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We report the observation of multiple ionization of Argon through multi-XUV-photon absorption induced by an unprecedentedly powerful laser driven high-harmonic-generation source. Comparing the measured intensity dependence of the yield of…

When atoms and molecules are irradiated by an x-ray free-electron laser (XFEL), they are highly ionized via a sequence of one-photon ionization and relaxation processes. To describe the ionization dynamics during XFEL pulses, a rate…

Atomic Physics · Physics 2013-03-13 Sang-Kil Son , Robin Santra

Here, we report on the nonlinear ionization of argon atoms in the short wavelength regime using ultraintense x rays from the European XFEL. After sequential multiphoton ionization, high charge states are obtained. For photon energies that…

In this paper, we theoretically study x-ray multiphoton ionization dynamics of heavy atoms taking into account relativistic and resonance effects. When an atom is exposed to an intense x-ray pulse generated by an x-ray free-electron laser…

Atomic Physics · Physics 2017-04-26 Koudai Toyota , Sang-Kil Son , Robin Santra

We investigate molecular dynamics of multiple ionization in N2 through multiple core-level photoabsorption and subsequent Auger decay processes induced by intense, short X-ray free electron laser pulses. The timing dynamics of the…

X-ray free electron laser (XFEL) can provide X-ray light with about four order of magnitude higher flux than synchrotron radiation. Pulse light from XFEL interacts with the target and the resulting photons are collected by detectors. The…

Instrumentation and Detectors · Physics 2021-10-13 Shuo Zhang , Jing-Kai Xia , Xu-Dong Ju

We review the main aspects of multiple photoionization processes in atoms exposed to intense, short wavelength radiation. The main focus is the theoretical framework for the description of such processes as well as the conditions under…

Atomic Physics · Physics 2014-01-21 P. Lambropoulos , G. M. Nikolopoulos

Ultraintense pulses from X-ray free-electron lasers can drive, within femtoseconds, multiple processes in the inner shells of atoms and molecules in all phases of matter. The ensuing complex ionization pathways of outer-shell electrons from…

In order to effectively improve the output quality of X-ray free electron laser (XFEL), we theoretically propose an XFEL scheme seeded by atomic inner-shell laser. As well known, an atomic inner-shell laser based on neutral atoms and pumped…

Accelerator Physics · Physics 2018-08-01 Han Zhang , Kai Li , Jiawei Yan , Haixiao Deng , Baoyuan Sun

Since the advent of x-ray free-electron lasers (XFELs), considerable efforts have been devoted to achieve x-ray pulses with better temporal coherence. Here, we put forward a scheme to generate fully coherent x-ray lasers (XRLs) based on…

Atomic Physics · Physics 2018-01-09 Chunhai Lyu , Stefano M. Cavaletto , Christoph H. Keitel , Zoltán Harman

It was recently discovered that molecular ionization at high x-ray intensity is enhanced, in comparison with that of isolated atoms, through a phenomenon called CREXIM (charge-rearrangement-enhanced x-ray ionization of molecules). X-ray…

Chemical Physics · Physics 2019-07-10 Yajiang Hao , Ludger Inhester , Sang-Kil Son , Robin Santra

Serial femtosecond X-ray crystallography (SFX) captures the structure and dynamics of biological macromolecules at high spatial and temporal resolutions. The ultrashort pulse produced by an X-ray free electron laser (XFEL) 'outruns' much of…

Plasma Physics · Physics 2025-06-03 Spencer K. Passmore , Alaric L. Sanders , Andrew V. Martin , Harry M. Quiney

In a recent experiment at the VUV free-electron laser facility at DESY in Hamburg, the generation of multiply charged ions in a gas of atomic xenon was observed. This paper develops a theoretical description of multiphoton ionization of…

Atomic Physics · Physics 2009-11-10 Robin Santra , Chris H. Greene

Absolute Ar XK (3 keV) and Xe XL (4 keV) photon yields are measured as a function of laser peak intensity, for large (104 - 105 atoms) argon and xenon clusters submitted to intense laser pulses. A clear threshold behavior is observed. The…

Atomic and Molecular Clusters · Physics 2007-05-23 C. Prigent , L. Adoui , E. Lamour , J. -P. Rozet , D. Vernhet , O. Gobert , P. Meynadier , D. Normand , M. Perdrix

A nonlinear interaction between photons is observed in a process that involves charge sources. To observe this process in a vacuum, there are a growing number of theoretical and experimental studies. This process may contain exotic…

High Energy Physics - Experiment · Physics 2017-07-04 T. Inada , T. Yamazaki , T. Yamaji , Y. Seino , X. Fan , S. Kamioka , T. Namba , S. Asai

We present the first measurements of photoelectron spectra of atomic clusters embedded in superfluid helium (He) nanodroplets. Owing to the large absorption cross section of xenon (Xe) around 100 eV photon energy (4d inner-shell…

The importance of investigating magnetized plasmas/solids in extreme conditions has grown over the last decades, particularly in the field of high energy density physics (HEDP), such as laboratory astrophysics and inertial confinement…

X-ray free electron lasers (XFEL) create femtosecond X-ray pulses with high brightness and high longitudinal coherence allowing to extend X-ray spectroscopy and scattering techniques into the ultrafast time-domain. These X-rays are a…

Using the photon-ion merged-beams technique at a synchrotron light source, we have measured relative cross sections for single and up to five-fold photoionization of Fe$^{2+}$ ions in the energy range 690--920 eV. This range contains…

The balance of the linear photon momentum in multiphoton ionization is studied experimentally. In the experiment argon and neon atoms are singly ionized by circularly polarized laser pulses with a wavelength of 800 nm and 1400 nm in the…

Optics · Physics 2011-06-01 C Smeenk , L Arissian , B Zhou , A Mysyrowicz , D M Villeneuve , A Staudte , P B Corkum
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