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Over the last few years, Sr$_2$IrO$_4$, a single-layer member of the Ruddlesden-Popper series iridates, has received much attention as a close analog of cuprate high-temperature superconductors. Although there is not yet firm evidence for…

Strongly Correlated Electrons · Physics 2019-02-15 Joel Bertinshaw , Y. K. Kim , Giniyat Khaliullin , B. J. Kim

The Ruddlesden-Popper (RP) series of iridates (Srn+1IrnO3n+1) have been the subject of much recent attention due to the anticipation of emergent physics arising from the cooperative action of spin-orbit (SO) driven band splitting and…

Layered perovskite iridates realize a rare class of Mott insulators that are predicted to be strongly spin-orbit coupled analogues of the parent state of cuprate high-temperature superconductors. Recent discoveries of pseudogap, magnetic…

Strongly Correlated Electrons · Physics 2017-04-25 H. Chu , L. Zhao , A. de la Torre , T. Hogan , S. D. Wilson , D. Hsieh

A rare combination of strong spin-orbit coupling and electron-electron correlations makes the iridate Mott insulator Sr$_2$IrO$_4$ a promising host for novel electronic phases of matter. The resemblance of its crystallographic, magnetic and…

Strongly Correlated Electrons · Physics 2016-01-11 L. Zhao , D. H. Torchinsky , H. Chu , V. Ivanov , R. Lifshitz , R. Flint , T. Qi , G. Cao , D. Hsieh

The similarities to cuprates make iridates an interesting potential platform for investigating superconductivity. Equally attractive are their puzzling complex intrinsic interactions. Here, we report an ultrafast optical spectroscopy…

Strongly Correlated Electrons · Physics 2019-04-02 L. L. Hu , M. Yang , Y. L. Wu , Q. Wu , H. Zhao , F. Sun , W. Wang , Rui He , S. L. He , H. Zhang , R. J. Huang , L. F. Li , Y. G. Shi , Jimin Zhao

Neutron diffraction measurements are presented exploring the magnetic and structural phase behaviors of the candidate J$_{eff}=1/2$ Mott insulating iridate Sr$_2$IrO$_4$. Comparisons are drawn between the correlated magnetism in this single…

Strongly Correlated Electrons · Physics 2013-04-09 Chetan Dhital , Tom Hogan , Z. Yamani , Clarina de la Cruz , Xiang Chen , Sovit Khadka , Zhensong Ren , Stephen D. Wilson

The motion of doped electrons or holes in an antiferromagnetic lattice with strong on-site Coulomb interactions touches one of the most fundamental open problems in contemporary condensed matter physics. The doped charge may strongly couple…

The semi-metallic behavior of the perovskite iridate SrIrO3 shifts the end-member of the strongly spin-orbit (SO) coupled Ruddlesden-Popper series Srn+1IrnO3n+1 away from the Mott insulating regime and the half-filled pseudospin Jeff=1/2…

Strongly Correlated Electrons · Physics 2025-02-06 Dirk Fuchs , Arun Kumar Jaiswal , Fabrice Wilhelm , Di Wang , Andre Rogalev , Matthieu Le Tacon

The spin-orbit Mott insulator Sr${}_2$IrO${}_4$ has attracted a lot of interest in recent years from theory and experiment due to its close connection to isostructural high-temperature copper oxide superconductors. Despite of not being…

Strongly Correlated Electrons · Physics 2019-05-22 Benjamin Lenz , Cyril Martins , Silke Biermann

Here we report on the low-energy excitations within the paramagnetic spin-orbit insulator Sr$_3$Ir$_2$O$_7$F$_2$ studied via resonant inelastic X-ray scattering, \textit{ab initio} quantum chemical calculations, and model-Hamiltonian…

Strongly Correlated Electrons · Physics 2022-09-26 Zach Porter , Paul M. Sarte , Thorben Petersen , Mary H. Upton , Liviu Hozoi , Stephen D. Wilson

Novel phases of two dimensional electron systems resulting from new surface or interface modified electronic structures have generated significant interest in material science. We utilize photoemission spectroscopy to show that the…

Sr$_2$IrO$_4$ has attracted a lot of attention due to its structural and electronic similarities to La$_2$CuO$_4$ which is the parent compound of high-T$_c$ superconducting cuprates. It was proposed to be a strong spin-orbit coupled…

$\rm Sr_2IrO_4$ is an archetypal spin-orbit-coupled Mott insulator and has been extensively studied in part because of a wide range of predicted novel states. Limited experimental characterization of these states thus far brings to light…

Strongly Correlated Electrons · Physics 2020-09-14 Feng Ye , Christina Hoffmann , Wei Tian , Hengdi Zhao , G. Cao

The combination of strong spin-orbit coupling and Coulomb interactions makes the $5d$ iridates a unique platform for realizing novel correlated electronic states. Here, utilizing infrared spectroscopy, we demonstrate that a robust Mott…

Strongly Correlated Electrons · Physics 2026-03-06 Kai Wang , Jun Yang , Chaoyang Kang , Weikang Wu , Wenka Zhu , Jianzhou Zhao , Yaomin Dai , Bing Xu

Recent years have seen many examples of how the strong spin-orbit coupling (SOC) present in iridates can stabilize new emergent states that are difficult or impossible to realize in more conventional materials. In this review we outline a…

Strongly Correlated Electrons · Physics 2019-06-10 Lin Hao , D. Meyers , M. P. M. Dean , Jian Liu

We investigate the electronic structure at the surface of the correlated oxide Ca$_3$Ru$_2$O$_7$, a low-symmetry ruthenate oxide which hosts an unconventional polar-metal phase. From a combination of angle-resolved photoemission…

We study possible superconductivity in a carrier-doped iridium oxide insulator Sr$_{2}$IrO$_{4}$ based on an effective $t_{2g}$ three-orbital Hubbard model on the square lattice with a large spin-orbit coupling (SOC). Numerically solving…

Superconductivity · Physics 2019-09-02 Kazutaka Nishiguchi , Tomonori Shirakawa , Hiroshi Watanabe , Ryotaro Arita , Seiji Yunoki

We report on the tuning of magnetic interactions in superlattices composed of single and bilayer SrIrO$_3$ inter-spaced with SrTiO$_3$. Magnetic scattering shows predominately $c$-axis antiferromagnetic orientation of the magnetic moments…

We report high-resolution spin-resolved photoemission spectroscopy (Spin-ARPES) measurements on the parent compound Sb of the recently discovered 3D topological insulator Bi1-xSbx [D. Hsieh et al., Nature 452, 970 (2008)]. By modulating the…

Mesoscale and Nanoscale Physics · Physics 2010-01-12 D. Hsieh , L. A. Wray , D. Qian , Y. Xia , Y. S. Hor , R. J. Cava , M. Z. Hasan

Through a neutron scattering, charge transport, and magnetization study, the correlated ground state in the bilayer iridium oxide Sr$_3$Ir$_2$O$_7$ is explored. Our combined results resolve scattering consistent with a high temperature…

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