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Unlike in many other semiconductors, the band gap of PbTe increases considerably with temperature. We compute the thermoelectric transport properties of n-type PbTe from first principles including the temperature variation of the electronic…

Materials Science · Physics 2019-12-19 Jiang Cao , José D. Querales-Flores , Stephen Fahy , Ivana Savić

Including phonon-assisted inelastic process in thermoelectric devices is able to enhance the performance of nonequilibrium work extraction. In this work, we demonstrate that inelastic phonon-thermoelectric devices have a fertile…

Mesoscale and Nanoscale Physics · Physics 2023-02-24 Jincheng Lu , Zi Wang , Rongqian Wang , Jiebin Peng , Chen Wang , Jian-Hua Jiang

Thermoelectric device is a promising next-generation energy solution owing to its capability to transform waste heat into useful electric energy, which can be realized in materials with high elec- tric conductivities and low thermal…

Materials Science · Physics 2018-07-10 Kisung Chae , Seoung-Hun Kang , Seon-Myeong Choi , Duck Young Kim , Young-Woo Son

The thermoelectric transport through a molecular bridge is discussed, with an emphasis on the effects of inelastic processes of the transport electrons caused by the coupling to the vibrational modes of the molecule. In particular it is…

Mesoscale and Nanoscale Physics · Physics 2015-03-17 O. Entin-Wohlman , Y. Imry , A. Aharony

Thermoelectrics (TE) materials manifest themselves in direct conversion of temperature differences to electric power and vice versa. Despite remarkable advances have been achieved in the past decades for various TE systems, the energy…

Materials Science · Physics 2017-07-11 Yanguang Zhou , Xiaojing Gong , Ben Xu , Ming Hu

Several models of thermionic energy nanoconverters have been proposed to study the transport phenomena that take place in electronic devices. For example, in resonant tunneling junctions those phenomena are manifested through the…

Mesoscale and Nanoscale Physics · Physics 2020-06-02 G. Valencia-Ortega , L. A. Arias-Hernandez

Topological heavy-fermion systems in three dimensions are usually classified as topological insulators or semimetals. Here, we theoretically predict a different type of heavy-fermion system (dubbed exceptional heavy-fermion semimetal) by…

Strongly Correlated Electrons · Physics 2023-02-01 Yu-Liang Tao , Tao Qin , Yong Xu

We study the electronic transport coefficients and the thermoelectric figure of merit ZT in $n$-doped Mg$_3$Sb$_2$ based on density-functional electronic structure and Bloch-Boltzmann transport theory with an energy- and…

Materials Science · Physics 2019-01-07 Roberta Farris , Maria Barbara Maccioni , Alessio Filippetti , Vincenzo Fiorentini

We present a detailed study of the non-linear thermoelectric properties of a molecular junction, represented by a dissipative Anderson-Holstein model. A single orbital level with strong Coulomb interaction is coupled to a localized…

Mesoscale and Nanoscale Physics · Physics 2013-01-10 M. Leijnse , M. R. Wegewijs , K. Flensberg

Whether porosity can effectively improve thermoelectric performance is still an open question. Herein we report that thermoelectric performance can be significantly enhanced by creating porosity in n-type Mg3.225Mn0.025Sb1.5Bi0.49Te0.01,…

Thermal energy can be directly converted to electrical energy as a result of thermoelectric effects. Because this conversion realises clean energy technology, such as waste heat recovery and energy harvesting, substantial efforts have been…

Materials Science · Physics 2023-03-30 Byungki Ryu , Jaywan Chung , SuDong Park

We predict high thermoelectric efficiency in the layered perovskite La$_2$Ti$_2$O$_7$, based on calculations (mostly ab-initio) of the electronic structure, transport coefficients, and thermal conductivity in a wide temperature range. The…

Materials Science · Physics 2019-03-06 Vincenzo Fiorentini , Roberta Farris , Edoardo Argiolas , Maria Barbara Maccioni

Enhancing the dimensionless figure of merit zT is central to developing better thermoelectric materials and advancing thermoelectric generation technology. However, the intrinsic interdependence between electrical conductivity, the Seebeck…

Materials Science · Physics 2024-12-20 D. Beretta

The thermoelectric properties of polythiophene (PT) coupled to the Au (111) electrodes are studied based on density functional theory combined with nonequilibrium Green function formalism. Specially, the effect of Li and Cl adsorbents on…

Mesoscale and Nanoscale Physics · Physics 2018-04-04 Zahra Golsanamlou , Meysam Bagheri Tagani , Hamid Rahimpour Soleimani

The thermoelectric properties of n type semiconductor, TiNiSn is optimized by partial substitution with metallic, MnNiSb in the half Heusler structure. Herein, we study the transport properties and intrinsic phase separation in the system.…

Disordered Systems and Neural Networks · Physics 2016-12-06 T. Berry , S. Ouardi , G. H. Fecher , B. Balke , G. Kreiner , G. Auffermann , W. Schnelle , C. Felser

Materials exhibiting topological order host exotic phenomena that could form the basis for novel developments in areas ranging from low-power electronics to quantum computers. The past decade has witnessed multiple experimental realizations…

Materials Science · Physics 2019-10-23 Bo Peng , Ivona Bravić , Judith L. MacManus-Driscoll , Bartomeu Monserrat

Molecular junctions are a versatile test bed for investigating thermoelectricity on the nanoscale1-10 and contribute to the design of new cost-effective environmentally-friendly organic thermoelectric materials11. It has been suggested that…

We predict an enormous order-dependent quantum enhancement of thermoelectric effects in the vicinity of a higher-order `supernode' in the transmission spectrum of a nanoscale junction. Single-molecule junctions based on 3,3'-biphenyl and…

Mesoscale and Nanoscale Physics · Physics 2011-08-04 J. P. Bergfield , M. Solis , C. A. Stafford

The response of electric devices to an applied thermal gradient has, so far, been studied almost exclusively in two-terminal devices. Here we present measurements of the response to a thermal bias of a four-terminal, quasi-ballistic…

Mesoscale and Nanoscale Physics · Physics 2012-06-15 Jason Matthews , David Sánchez , Marcus Larsson , Heiner Linke

The electronic and thermoelectric properties of molecular junctions formed from iron and ruthenium metal-acetylide were studied using complementary experimental techniques and quantum chemical simulations. We performed physical…

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