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To examine the insulating mechanism of 5$d$ transition metal oxide Sr$_2$IrO$_4$, we study the ground state properties of a three-orbital Hubbard model with a large relativistic spin-orbit coupling on a square lattice. Using a variational…

Strongly Correlated Electrons · Physics 2014-09-22 Hiroshi Watanabe , Tomonori Shirakawa , Seiji Yunoki

Majority of the A$_2$B$_3$ type chalcogenide systems with strong spin-orbit coupling, like Bi$_2$Se$_3$, Bi$_2$Te$_3$ and Sb$_2$Te$_3$ etc., are topological insulators. One important exception is Sb$_2$Se$_3$, where a topological…

Mesoscale and Nanoscale Physics · Physics 2018-06-13 Shekhar Das , Suman Kamboj , Anshu Sirohi , Aastha Vasdev , Sirshendu Gayen , Prasenjit Guptasarma , Goutam Sheet

We study the optical properties of the Ruddlesden-Popper series of iridates Sr$_{n+1}$Ir$_n$O$_{3n+1}$ ($n$=1, 2 and $\infty$) by solving the Bethe-Salpeter equation (BSE), where the quasiparticle (QP) energies and screened interactions $W$…

Strongly Correlated Electrons · Physics 2018-08-08 Peitao Liu , Bongjae Kim , Xing-Qiu Chen , D. D. Sarma , Georg Kresse , Cesare Franchini

The effect of isoelectronic substitution within single crystals of (Sr1-xCax)2-yIrO4+z is explored. The nominal n=1 Ruddlesden-Popper phase with y=0, z=0 remains stable from x=0 until x=0.11, where the antiferromagnet spin-orbit Mott…

Materials Science · Physics 2016-11-23 Xiang Chen , Stephen D. Wilson

The interplay of spin-orbit interactions and electronic correlations dominates the physical properties of pyrochlore iridates, R2Ir2O7 (R = Y, rare earth element), which are typically magnetic insulators. We report an…

Strongly Correlated Electrons · Physics 2015-06-03 T. F. Qi , O. B. Korneta , Xiangang Wan , L. E. DeLong , P. Schlottmann , G. Cao

The pseudogap, d-wave superconductivity and electron-boson coupling are three intertwined key ingredients in the phase diagram of the cuprates. Sr$_2$IrO$_4$ is a 5d-electron counterpart of the cuprates in which both the pseudogap and a…

We study the electronic spectral properties in two examples of strongly interacting systems: a Mott-Hubbard insulator with additional electron-boson interactions, and a polaronic semiconductor. An approximate unified framework is developed…

Strongly Correlated Electrons · Physics 2009-11-11 S. Fratini , S. Ciuchi

For iridates with large spatially extended 5d orbitals, it may be anticipated that distant neighbor interactions would play a crucial role in their ground state properties. From this perspective, we investigate the magnetic structure of…

Materials Science · Physics 2019-09-04 Vijeta Singh , J. J. Pulikkotil

We report high-resolution spin-resolved photoemission spectroscopy (Spin-ARPES) measurements on the parent compound Sb of the first discovered 3D topological insulator Bi{1-x}Sb{x} [D. Hsieh et al., Nature 452, 970 (2008) Submitted 2007].…

Mesoscale and Nanoscale Physics · Physics 2011-03-18 D. Hsieh , Y. Xia , L. Wray , D. Qian , J. H. Dil , F. Meier , L. Patthey , J. Osterwalder , G. Bihlmayer , Y. S. Hor , R. J. Cava , M. Z. Hasan

The unusual magnetic and electronic ground states of 5d iridates has been shown to be driven by intrinsically enhanced spin-orbit coupling (SOC). The influence of appreciable but reduced SOC in creating the manifested magnetic insulating…

Strongly Correlated Electrons · Physics 2015-12-01 S. Calder , L. Li , S. Okamoto , Y. Choi , R. Mukherjee , D. Haskel , D. Mandrus

Many complex electronic systems exhibit so-called pseudogaps, which are poorly-understood suppression of low-energy spectral intensity in the absence of an obvious gap-inducing symmetry. Here we investigate the superconductor…

A new iridium containing layered cuprate material, IrSr_2Sm_{1.15}Ce_{0.85}Cu_{2.175}O_{10, has been synthesized by conventional ambient-pressure solid-state techniques. The material's structure has been fully characterized by Rietveld…

Materials Science · Physics 2012-09-22 R. H. Colman , A. C. Mclaughlin

We have carried out a detailed first-principles study of a d$^{4.5}$ quaternary iridate Ba$_3$YIr$_2$O$_9$ both in its 6H-perovskite-type ambient pressure (AP) phase and also for the high pressure (HP) cubic phase. Our analysis reveals that…

Strongly Correlated Electrons · Physics 2015-11-11 S. K. Panda , S. Bhowal , Ying Li , S. Ganguly , Roser Valentí , L. L. Nordström , I. Dasgupta

Polaronic features similar to those previously observed in the photoinduced spectra of cuprates have been detected in the reflectivity spectra of chemically doped parent compounds of high-critical-temperature superconductors, both $n$-type…

supr-con · Physics 2009-10-28 P. Calvani , M. Capizzi , S. Lupi , P. Maselli , A. Paolone , P. Roy

The nature of insulating phase in 5$d$ based Sr$_2$IrO$_4$ is quite debated as the theoretical as well as experimental investigations have put forward evidences in favor of both magnetically driven Slater-type and interaction driven…

Strongly Correlated Electrons · Physics 2017-02-08 Imtiaz Noor Bhatti , A. K. Pramanik

We perform a time-resolved optical study of Sr$_2$IrO$_4$ to understand the influence of magnetic ordering on the low energy electronic structure of a strongly spin-orbit coupled $J_{eff}$=1/2 Mott insulator. By studying the recovery…

Strongly Correlated Electrons · Physics 2012-03-21 D. Hsieh , F. Mahmood , D. H. Torchinsky , G. Cao , N. Gedik

Sr$_{2}$IrO$_{4}$ has often been described via a simple, one-band pseudo-spin 1/2 model, subject to electron-electron interactions, on a square lattice, fostering analogies with cuprate superconductors, believed to be well described by a…

Recently, strong reduction of the quasiparticle peaks and pronounced incoherent structures have been observed in the photoemission spectra of layered cobaltates. Surprisingly, these many-body effects are found to increase near the band…

Strongly Correlated Electrons · Physics 2009-11-13 J. Chaloupka , G. Khaliullin

Strong spin-orbit coupling fosters exotic electronic states such as topological insulators and superconductors, but the combination of strong spin-orbit and strong electron-electron interactions is just beginning to be understood. Central…

We report on the selective fabrication of high-quality Sr$_2$IrO$_4$ and SrIrO$_3$ epitaxial thin films from a single polycrystalline Sr$_2$IrO$_4$ target by pulsed laser deposition. Using a combination of X-ray diffraction and…

Strongly Correlated Electrons · Physics 2017-12-25 Xiaoran Liu , Yanwei Cao , B. Pal , S. Middey , M. Kareev , Y. Choi , P. Shafer , D. Haskel , E. Arenholz , J. Chakhalian