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Oxide heterostructures are of great interest both for fundamental and applicative reasons. In particular the two-dimensional electron gas at the LaAlO$_3$/SrTiO$_3$ or LaTiO$_3$/SrTiO$_3$ interfaces displays many different physical…

Mesoscale and Nanoscale Physics · Physics 2016-01-20 N. Scopigno , D. Bucheli , S. Caprara , J. Biscaras , N. Bergeal , J. Lesueur , M. Grilli

Interface structure at polar/non-polar interfaces has been shown to be a key factor in controlling emergent behavior in oxide heterostructures, including the LaFeO$_3$/$\textit{n}$-SrTiO$_3$ system. We demonstrate via high energy resolution…

Materials Science · Physics 2016-11-28 Ryan Comes , Scott Chambers

Understanding and controlling the growth of chalcogenide perovskite thin films through interface design is important for tailoring film properties. Here, the film and interface structure of BaZr(S,Se)$_3$ thin films grown on LaAlO$_3$ by…

Materials Science · Physics 2024-08-01 Michael Xu , Kevin Ye , Ida Sadeghi , Rafael Jaramillo , James M. LeBeau

Among the interfacial transport modulations to the LaAlO3/SrTiO3 (LAO/STO) heterostructure, mechanical strain has been proven to be an effective approach by growing the LAO/STO films on different substrates with varying lattice mismatches…

Materials Science · Physics 2016-07-12 Fang Zhang , Yue-Wen Fang , Ngai Yui Chan , Wing Chong Lo , Dan Feng Li , Chun-Gang Duan , Feng Ding , Ji Yan Dai

LaAlO$_{3}$ and NdGaO$_{3}$ thin films of different thickness have been grown by pulsed laser deposition on TiO$_2$-terminated SrTiO$_{3}$ single crystals and investigated by soft X-ray photoemission spectroscopy. The surface sensitivity of…

We investigate pulsed laser deposition of LaGaO3/SrTiO3 at 10-1 mbar oxygen background pressure, demonstrating the critical effect of the target-to-substrate distance, dTS, on the interface sheet resistance, Rs. The interface turns from…

Selective optical excitation of a substrate lattice can drive phase changes across hetero-interfaces. This phenomenon is a non-equilibrium analogue of static strain control in heterostructures and may lead to new applications in optically…

Recently a metallic state was discovered at the interface between insulating oxides, most notably LaAlO3 and SrTiO3. Properties of this two-dimensional electron gas (2DEG) have attracted significant interest due to its potential…

The interface superconductivity in LaAlO$_{3}$-SrTiO$_{3}$ heterostructures reveals a non-monotonic behavior of the critical temperature as a function of the two-dimensional density of charge carriers. We develop a theoretical description…

Superconductivity · Physics 2014-07-22 S. N. Klimin , J. Tempere , J. T. Devreese , D. van der Marel

Variations in growth conditions associated with different deposition techniques can greatly affect the phase stability and defect structure of complex oxide heterostructures. We synthesized superlattices of the paramagnetic metal LaNiO3 and…

Strongly Correlated Electrons · Physics 2017-01-31 F. Wrobel , A. F. Mark , G. Christiani , W. Sigle , H. -U. Habermeier , P. A. van Aken , G. Logvenov , B. Keimer , E. Benckiser

Controlling the surface structure on the atomic scale is a major difficulty for most transition metal oxides; this is especially true for the ternary perovskites. The influence of surface stoichiometry on the atomic structure of the…

Materials Science · Physics 2018-04-13 Stefan Gerhold , Zhiming Wang , Michael Schmid , Ulrike Diebold

Hexagonal perovskites are an attractive group of materials due to their various polymorph phases and rich structure-property relationships. BaRuO3 (BRO) is a prototypical hexagonal perovskite, in which the electromagnetic properties are…

Materials Science · Physics 2021-07-16 Sangmoon Yoon , Jong Mok Ok , Sang A Lee , Jegon Lee , Andrew R. Lupini , Woo Seok Choi , Ho Nyung Lee

Atomically sharp oxide heterostructures exhibit a range of novel physical phenomena that do not occur in the parent bulk compounds. The most prominent example is the appearance of highly conducting and superconducting states at the…

We report on the non-trivial nanoscale kinetics of the deposition of novel complex oxide heterostructures composed of a unit-cell thick correlated metal LaNiO3 and dielectric LaAlO3. The multilayers demonstrate exceptionally good…

Strongly Correlated Electrons · Physics 2015-05-18 M. Kareev , S. Prosandeev , Jian Liu , B. Gray , P. Ryan , A. Kareev , Eun Ju Moon , J. Chakhalian

The properties of single-crystal SrTiO$_{3}$ substrates and homoepitaxial SrTiO$_{3}$ films grown by pulsed laser deposition have been compared, in order to understand the loss of interfacial conductivity when more than a critical thickness…

Metal halide perovskite-based semi-conducting hetero-structures have emerged as promising electronics for solar cells, light-emitting diodes, detectors, and photo-catalysts. Perovskites' efficiency, electronic properties and their long-term…

Materials Science · Physics 2024-05-21 Paramvir Ahlawat , Cecilia Clementi , Felix Musil , Maria-Andreea Filip

We have investigated the effects of low-energy ion beam irradiations using argon clusters on the chemical and electronic properties of LaAlO3/SrTiO3 (LAO/STO) heterointerfaces by combining X-ray photoelectron spectroscopy (XPS) and…

Strongly Correlated Electrons · Physics 2018-01-24 Karl Ridier , Damien Aureau , Bruno Bérini , Yves Dumont , Niels Keller , Jackie Vigneron , Arnaud Etcheberry , Arnaud Fouchet

The spinel/perovskite heterointerface $\gamma$-Al$_2$O$_3$/SrTiO$_3$ hosts a two-dimensional electron system (2DES) with electron mobilities exceeding those in its all-perovskite counterpart LaAlO$_3$/SrTiO$_3$ by more than an order of…

First-principles calculations demonstrate the evolution of the band alignment at La0.7A0.3MnO3|La1-xAx|TiO2|SrTiO3(001) heterointerfaces, where A = Ca, Sr, or Ba, as the interfacial A-site composition, La1-Ax, is varied from x = 0.5 to x =…

Materials Science · Physics 2010-10-13 J. D. Burton , E. Y. Tsymbal

Here we investigate LaAlO_3-SrTiO_3 heterostructure with\delta-doping of the interface by LaMnO_3 at less than one monolayer. This doping strongly inhibits the formation of mobile electron layer at the interface. This results in giant…

Strongly Correlated Electrons · Physics 2014-07-04 A. Rastogi , S. Tiwari , J. J. Pulikkotil , Z. Hossain , D. Kumar , R. C. Budhani