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Near-infrared magneto-optical spectroscopy of single-walled carbon nanotubes reveals two absorption peaks with an equal strength at high magnetic fields ($>$ 55 T). We show that the peak separation is determined by the Aharonov-Bohm phase…

One- and two-photon luminescence excitation spectroscopy showed a series of distinct excitonic states in single-walled carbon nanotubes. The energy splitting between one- and two-photon-active exciton states of different wavefunction…

Materials Science · Physics 2007-05-23 J. Maultzsch , R. Pomraenke , S. Reich , E. Chang , D. Prezzi , A. Ruini , E. Molinari , M. S. Strano , C. Thomsen , C. Lienau

We report a detailed analysis of the optical properties of single wall carbon nanotubes with different mean diameters as produced by laser ablation. From a combined study of optical absorption, high resolution electron energy-loss…

Materials Science · Physics 2009-11-07 X. Liu , T. Pichler , M. Knupfer , M. S. Golden , J. Fink , H. Kataura , Y. Achiba

The absorption cross section of highly luminescent individual single-walled carbon nanotubes is determined using time-resolved and cw luminescence spectroscopy. A mean value of 1x10-17 cm2 per carbon atom is obtained for (6,5) tubes excited…

Materials Science · Physics 2009-01-08 Stephane Berciaud , Laurent Cognet , Brahim Lounis

The conduction of a single-wall carbon nanotube depends on the pitch. If there are an integral number of carbon hexagons per pitch, then the system is periodic along the tube axis and allows "holes" (, and not "electrons",) to move inside…

Mesoscale and Nanoscale Physics · Physics 2010-03-30 S. Fujita , S. Moon , Y. Takato , James McNabb , S. Godoy

We investigate the ultrafast dynamics of excitons in a 2.6 nm-thick $\mathrm{ZnO/Zn_{0.84}Mg_{0.16}O}$ quantum well grown on a c-axis sapphire substrate, using non-degenerate time-resolved pump-probe spectroscopy. A pump pulse at 266 nm…

A (10x10) single-walled carbon nanotube consisting of 400 atoms with 20 layers is simulated under tensile loading using our developed O(N) parallel tight-binding molecular-dynamics algorithms. It is observed that the simulated carbon…

Condensed Matter · Physics 2009-11-10 G. Dereli , C. Ozdogan

A single-walled carbon nanotube presents a seamless cylindrical graphene surface and is thus an ideal adsorption substrate for investigating the physics of atoms and molecules in two dimensions and approaching the one-dimensional limit.…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 Boris Dzyubenko , Hao-Chun Lee , Oscar E. Vilches , David H. Cobden

Comparative studies of the resonant transmission of light in the vicinity of exciton resonances, measured for 15 few-micron GaAs crystal slabs with different impurity concentrations $N$, reveal an unexpected tendency. While $N$ spans almost…

Mesoscale and Nanoscale Physics · Physics 2015-01-13 D. A. Zaitsev , N. D. Ilinskaya , A. V. Koudinov , N. K. Poletaev , A. Yu. Egorov , A. V. Kavokin , R. P. Seisyan

We consider a semi-infinite dielectric with multiple spatially dispersive resonances in the susceptibility. The effect of the boundary is described by an arbitrary reflection coefficient for polarization waves in the material at the…

Optics · Physics 2017-05-10 R. J. Churchill , T. G. Philbin

We have combined spatially-resolved steady-state micro-photoluminescence ($\mu$PL) with time-resolved photoluminescence (TRPL) to investigate the exciton diffusion in a WSe$_2$ monolayer encapsulated with hexagonal boron nitride (hBN). At…

Mesoscale and Nanoscale Physics · Physics 2018-05-09 F. Cadiz , C. Robert , E. Courtade , M. Manca , L. Martinelli , T. Taniguchi , K. Watanabe , T. Amand , A. C. H. Rowe , D. Paget , B. Urbaszek , X. Marie

Nanomaterials exhibit unique optical phenomena, in particular excitonic quantum processes occurring at room temperature. The low dimensionality, however, imposes strict requirements for conventional optical excitation, and an approach for…

Mesoscale and Nanoscale Physics · Physics 2023-12-15 N. Fang , D. Yamashita , S. Fujii , M. Maruyama , Y. Gao , Y. R. Chang , C. F. Fong , K. Otsuka , K. Nagashio , S. Okada , Y. K. Kato

We have investigated excitons in highly-aligned single-walled carbon nanotubes (SWCNTs) through optical spectroscopy at low temperature (1.5 K) and high magnetic fields ($\textbf{\textit{B}}$) up to 55 T. SWCNT/polyacrylic acid films were…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 J. Shaver , S. A. Crooker , J. A. Fagan , E. K. Hobbie , N. Ubrig , O. Portugall , V. Perebeinos , Ph. Avouris , J. Kono

Femtosecond optical pump-probe technique is used to study charge carrier dynamics in few-layer MoS2 samples fabricated by mechanical exfoliation. An ultrafast pump pulse excites carriers and differential reflection of a probe pulse tuned to…

Mesoscale and Nanoscale Physics · Physics 2011-11-01 Rui Wang , Brian A. Ruzicka , Nardeep Kumar , Matthew Z. Bellus , Hsin-Ying Chiu , Hui Zhao

We examine the excitonic nature of high-lying optical transitions in single-walled carbon nanotubes by means of Rayleigh scattering spectroscopy. A careful analysis of the principal transitions of individual semiconducting and metallic…

Mesoscale and Nanoscale Physics · Physics 2010-01-27 Stephane Berciaud , Christophe Voisin , Hugen Yan , Bhupesh Chandra , Robert Caldwell , Yuyao Shan , Louis E. Brus , James Hone , Tony F. Heinz

Resonant Raman spectroscopy of single carbon nanotubes suspended across trenches displays red shifts of up to 30 meV of the electronic transition energies as a function of the surrounding dielectric environment. We develop a simple scaling…

Light emission from carbon nanotubes is expected to be dominated by excitonic recombination. Here we calculate the properties of excitons in nanotubes embedded in a dielectric, for a wide range of tube radii and dielectric environments. We…

Materials Science · Physics 2009-11-10 Vasili Perebeinos , J. Tersoff , Phaedon Avouris

Carbon nanotubes are quantum sources whose emission can be tuned at telecommunication wavelengths by choosing the diameter appropriately. Most applications require the smallest possible linewidth. Therefore, the study of the underlying…

Mesoscale and Nanoscale Physics · Physics 2015-03-19 V. Ardizzone , Y. Chassagneux , F. Vialla , G. Delport , C. Delcamp , N. Belabas , E. Deleporte , Ph. Roussignol , I. Robert-Philip , C. Voisin , J. S. Lauret

We report that dark excitons can have a large contribution to the emission intensity in carbon nanotubes due to an efficient exciton conversion from a dark state to a bright state. Time-resolved photoluminescence measurements are used to…

Mesoscale and Nanoscale Physics · Physics 2019-12-11 A. Ishii , H. Machiya , Y. K. Kato

Coherence transfer is a multi-disciplinary topic of interest, including chemistry, biology and physics. In quantum technologies, achieving non-local coherent coupling between solid-state qubits is of the utmost importance. Here, we…