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We employed first-principles calculations to investigate the thermoelectric transport properties of the compound As$_2$Se$_3$. Early experiments and calculations have indicated that these properties are controlled by a kind of native defect…

Materials Science · Physics 2023-07-27 Anderson S. Chaves , Murilo Aguiar Silva , Alex Antonelli

Theoretical analysis of the effect of thermoelectric phenomena on the relation of effective electrical and thermal conductivity in the macroscopically inhomogeneous media is carried out. Plane-layered structures, two-dimensional self-dual…

Materials Science · Physics 2011-09-09 A. A. Snarskii , M. I. Zhenirovskii , I. V. Bezsudnov

Thermoelectrics are a promising class of materials for renewable energy owing to their capability to generate electricity from waste heat, with their performance being governed by a competition between charge and thermal transport. A…

A first-principles approach is presented for the thermoelectricity in molecular junctions formed by a single molecule contact. The study investigates the Seebeck coefficient considering the source-drain electrodes with distinct temperatures…

Mesoscale and Nanoscale Physics · Physics 2009-05-07 Yu-Shen Liu , Yu-Chang Chen

A three terminal nanoscale refrigeration concept based on a vibron-coupled quantum dot hybrid system coupled to two electronic reservoirs and a phonon bath is proposed and analyzed in detail. While investigating the non-trivial role of…

Mesoscale and Nanoscale Physics · Physics 2021-02-03 Swarnadip Mukherjee , Bitan De , Bhaskaran Muralidharan

N-type Bi100-xSbx alloys have the highest thermoelectric figure of merit (zT) of all materials below 200K; here we investigate how filling multiple valence band pockets at T and H-points of the Brillouin zone produces high zT in p-type…

Materials Science · Physics 2013-08-13 Hyungyu Jin , Christopher M. Jaworski , Joseph P. Heremans

We study the resistivity of three-dimensional semimetals with linear dispersion in the presence of on-site electron-electron interaction. The well-known quadratic temperature dependence of the resistivity of conventional metals is turned…

Strongly Correlated Electrons · Physics 2021-05-26 Niklas Wagner , Sergio Ciuchi , Alessandro Toschi , Björn Trauzettel , Giorgio Sangiovanni

Recently SnSe compound was reported to have a peak thermoelectric figure-5 of-merit (ZT) of 2.62 at 923 K, but the ZT values at temperatures below 750 K are relatively low. In this work, the electronic structures of SnSe are calculated…

Materials Science · Physics 2015-04-09 Aijun Hong , Lin Li , Haixia Zhu , Zhibo Yan , Junming Liu , Zhifeng Ren

Non-symmetric variants of self-consistent field theory are proposed that served the basis for theoretical investigation of the effect of thermal conductivity of composite particles surface layers on the effective thermoelectric figure of…

Materials Science · Physics 2011-08-30 A. A. Snarskii , M. I. Zhenirovskyy

Recent experimental investigations have demonstrated that doping a semiconductor is a route to increase the thermal boundary conductance at metal/semiconductor interfaces. In this work, the influence of the electrical properties on heat…

In this work, we report the fabrication of a high temperature measurement setup to measure Figure of merit (ZT). This setup facilitates the simultaneous measurement of Seebeck coefficient ({\alpha}), thermal conductivity (\kappa), and…

Instrumentation and Detectors · Physics 2018-01-09 Ashutosh Patel , Sudhir K. Pandey

The correlated couple of electrical and thermal property is the challenge to realize a substantial leap in thermoelectric materials.Synthesis of semiconductor and metal composites is a significant and versatile design strategy to optimize…

Applied Physics · Physics 2018-05-23 Wenwen Zheng , Peng Bi , Fengming Liu , Yong Liu , Jing Shi , Rui Xiong , Ziyu Wang

The intense research for efficient low-temperature thermoelectric materials motivates the exploration of innovative compounds and composite systems. This study examines the effects of integrating low-dimensional titanium trisulfide…

We review many-body effects, their microscopic origin, as well as their impact onto thermoelectricity in correlated narrow-gap semiconductors. Members of this class---such as FeSi and FeSb$_2$---display an unusual temperature dependence in…

Strongly Correlated Electrons · Physics 2018-04-11 Jan M. Tomczak

In this paper, general relationships that allow evaluating the figure of merit of both two-dimensional superlattices and three-dimensional crystals with a quadratic and isotropic energy spectrum of free charge carriers are derived. It is…

Mesoscale and Nanoscale Physics · Physics 2015-11-03 P. V. Gorskyi

The principles of the thermoelectric phenomenon, including Seebeck effect, Peltier effect, and Thomson effect are discussed. The dependence of the thermoelectric devices on the figure of merit, Seebeck coefficient, electrical conductivity,…

Materials Science · Physics 2017-06-29 Ibrahim M Abdel-Motaleb , Syed M. Qadri

We investigate thermoelectric transport through interfaces with inelastic scatterings by developing a quantum theory, which has been extensively validated by existing theories. We find that under temperature bias, while a two-terminal…

Mesoscale and Nanoscale Physics · Physics 2020-07-01 Hangbo Zhou , Gang Zhang , Jian-Sheng Wang , Yong-Wei Zhang

A three-level system attached to three thermal baths is manipulated to be a microscopic thermal device integrating a valve, a refrigerator, an amplifier, and a thermometer in the quantum regime, via tuning the inner coupling strength of the…

Quantum Physics · Physics 2021-01-27 Yong Huangfu , Shifan Qi , Jun Jing

We present a model for P-N-P abrupt heterostructures vertical to temperature gradient to improve the thermoelectric performance. The P-N-P heterostructure is considered as an abrupt bipolar junction transistor due to an externally applied…

Materials Science · Physics 2020-09-24 Bohang Nan , Guiying Xu , Quanxin Yang , Tao Guo

Recent studies have shown the potential for bipolar thermoelectricity in superconducting tunnel junctions with asymmetric energy gaps. The thermoelectric performance of these systems is significantly impacted by the inverse proximity…

Mesoscale and Nanoscale Physics · Physics 2023-06-14 A. Hijano , F. S. Bergeret , F. Giazotto , A. Braggio