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Structural disorder in the magnetically frustrated pyrochlore system leads to intriguing magnetic states. We present the thermodynamic behavior and short range magnetic correlations in Tb$_{2}$Zr$_{2}$O$_{7}$ and…

Strongly Correlated Electrons · Physics 2026-04-16 Sujata Singh , Leon Carstens , M. Duc Le , R. Klingeler , C. S. Yadav

Thermal fluctuations lift the high ground state degeneracy of the classical nearest neighbour pyrochlore antiferromagnet, with easy plane anisotropy, giving a first order phase transition to a long range ordered state. We show, from spin…

Condensed Matter · Physics 2009-11-10 J D M Champion , P C W Holdsworth

The magnetic pyrochlore oxide materials of general chemical formula R2Ti2O7 and R2Sn2O7 (R = rare earth) display a host of interesting physical behaviours depending on the flavour of rare earth ion. These properties depend on the value of…

Statistical Mechanics · Physics 2015-06-24 Adrian G. Del Maestro , Michel J. P. Gingras

In divalent Eu systems, the 4f local moment has a pure spin state J=S=7/2. Although the absence of orbital moment precludes crystal electric field effects, we report a sizeable magnetic anisotropy in single crystals of EuRh2Si2. We observed…

Materials Science · Physics 2019-01-23 Silvia Seiro , Christoph Geibel

The intrinsic noncollinear spin patterns in rare-earth pyrochlore are physically interesting, hosting many emergent properties, e.g. spin ice and monopole-type excitation. Recently, the magnetic monopole excitation of spin ice systems was…

Materials Science · Physics 2015-12-18 Lin Lin , Y. L. Xie , J. -J. Wen , Shuai Dong , Z. B. Yan , J. -M. Liu

We report the experimental observation of spin reorientation in the double perovskite Ho$_2$FeCoO$_6$. The magnetic phase transitions in this compound are characterized and studied through magnetization and specific heat, and the magnetic…

Frustrated magnetic systems exhibit highly degenerate ground states and strong fluctuations, often leading to new physics. An intriguing example of current interest is the antiferromagnet on a diamond lattice, realized physically in A-site…

Materials Science · Physics 2011-09-21 G. J. MacDougall , D. Gout , J. L. Zarestky , G. Ehlers , A. Podlesnyak , M. A. McGuire , D. Mandrus , S. E. Nagler

The ordered hexagonal perovskite Ba2CuTeO6 hosts weakly coupled S=1/2 spin ladders produced by an orbital ordering of Cu2+. The magnetic susceptibility chi(T) of Ba2CuTeO6 is well described by that expected for isolated spin ladders with…

Collective behaviour of electrons, frustration induced quantum fluctuations and entanglement in quantum materials underlie some of the emergent quantum phenomena with exotic quasi-particle excitations that are highly relevant for…

The origin of the spin liquid state in Tb$_2$Ti$_2$O$_7$ has challenged experimentalists and theorists alike for nearly 20 years. To improve our understanding of the exotic magnetism in Tb$_2$Ti$_2$O$_7$, we have synthesized a chemical…

We present magnetization and Hall effect measurements on the pyrochlore iridate Nd2Ir2O7. Previous muon spin rotation measurements have shown that the system undergoes an unusual transition at T$_M$ = 110 K into a magnetic phase lacking…

Strongly Correlated Electrons · Physics 2015-06-12 S. M. Disseler , S. R. Giblin , Chetan Dhital , K. C. Lukas , Stephen D. Wilson , M. J. Graf

The magnetic properties of NiTa$_2$O$_6$ were investigated by magnetic susceptibility, specific heat, electron paramagnetic resonance, neutron powder diffraction and pulse field magnetization measurements. Accompanying \textit{ab initio}…

Strongly Correlated Electrons · Physics 2015-06-18 J. M. Law , H. -J. Koo , M. -H. Whangbo , E. Bruecher , V. Pomjakushin , R. K. Kremer

The pyrochlore magnet Tb$_{2}$Ti$_{2}$O$_{7}$ shows a lack of magnetic order to low temperatures and is considered to be a quantum spin liquid candidate. We perform time-domain THz spectroscopy on high quality Tb$_{2}$Ti$_{2}$O$_{7}$…

Strongly Correlated Electrons · Physics 2021-04-21 Xinshu Zhang , Yi Luo , T. Halloran , J. Gaudet , Huiyuan Man , S. M. Koohpayeh , N. P. Armitage

Dy$_{2}$Zr$_{2}$O$_{7}$ a disordered pyrochlore system, exhibits the spin ice freezing under the application of magnetic field. Our studies suggest the stabilization of pyrochlore phase in Dy$_{2-x}$La$_{x}$Zr$_{2}$O$_{7}$ with the…

Strongly Correlated Electrons · Physics 2021-10-12 Sheetal , C. S. Yadav

Comprehensive muon spin rotation/relaxation (muSR) and neutron powder diffraction (NPD) studies supported via bulk measurements have been performed on the ordered double perovskite Sr2YbRuO6 to investigate the nature of the magnetic ground…

We address the concomitant metal-insulator transition (MIT) and antiferromagnetic ordering in the novel pyrochlore iridate Eu2Ir2O7 by combining x-ray absorption spectroscopy, x-ray and neutron diffractions and density functional theory…

Effect of structural disorder is investigated for an $XY$ pyrochlore antiferromagnet with continuous degeneracy of classical ground states. Two types of disorder, vacancies and weakly fluctuating exchange bonds, lift degeneracy selecting…

Strongly Correlated Electrons · Physics 2014-09-26 V. S. Maryasin , M. E. Zhitomirsky

We report a study of the geometrically frustrated magnetic material Tb2Sn2O7 by the positive muon spin relaxation technique. No signature of a static magnetically ordered state is detected while neutron magnetic reflections are observed in…

Strongly Correlated Electrons · Physics 2009-11-11 P. Dalmas de Reotier , A. Yaouanc , L. Keller , A. Cervellino , B. Roessli , C. Baines , A. Forget , C. Vaju , P. C. M. Gubbens , A. Amato , P. J. C. King

We present high-resolution single crystal time-of-flight neutron scattering measurements on the candidate quantum spin liquid pyrochlore Tb2Ti2O7 at low temperature and in a magnetic field. At ~70 mK and in zero field, Tb2Ti2O7 reveals…

Strongly Correlated Electrons · Physics 2013-04-16 K. Fritsch , K. A. Ross , Y. Qiu , J. R. D. Copley , T. Guidi , R. I. Bewley , H. A. Dabkowska , B. D. Gaulin

We report neutron scattering and muon spin relaxation measurements (muSR) on the pyrochlore antiferromagnet Yb2Ge2O7. Inelastic neutron scattering was used to probe the transitions between crystal electric field levels, allowing us to…

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