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A nitrogen-vacancy (NV) center in a diamond enables the access to an electron spin, which is expected to present highly sensitive quantum sensors. Although exploiting a nitrogen nuclear spin improves the sensitivity, manipulating it using a…

Dynamic nuclear polarization transfers spin polarization from electrons to nuclei. We have achieved this by a new method, simultaneously exciting transitions of electronic and nuclear spins. The efficiency of this technique improves with…

Quantum Physics · Physics 2008-09-11 G. W. Morley , K. Porfyrakis , A. Ardavan , J. van Tol

Experiments suggest that nuclear spins play a significant role in the quantum Hall effect (QHE) near integer and fractional QHE spin transitions, but many of these phenomena still remain to be understood. Here we study theoretically the…

Mesoscale and Nanoscale Physics · Physics 2026-02-03 Haotian Zhou , Yuli Lyanda-Geller

We experimentally isolate, characterize and coherently control up to six individual nuclear spins that are weakly coupled to an electron spin in diamond. Our method employs multi-pulse sequences on the electron spin that resonantly amplify…

Mesoscale and Nanoscale Physics · Physics 2012-10-23 T. H. Taminiau , J. J. T. Wagenaar , T. van der Sar , F. Jelezko , V. V. Dobrovitski , R. Hanson

The ability to optically initialize the electronic spin of the nitrogen-vacancy (NV) center in diamond has long been considered a valuable resource to enhance the polarization of neighboring nuclei, but efficient polarization transfer to…

Mesoscale and Nanoscale Physics · Physics 2018-08-01 F. Shagieva , S. Zaiser , P. Neumann , D. B. R. Dasari , R. Stöhr , A. Denisenko , R. Reuter , C. A. Meriles , J. Wrachtrup

We study the role of dipolar interactions in the standard protocol used to achieve dynamic nuclear polarization (DNP). In the so-called spin-temperature regime, where the interactions establish an effective thermodynamic behavior in the…

Strongly Correlated Electrons · Physics 2016-07-13 Andrea De Luca , Inés Rodríguez Arias , Markus Müller , Alberto Rosso

The negatively charged nitrogen-vacancy centre (NV$^-$) in diamond has been utilized in a wide variety of sensing applications. The centre's long spin coherence and relaxation times ($T_2^*$, $T_2$ and $T_1$) at room temperature are crucial…

The main source of decoherence for an electron spin confined to a quantum dot is the hyperfine interaction with nuclear spins. To analyze this process theoretically we diagonalize the central spin Hamiltonian in the high magnetic B-field…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 Oleksandr Tsyplyatyev , Daniel Loss

Optically addressable molecular triplet spins provide a chemically tunable platform for quantum application, but their coherence is often limited by interactions with surrounding spin baths. Here we demonstrate controlled suppression of…

High-fidelity multi-qubit initialization is vital for quantum simulation, quantum information processing (QIP), and quantum sensing. In diamond platforms, nuclear spin registers can be initialized through polarization transfer from a nearby…

Quantum Physics · Physics 2026-03-02 Soham Pal , Oliver T. Whaites , Wolfgang Knolle , Tania S. Monteiro , Helena S. Knowles

We experimentally resolve several weakly coupled nuclear spins in diamond using a series of novelly designed dynamical decoupling controls. Some nuclear spin signals, hidden by decoherence under ordinary dynamical decoupling controls, are…

Nitrogen-vacancy centres (NVs) in diamond are attractive for research straddling quantum information science and nanoscale magnetometry and thermometry. While ultrapure bulk diamond NVs sustain the longest spin coherence times among…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Helena S. Knowles , Dhiren M. Kara , Mete Atature

Symmetry considerations are used in presenting a model of the electronic structure and the associated dynamics of the nitrogen-vacancy center in diamond. The model accounts for the occurrence of optically induced spin polarization, for the…

Materials Science · Physics 2013-05-29 N. B. Manson , J. P. Harrison , M. J. Sellars

The use of nitrogen-vacancy centers in diamond as a non-invasive platform for hyperpolarizing nuclear spins in molecular samples is a promising area of research with the potential to enhance the sensitivity of nuclear magnetic resonance…

Quantum Physics · Physics 2024-08-08 H. Espinós , C. Munuera-Javaloy , I. Panadero , P. Acedo , R. Puebla , J. Casanova , E. Torrontegui

We present experimental observations and a study of quantum dynamics of strongly interacting electronic spins, at room temperature in the solid state. In a diamond substrate, a single nitrogen vacancy (NV) center coherently interacts with…

Quantum Physics · Physics 2018-06-20 Emma L. Rosenfeld , Linh M. Pham , Mikhail D. Lukin , Ronald L. Walsworth

We develop a theoretical model for transverse dynamics of a single electron spin interacting with a nuclear spin bath. The approach allows a simple diagrammatic representation and analytical expressions of different nuclear spin excitation…

Mesoscale and Nanoscale Physics · Physics 2011-11-09 S. K. Saikin , Wang Yao , L. J. Sham

We propose a method for the estimation of the initial polarization of spinful nuclei of the 13 C isotope in diamond via a measurement of the evolution of the coherence of an NV center spin qubit. Existing polarization measurement methods…

Quantum Physics · Physics 2025-04-01 Mateusz Kuniej , Katarzyna Roszak

We perform a detailed theoretical-experimental study of the dynamical decoupling (DD) of the nitrogen-vacancy (NV) center in diamond. We investigate the DD sequences applied to suppress the dephasing of the electron spin of the NV center…

Quantum Physics · Physics 2012-05-29 Zhi-Hui Wang , G. de Lange , D. Riste , R. Hanson , V. V. Dobrovitski

Control of electron spin decoherence in contact with a mesoscopic bath of many interacting nuclear spins in an InAs quantum dot is studied by solving the coupled quantum dynamics. The nuclear spin bath, because of its bifurcated evolution…

Mesoscale and Nanoscale Physics · Physics 2011-11-09 Ren-Bao Liu , Wang Yao , L. J. Sham

We investigate the spin-coherence decay of NV$^-$-spins interacting with the strongly-coupled bath of nitrogen defects in diamond layers. For thin diamond layers, we demonstrate that the spin-coherence times exceed those of bulk diamond,…

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