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The dominant source of decoherence for an electron spin in a quantum dot is the hyperfine interaction with the surrounding bath of nuclear spins. The decoherence process may be slowed down by subjecting the electron spin to suitable…

Mesoscale and Nanoscale Physics · Physics 2017-08-23 Wenxian Zhang , V. V. Dobrovitski , Lea F. Santos , Lorenza Viola , B. N. Harmon

Color centers in solids, such as the nitrogen-vacancy center in diamond, offer well-protected and well-controlled localized electron spins that can be employed in various quantum technologies. Moreover, the long coherence time of the…

Quantum Physics · Physics 2020-08-11 Wenzheng Dong , F. A. Calderon-Vargas , Sophia E. Economou

Dynamic nuclear polarization (DNP) can increase nuclear magnetic resonance (NMR) signals by orders of magnitude. DNP in diamond proceeds through different DNP mechanisms with a possible temperature-dependence. We report on 13C dynamic…

The dynamics of single electron and nuclear spins in a diamond lattice with different 13C nuclear spin concentration is investigated. It is shown that coherent control of up to three individual nuclei in a dense nuclear spin cluster is…

Nuclear spins and paramagnetic centers in a solid randomly group to form clusters featuring nearly-degenerate, hybrid states whose dynamics are central to processes involving nuclear spin-lattice relaxation and diffusion. Their…

We demonstrate fluorescence thermometry techniques with sensitivities approaching 10 mK Hz^(-1/2) based on the spin-dependent photoluminescence of nitrogen vacancy (NV) centers in diamond. These techniques use dynamical decoupling protocols…

Mesoscale and Nanoscale Physics · Physics 2013-05-24 David M. Toyli , Charles F. de las Casas , David J. Christle , Viatcheslav V. Dobrovitski , David D. Awschalom

Spin qubit coherence is a fundamental resource for the realization of quantum technologies. For solid-state platforms, spin decoherence is dominated by the magneto-active environment in the lattice, limiting their applicability. While…

By efficient nanoscale plasma etching, the nitrogen-vacancy (NV) centers in diamond were brought to the sample surface step by step successfully. At each depth, we used the relative ratios of spin coherence times before and after applying…

Mesoscale and Nanoscale Physics · Physics 2018-01-03 Wenlong Zhang , Jian Zhang , Junfeng Wang , Fupan Feng , Shengran Lin , Liren Lou , Wei Zhu , Guanzhong Wang

The magnetic interactions between the spin of an unpaired electron and the surrounding nuclear spins can be exploited to gain structural information, to reduce nuclear relaxation times as well as to create nuclear hyperpolarization via…

The room temperature compatibility of the negatively-charged nitrogen-vacancy (NV-) in diamond makes it the ideal quantum system for a university teaching lab. Here, we describe a low-cost experimental setup for coherent control experiments…

The nitrogen-vacancy (NV) center in diamond is a promising quantum system for magnetometry applications exhibiting optical readout of minute energy shifts in its spin sub-levels. Key material requirements for NV ensembles are a high NV$^-$…

The ground state spin of the negatively charged nitrogen-vacancy center in diamond has many exciting applications in quantum metrology and solid state quantum information processing, including magnetometry, electrometry, quantum memory and…

Materials Science · Physics 2012-06-05 M. W. Doherty , F. Dolde , H. Fedder , F. Jelezko , J. Wrachtrup , N. B. Manson , L. C. L. Hollenberg

In many realizations of electron spin qubits the dominant source of decoherence is the fluctuating nuclear spin bath of the host material. The slowness of this bath lends itself to a promising mitigation strategy where the nuclear spin bath…

Mesoscale and Nanoscale Physics · Physics 2010-11-30 Hendrik Bluhm , Sandra Foletti , Diana Mahalu , Vladimir Umansky , Amir Yacoby

We present theoretical proposals for two-dimensional nuclear magnetic resonance spectroscopy protocols based on Nitrogen-vacancy (NV) centers in diamond that are strongly coupled to the target nuclei. Continuous microwave and…

Quantum Physics · Physics 2024-10-31 Matthias Kost , Jianming Cai , Martin B. Plenio

After initial proof-of-principle demonstrations, optically pumped nitrogen-vacancy (NV) centres in diamond have been proposed as a non-invasive platform to achieve hyperpolarisation of nuclear spins in molecular samples over macroscopic…

Mesoscale and Nanoscale Physics · Physics 2021-01-27 J. -P. Tetienne , L. T. Hall , A. J. Healey , G. A. L. White , M. -A. Sani , F. Separovic , L. C. L. Hollenberg

Nitrogen vacancy (NV) centers, optically-active atomic defects in diamond, have attracted tremendous interest for quantum sensing, network, and computing applications due to their excellent quantum coherence and remarkable versatility in a…

The nitrogen-vacancy (N-V) center in diamond is promising as an electron spin qubit due to its long-lived coherence and optical addressability. The ground state is a spin triplet with two levels ($m_s = \pm 1$) degenerate at zero magnetic…

Other Condensed Matter · Physics 2007-10-15 T. P. Mayer Alegre , C. Santori , G. Medeiros-Ribeiro , R. G. Beausoleil

Precise knowledge of a quantum system's Hamiltonian is a critical pre-requisite for its use in many quantum information technologies. Here, we report a method for the precise characterization of the non-secular part of the excited-state…

Quantum Physics · Physics 2017-06-20 F. Poggiali , P. Cappellaro , N. Fabbri

The electronic spins of the nitrogen-vacancy centers (NV centers) in Chemical-Vapor-Deposition (CVD) grown diamonds form ideal probes of magnetic fields and temperature, as well as promising qu-bits for quantum information processing.…

Quantum Physics · Physics 2021-03-31 C. Pellet-Mary , P. Huillery , M. Perdriat , A. Tallaire , G. Hétet

Chemically induced dynamic nuclear polarization is a signature of spin order appearing in many photosynthetic reaction centers. Such polarization, significantly enhanced above thermal equilibrium, is known to result from the nuclear spin…

Quantum Physics · Physics 2015-06-12 I. K. Kominis