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Through ultrafast pump-probe spectroscopy with intense pump pulses and a wide continuum probe, we show that interband exciton peaks in single-walled carbon nanotubes (SWNTs) are extremely stable under high laser excitations. Estimates of…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 G. N. Ostojic , S. Zaric , J. Kono , V. C. Moore , R. H. Hauge , R. E. Smalley

We study both experimentally and theoretically the fundamental interplay of exciton localization and polarization in semiconducting single-walled carbon nanotubes. From Stark spectroscopy of individual carbon nanotubes at cryogenic…

We report a femtosecond mid-infrared study of the broadband low-energy response of individually separated (6,5) and (7,5) single-walled carbon nanotubes. Strong photoinduced absorption is observed around 200 meV, whose transition energy,…

Mesoscale and Nanoscale Physics · Physics 2010-07-16 Jigang Wang , Matt W. Graham , Yingzhong Ma , Graham R. Fleming , Robert A. Kaindl

Spatiotemporal dynamics of electron-hole pairs locally excited in a silicon-on-insulator structure by indirect interband absorption are studied by measuring differential transmission caused by free-carrier absorption of a probe pulse tuned…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Hui Zhao

We demonstrate a possibility for exciton Bose-Einstein condensation in individual small-diameter (~1-2 nm) semiconducting carbon nanotubes. The effect occurs under the exciton-interband-plasmon coupling controlled by an external…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 I. V. Bondarev , A. V. Meliksetyan

We present a quantitative theory of optical absorption polarized transverse to the tube axes in semiconducting single-walled carbon nanotubes. Transverse optical absorption in semiconducting single-walled carbon nanotubes is to an exciton…

Materials Science · Physics 2009-11-13 Zhendong Wang , Hongbo Zhao , Sumit Mazumdar

Single-walled carbon nanotubes (SWCNTs) are quasi-one-dimensional systems with poor Coulomb screening and enhanced electron-phonon interaction, and are good candidates for excitons and exciton-phonon couplings in metallic state. Here we…

Materials Science · Physics 2009-04-20 Hualing Zeng , Hongbo Zhao , Fu-Chun Zhang , Xiaodong Cui

Microwave treated water soluble and amide functionalized single walled carbon nanotubes have been investigated using femtosecond degenerate pump-probe and nonlinear transmission experiments. The time resolved differential transmission using…

The picosecond dynamics of excitons in colloidal CdSe nanorods are directly measured via their 1s to 2p-like internal transitions by ultra-broadband terahertz spectroscopy. Broadened absorption peaks from both the longitudinal and…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 David G. Cooke , Peter Uhd Jepsen , Jun Yan Lek , Yeng Ming Lam , Fredrik Sy , Marc M. Dignam

Electroabsorption spectroscopy of well-identified index-defined semiconducting carbon nanotubes is reported. The measurement of high definition electroabsorption spectra allows direct indexation with unique nanotube chirality. Results show…

We present a detailed electron diffraction study of individual single-walled carbon nanotubes. A novel sample preparation procedure provides well-separated, long and straight individual single-shell nanotubes. Diffraction experiments are…

Materials Science · Physics 2007-05-23 Jannik C. Meyer , Matthieu Paillet , Georg S. Duesberg , Siegmar Roth

We report optical studies of quantum dot excitons in individual suspended carbon nanotubes at cryogenic temperatures. Narrow optical linewidths, strongly suppressed spectral wandering, and photoluminescence lifetimes in the range of…

Mesoscale and Nanoscale Physics · Physics 2014-10-03 Matthias S. Hofmann , Jan T. Glückert , Alexander Högele

We present direct experimental observation of exciton-phonon bound states in the photoluminescence excitation spectra of isolated single walled carbon nanotubes in aqueous suspension. The photoluminescence excitation spectra from several…

Materials Science · Physics 2009-11-11 Flavio Plentz , Henrique B. Ribeiro , Ado Jorio , Marcos A. Pimenta , Michael S. Strano

We calculate the radiative lifetime and energy bandstructure of excitons in semiconducting carbon nanotubes, within a tight-binding approach. In the limit of rapid interband thermalization, the radiative decay rate is maximized at…

Materials Science · Physics 2015-06-25 Vasili Perebeinos , J. Tersoff , Phaedon Avouris

We present the numerical tool DECaNT (Diffusion of Excitons in Carbon NanoTubes) that simulates exciton transport in thin films of carbon nanotubes. Through a mesh of nanotubes generated using the Bullet Physics C++ library, excitons move…

Mesoscale and Nanoscale Physics · Physics 2021-04-01 S. W. Belling , Y. C. Li , A. H. Davoody , A. J. Gabourie , I. Knezevic

We have investigated ultrafast carriers dynamics in crystalline silicon nano-pillars structure using a pump-probe reflectivity method with 800 nm, 150 fs laser pulses and fluence in the range of {17 - 170} mJ/cm^2. Dimensions of the…

Materials Science · Physics 2009-02-06 D. Chekulaev , A. Kaplan

By means of analytical calculations and numerical simulations we study the diffusion properties in quasi-two-dimensional structures with two exciton subsystems with an exchange between them. The experimental realisation is possible in…

Statistical Mechanics · Physics 2024-07-18 Oluwafemi P. Adejumobi , Vladimir N. Mantsevich , Vladimir V. Palyulin

An analytical expression is obtained for the biexciton binding energy as a function of the inter-exciton distance and binding energy of constituent quasi-one-dimensional excitons in carbon nanotubes. This allows one to trace biexciton…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 I. V. Bondarev

The optical absorption spectrum of the carbon (4,2) nanotube is computed using an ab-initio many-body approach which takes into account excitonic effects. We develop a new method involving a local basis set which is symmetric with respect…

Materials Science · Physics 2009-11-10 Eric Chang , Giovanni Bussi , Alice Ruini , Elisa Molinari

We study theoretically the interactions of excitonic states with surface electromagnetic modes of small-diameter (~1 nm) semiconducting single-walled carbon nanotubes. We show that these interactions can result in strong…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 I. V. Bondarev , K. Tatur , L. M. Woods