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We report on a polarized-neutron Laue diffraction experiment on a single crystal of neodynium doped lanthanum magnesium nitrate hydrate containing polarized proton spins. By using dynamic nuclear polarization to polarize the proton spins,…

The nitrogen-vacancy (NV) center spin represents an appealing candidate for quantum information processing. Besides the widely used microwave control, its coherent manipulation may also be achieved using laser as mediated by the excited…

Quantum Physics · Physics 2022-05-05 Jiazhao Tian , Tianyi Du , Yu Liu , Haibin Liu , Fangzhou Jin , Ressa S. Said , Jianming Cai

Electron spin qubit coherence in quantum dots is ultimately limited by random nuclear spin bath fluctuations. Here we aim to eliminate this randomness by making spin bath evolution deterministic. We introduce spin bath control sequences,…

Mesoscale and Nanoscale Physics · Physics 2019-07-18 A. M. Waeber , M. Hopkinson , M. S. Skolnick , E. A. Chekhovich

Nitrogen vacancy centers (NV) in proximity to diamond surfaces are promising nanoscale quantum sensors. However, their coherence properties are negatively affected by magnetic and electric surface noise, whose origin and detailed impact…

Quantum Physics · Physics 2025-12-12 Jonah Nagura , Mykyta Onizhuk , Giulia Galli

The nature of the nano-scale environment presents a major challenge for solid-state implementation of spin-based qubits. In this work, a single electron spin in an optically pumped nanometer-sized III-V semiconductor quantum dot is used to…

Nitrogen-vacancy (NV) center in diamond was found to be a powerful tool for various sensing applications. The main work horse of this center so far has been optically detected electron resonance. Utilization of the nuclear spin has the…

Efficient hyperpolarisation of nuclear spins via optically active defect centers, such as the nitrogen vacancy (NV) center in diamond, has great potential for enhancing NMR based quantum information processing and nanoscale magnetic…

The integration of NMR and high pressure technique brings unique opportunities to study electronic, structural and dynamical properties under extreme conditions. Despite a great degree of success has been achieved using coil-based schemes,…

Quantum Physics · Physics 2022-03-22 Yan-Xing Shang , Fang Hong , Jian-Hong Dai , Ya-Nan Lu , Hui Yu , Yong-Hong Yu , Xiao-Hui Yu , Xin-Yu Pan , Gang-Qin Liu

Nitrogen impurities help to stabilize the negatively-charged-state of NV$^-$ in diamond, whereas magnetic fluctuations from nitrogen spins lead to decoherence of NV$^-$ qubits. It is not known what donor concentration optimizes these…

Using fast electron spin resonance spectroscopy of a single nitrogen-vacancy defect in diamond, we demonstrate real-time readout of the Overhauser field produced by its nuclear spin environment under ambient conditions. These measurements…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 A. Dréau , P. Jamonneau , O. Gazzano , S. Kosen , J. -F. Roch , J. R. Maze , V. Jacques

Nanodiamonds containing negatively charged nitrogen vacancy centres (${\text{NV}}^{-}$) have applications as localized sensors in biological material and have been proposed as a platform to probe the macroscopic limits of spatial…

The ability to design quantum systems that decouple from environmental noise sources is highly desirable for development of quantum technologies with optimal coherence. The chemical tunability of electronic states in magnetic molecules…

The available theoretical approaches aiming at describing Dynamic Nuclear spin Polarization (DNP) in solutions containing molecules of biomedical interest and paramagnetic centers are not able to model the behaviour observed upon varying…

Statistical Mechanics · Physics 2014-06-06 Sonia Colombo Serra , Marta Filibian , Pietro Carretta , Alberto Rosso , Fabio Tedoldi

Dynamic nuclear polarization (DNP) is a promising strategy for generating a significantly increased non-thermal spin polarization in nuclear magnetic resonance (NMR) applications thereby circumventing the need for strong magnetic fields.…

Quantum Physics · Physics 2015-07-15 Alexander Karabanov , Daniel Wisniewski , Igor Lesanovsky , Walter Köckenberger

We present systematic measurements of longitudinal relaxation rates ($1/T_1$) of spin polarization in the ground state of the nitrogen-vacancy (NV$^-$) color center in synthetic diamond as a function of NV$^-$ concentration and magnetic…

Quantum Physics · Physics 2015-12-17 A. Jarmola , A. Berzins , J. Smits , K. Smits , J. Prikulis , F. Gahbauer , R. Ferber , D. Erts , M. Auzinsh , D. Budker

In double quantum dots, the exchange interaction between two electron spins renormalizes the excitation energy of pair-flips in the nuclear spin bath, which in turn modifies the non-Markovian bath dynamics. As the energy renormalization…

Mesoscale and Nanoscale Physics · Physics 2008-03-07 W. Yang , R. B. Liu

The central spin decoherence problem has been researched for over 50 years in the context of both nuclear magnetic resonance and electron spin resonance. Until recently, theoretical models have employed phenomenological stochastic…

Mesoscale and Nanoscale Physics · Physics 2012-08-03 Wayne M. Witzel , Malcolm S. Carroll , Lukasz Cywinski , S. Das Sarma

Most of dynamic nuclear polarization (DNP) has been requiring helium cryogenics and strong magnetic fields for a high degree of polarization. In this work, we instead demonstrate an optical hyperpolarization of naturally abundant $^{13}$C…

We present how optical coherent population trapping (CPT) of the spin of localized semiconductor electrons stabilizes the surrounding nuclear spin bath via the hyperfine interaction, resulting in a state which is more ordered than the…

Mesoscale and Nanoscale Physics · Physics 2018-10-17 Alexander R. Onur , Caspar H. van der Wal

This work is a theoretical investigation on the spin-polariton (polarized single photon) entanglement in nitrogen vacancy (NV) centers in diamond in order to interpret the results of two landmark experiments reported by the teams of Buckley…

General Physics · Physics 2012-02-23 Xiaodong Qi
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