this work we study singlet fission in tetracene para-dimers, covalently linked by a phenyl group. In contrast to most previous works, we account for the full quantum dynamics of the combined excitonic and vibrational system. For our…

Materials Science · Physics 2021-11-17 Sam Mardazad , Yihe Xu , Xuexiao Yang , Martin Grundner , Ulrich Schollwöck , Haibo Ma , Sebastian Paeckel

Narrow line-widths and the possibility of enhanced spontaneous emission via coupling to microcavities make semiconductor quantum dots ideal for harnessing coherent quantum phenomena at the single photon level. So far, however, all…

Mesoscale and Nanoscale Physics · Physics 2007-07-26 A. Muller , E. B. Flagg , P. Bianucci , D. G. Deppe , W. Ma , J. Zhang , G. J. Salamo , C. K. Shih

Collective behavior where a set of elements interact and generate effects that are beyond the reach of the individual non interacting elements, are always of great interest in physics. Quantum collective effects that have no classical…

Quantum Physics · Physics 2016-08-17 Raam Uzdin

Long-lived electronic coherences in various photosynthetic complexes at cryogenic and room temperature have generated vigorous efforts both in theory and experiment to understand their origins and explore their potential role to biological…

Quantum Physics · Physics 2010-12-16 Patrick Rebentrost , Sangwoo Shim , Joel Yuen-Zhou , Alán Aspuru-Guzik

In a thermal ensemble of atoms driven by coherent fields, how does evolution of quantum superposition compete with classical dynamics of optical pumping and atomic diffusion? Is it optical pumping that first prepares a thermal ensemble,…

Atomic Physics · Physics 2016-06-22 Arif Warsi Laskar , Niharika Singh , Arunabh Mukherjee , Saikat Ghosh

Coherent excitation of materials via ultrafast laser pulses can have interesting, observable dynamics in time-resolved photoemission measurements. The broad spectral width of ultrafast pump pulses can coherently excite multiple exciton…

Mesoscale and Nanoscale Physics · Physics 2019-03-27 Avinash Rustagi , Alexander F. Kemper

We consider the dissipative charging process of quantum batteries in terms of a collisional model, where the batteries are coupled to a heat bath using non-energy preserving interactions. First, we show that for low temperatures the…

Quantum Physics · Physics 2022-06-07 Franco Mayo , Augusto J. Roncaglia

Hybrid quantum-classical algorithms are among the most promising systems to implement quantum computing under the Noisy-Intermediate Scale Quantum (NISQ) technology. In this paper, at first, we investigate a quantum dynamics algorithm for…

Quantum Physics · Physics 2020-08-13 Mahmoud Mahdian , H. Davoodi Yeganeh

In this Article we perform a systematic study of the global entanglement and exciton coherence length dynamics coherence in natural light-harvesting system Fenna-Matthews-Olson (FMO) complex across various parameters of a dissipative…

Quantum Physics · Physics 2024-06-18 Luis E. Herrera Rodríguez , Alexei A. Kananenka

We investigate the effects of noise-induced coherence on average current and current fluctuations in a simple model of quantum absorption refrigerator with degenerate energy levels. We describe and explain the differences and similarities…

Statistical Mechanics · Physics 2020-07-28 Viktor Holubec , Tomáš Novotný

We clarify different definitions of the density matrix by proposing the use of different names, the full density matrix for a single-closed quantum system, the compressed density matrix for the averaged single molecule state from an…

Quantum Physics · Physics 2007-05-23 Gui Lu Long , Yi-Fan Zhou , Jia-Qi Jin , Yang Sun , Hai-Woong Lee

Quantum dynamics of coherent states is studied within quantum field theory using two complementary methods: by organizing the evolution as a Taylor series in elapsed time and by perturbative expansion in coupling within the…

High Energy Physics - Theory · Physics 2021-10-13 Lasha Berezhiani , Michael Zantedeschi

Photosynthesis is the basic process used by plants to convert light energy in reaction centers into chemical energy. The high efficiency of this process is not yet understood today. Using the formalism for the description of open quantum…

Biological Physics · Physics 2017-06-12 Hichem Eleuch , Ingrid Rotter

We obtain exact analytic expressions for a class of functions expressed as integrals over the Haar measure of the unitary group in d dimensions. Based on these general mathematical results, we investigate generic dynamical properties of…

Quantum Physics · Physics 2013-04-30 Manuel Gessner , Heinz-Peter Breuer

Electronic coherences are key to understanding and controlling photo-induced molecular transformations. We identify a crucial quantum-mechanical feature of electron-nuclear correlation, the projected nuclear quantum momenta, essential to…

Chemical Physics · Physics 2024-11-13 Evaristo Villaseco Arribas , Neepa T. Maitra

We discuss the potential creation and measurement of coherences in both dispersive solids and qubit-like single levels using current generation time- and angle-resolved photoemission technology. We show that in both cases, when both the…

Mesoscale and Nanoscale Physics · Physics 2020-05-22 Alexander F. Kemper , Avinash Rustagi

A model multilevel molecule described by two sets of rotational internal energy levels of different parity and degenerate ground states, coupled by a constant interaction, is considered, by assuming that the random collisions in a gas of…

Quantum Physics · Physics 2013-05-31 Filippo Giraldi , Francesco Petruccione