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Considering certain interesting features in the previously reported 166Er Moessbauer effect and neutron diffraction data on the polycrystalline form of ErPd2Si2 crystallizing in ThCr2Si2-type tetragonal structure, we have carried out…

Strongly Correlated Electrons · Physics 2009-11-13 E. V. Sampathkumaran , Niharika Mohapatra , Kartik K Iyer , C. D. Cao , W. Loeser , G. Behr

A quantum spin liquid is a novel state of matter characterized by quantum entanglement and the absence of any broken symmetry. In condensed matter, the frustrated rare-earth pyrochlore magnets Ho$_2$Ti$_2$O$_7$ and Dy$_2$Ti$_2$O$_7$,…

Strongly Correlated Electrons · Physics 2017-04-05 E. Kermarrec , J. Gaudet , K. Fritsch , R. Khasanov , Z. Guguchia , C. Ritter , K. A. Ross , H. A. Dabkowska , B. D. Gaulin

Reentrance, the return of a system from an ordered phase to a previously encountered less-ordered one as a controlled parameter is continuously varied, is a recurring theme found in disparate physical systems, from condensed matter to black…

Strongly Correlated Electrons · Physics 2022-01-12 D. R. Yahne , D. Pereira , L. D. C. Jaubert , L. D. Sanjeewa , M. Powell , J. W. Kolis , Guangyong Xu , M. Enjalran , M. J. P. Gingras , K. A. Ross

The glassy behavior observed in the pyrochlore magnet Y2Mo2O7, where the magnetic Mo^{4+} ions interact predominantly via isotropic nearest neighbor antiferromagnetic exchange, possibly with additional weak disorder, is a distinct class of…

Statistical Mechanics · Physics 2010-09-08 Ka-Ming Tam , Adam J. Hitchcock , Michel J. P. Gingras

The XY pyrochlore antiferromagnet Er$_2$Ti$_2$O$_7$ exhibits a rare case of $Z_6$ discrete symmetry breaking in its $\psi_2$ magnetic ground state. Despite being well-studied theoretically, systems with high discrete symmetry breakings are…

Strongly Correlated Electrons · Physics 2017-02-15 J. Gaudet , A. M. Hallas , J. Thibault , N. P. Butch , H. A. Dabkowska , B. D. Gaulin

Frustrated pyrochlore lattices in transition-metal oxides provide an ideal platform for realizing exotic quantum states, including spin liquids with unconventional low-energy excitations arising from the macroscopic ground-state degeneracy…

Strongly Correlated Electrons · Physics 2026-05-26 Satish Kumar , U. Jena , A. Bandhopadhay , G. B. G. Stenning , D. T. Adroja , S. Petit , P. Khuntia

Neutron scattering, a.c. magnetic susceptibility and specific heat studies have been carried out on polycrystalline Dy2Zr2O7. Unlike the pyrochlore spin ice Dy2Ti2O7, Dy2Zr2O7 crystallizes into the fluorite structure and the magnetic Dy3+…

Disordered Systems and Neural Networks · Physics 2019-07-01 J. G. A. Ramon , C. W. Wang , L. Ishida , P. L. Bernardo , M. M. Leite , F. M. Vichi , J. S. Gardner , R. S. Freitas

A "supercooled" liquid develops when a fluid does not crystallize upon cooling below its ordering temperature. Instead, the microscopic relaxation times diverge so rapidly that, upon further cooling, equilibration eventually becomes…

We present a muon spin relaxation study on the Ising pyrochlore Nd$_2$Zr$_2$O$_7$ which develops an "all-in-all-out" magnetic order below 0.4~K. At 20~mK far below the ordering transition temperature, the zero-field muon spin relaxation…

Materials Science · Physics 2016-09-07 J. Xu , C. Balz , C. Baines , H. Luetkens , B. Lake

Sm$_2$Ti$_2$O$_7$, a member of rare-earth titanate pyrochlores, exhibits dipolar-octupolar antiferromagnetism below $T_N$ = 0.35 K. We observed two ferroelectric transitions at 182 ($T_{FE1}$) and 52 K ($T_{FE2}$), significantly higher than…

Materials Science · Physics 2024-07-30 S. Mukherjee , O. Ivashko , S. Majumdar , A. Kumar , S. Giri

We report the physical properties of Tb2Hf2O7 based on ac magnetic susceptibility \chi_ac(T), dc magnetic susceptibility \chi(T), isothermal magnetization M(H), and heat capacity C_p(T) measurements combined with muon spin relaxation…

Strongly Correlated Electrons · Physics 2018-03-06 V. K. Anand , L. Opherden , J. Xu , D. T. Adroja , A. D. Hillier , P. K. Biswas , T. Herrmannsdörfer , M. Uhlarz , J. Hornung , J. Wosnitza , E. Canevet , B. Lake

In this paper we present a study of magnetic order of quantum Heisenberg spins on pyrochlore type lattices: a lattice of corner sharing tetrahedra. We use the Cluster Variation Approximation with the tetrahedron as basic cluster. We find…

Strongly Correlated Electrons · Physics 2007-05-23 Wiebe Geertsma

We have recently reported that the Haldane spin-chain system, Er2BaNiO5, undergoing antiferromagnetic order below 32 K, is characterized by the onset of ferroelectricity near 60K due to magnetoelectric coupling induced by short-range…

Strongly Correlated Electrons · Physics 2015-06-22 Tathamay Basu , Kiran Singh , N. Mohapatra , E. V. Sampathkumaran

The spin ordering in RuO2 remains a highly debated topic, owing to its elusive nature, with reports ranging from a nonmagnetic ground state to signatures of unconventional magnetic order. Here we provide the first unambiguous, and direct…

Despite a Curie-Weiss temperature $\theta_{\rm CW} \sim -14$ K, the Tb2Ti2O7 pyrochlore magnetic material lacks long range magnetic order down to at least $T^*\approx 50$ mK. It has recently been proposed that the low temperature collective…

Statistical Mechanics · Physics 2009-05-07 Hamid R. Molavian , Michel J. P. Gingras

We have probed the low temperature magnetic behavior of the ordered spin ice material Tb2Sn2O7 through ac magnetic susceptibility measurements of both the pure material and samples with small percentages of Ti substituted on the Sn…

Strongly Correlated Electrons · Physics 2012-11-27 M. L. Dahlberg , M. J. Matthews , P. Jiramongkolchai , R. J. Cava , P. Schiffer

Conclusive evidence of order by disorder is scarce in real materials. Perhaps one of the strongest cases presented has been for the pyrochlore XY antiferromagnet Er2Ti2O7, with the ground state selection proceeding by order by disorder…

Strongly Correlated Electrons · Physics 2016-05-11 Jeffrey G. Rau , Sylvain Petit , Michel J. P. Gingras

The nature of the low temperature ground state of the pyrochlore compound Tb2Ti2O7 remains a puzzling issue. Dynamic fluctuations and short-range correlations persist down to 50 mK, as evidenced by microscopic probes. In parallel,…

Strongly Correlated Electrons · Physics 2012-08-02 E. Lhotel , C. Paulsen , P. Dalmas de Réotier , A. Yaouanc , C. Marin , S. Vanishri

Neutron scattering experiments on a polycrystalline sample of the frustrated pyrochlore magnet Tb2Ti2O7, which does not show any magnetic order down to 50 mK, have revealed that it shows condensation behavior below 0.4 K from a thermally…

Disordered Systems and Neural Networks · Physics 2011-12-13 Hiroshi Takatsu , Hiroaki Kadowaki , Taku J. Sato , Jeffrey W. Lynn , Yoshikazu Tabata , Teruo Yamazaki , Kazuyuki Matsuhira

The charge ordered structure of ions and vacancies characterizing rare-earth pyrochlore oxides serves as a model for the study of geometrically frustrated magnetism. The organization of magnetic ions into networks of corner-sharing…