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Related papers: Raman-induced Kerr-effect dual-comb spectroscopy

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Improvements to dual-comb interferometers will benefit precision spectroscopy and sensing, distance metrology, tomography, telecommunications etc. A specific requirement of such interferometers is to enforce mutual coherence between the two…

Optics · Physics 2018-08-10 Zaijun Chen , Ming Yan , Theodor W. Hänsch , Nathalie Picqué

We investigated ultrafast nonlinear optical effects in nitrogen-vacancy (NV)-containing diamond which is in contact with a gold-coated blazed diffraction grating using a pump-probe reflectivity technique. The reflectivity change caused by…

Optics · Physics 2025-08-27 Yuta Kimura , Toshu An , Muneaki Hase

We demonstrate a simple system for dual-comb spectroscopy based on two inherently coherent optical frequency combs generated via seeded parametric down-conversion. The inbuilt coherence is established by making the two combs share a common…

Optics · Physics 2024-08-13 Mikhail Roiz , Santeri Larnimaa , Touko Uotila , Mikko Narhi , Markku Vainio

Dual-comb spectroscopy in the ultraviolet (UV) and visible would enable broad bandwidth electronic spectroscopy with unprecedented frequency resolution. However, there are significant challenges in generation, detection and processing of…

Stimulated Raman spectroscopy has become a powerful tool to study the spatiodynamics of molecular bonds with high sensitivity, resolution and speed. However, sensitivity and speed of state-of-the-art stimulated Raman spectroscopy are…

The broad and equidistant spectrum of frequency combs has had a profound impact on spectroscopic studies. Particularly, experiments involving the coupling of frequency combs to cavities have already enabled unprecedented broadband and…

Optics · Physics 2024-12-10 Andrei Diakonov , Konstantin Khrizman , Eliran Zano , Liron Stern

Optical frequency combs are crucial for both fundamental science and applications demanding wide frequency spanning and ultra-precision resolutions. Recent advancements of nonlinear Kerr effect based optical frequency combs in microcavities…

Optics · Physics 2019-03-13 Yuanlin Zheng , Tian Qin , Jianfan Yang , Xianfeng Chen , Li Ge , Wenjie Wan

Two-photon excitation spectroscopy with broad spectral span is demonstrated at Doppler-limited resolution. We describe first Fourier transform two-photon spectroscopy of an atomic sample with two mode-locked laser oscillators in a dual-comb…

Frequency-modulated (FM) combs are produced by mode-locked lasers in which the electric field has a linearly chirped frequency and nearly constant amplitude. This regime of operation occurs naturally in certain laser systems and constitutes…

Spectral compression of femtosecond pulses by second harmonic generation in the presence of substantial group velocity dispersion provides a convenient source of narrowband Raman pump pulses for femtosecond stimulated Raman spectroscopy…

Optics · Physics 2015-06-12 E. Pontecorvo , C. Ferrante , C. G. Elles , T. Scopigno

Vibrational spectroscopy, comprised of infrared absorption and Raman scattering spectroscopy, is widely used for label-free optical sensing and imaging in various scientific and industrial fields. The group theory states that the two…

Chemical Physics · Physics 2019-10-09 Kazuki Hashimoto , Venkata Ramaiah Badarla , Akira Kawai , Takuro Ideguchi

We provide a theoretical, numerical, and experimental investigation of the Kerr nonlinearity impact on the performance of a frequency-multiplexed Extreme Learning Machine (ELM). In such ELM, the neuron signals are encoded in the lines of a…

Optics · Physics 2023-12-20 Marina Zajnulina , Alessandro Lupo , Serge Massar

We demonstrate the acquisition of stimulated Raman scattering spectra with the use of a single femtosecond pulse. High resolution vibrational spectra are obtained by shifting the phase of a narrow band of frequencies in the broadband input…

Optics · Physics 2015-05-20 Hadas Frostig , Ori Katz , Adi Natan , Yaron Silberberg

We propose a method for increasing the Raman scattering from an ensemble of molecules by up to four orders of magnitude. Our method requires an additional coherent source of IR radiation with the half-frequency of the Stokes shift. This…

Quantum Physics · Physics 2019-04-24 V. Yu. Shishkov , E. S. Andrianov , A. A. Pukhov , A. P. Vinogradov , A. A. Lisyansky

Dual-comb spectroscopy has emerged as an indispensable analytical technique in applications that require high resolution and broadband coverage within short acquisition times. Its experimental realization, however, remains hampered by…

Instrumentation and Detectors · Physics 2019-12-02 Łukasz A. Sterczewski , Aleksandra Przewłoka , Wawrzyniec Kaszub , Jarosław Sotor

On-chip frequency comb generations enable compact broadband sources for spectroscopic sensing and precision spectroscopy. Recent microcomb studies focus on infrared spectral regime and have difficulty in accessing visible regime. Here, we…

Optics · Physics 2014-10-21 Hojoong Jung , Rebecca Stoll , Xiang Guo , Debra Fischer , Hong X. Tang

We present gapless, high-resolution absorption and dispersion spectra obtained with quantum cascade laser frequency combs covering 55 cm$^{-1}$. Using phase-sensitive dual comb design, the comb lines are gradually swept over 10 GHz,…

We overview recent advances in the research on spatiotemporal beam shaping in nonlinear multimode optical fibers. An intense light beam coupled to a graded index (GRIN) highly multimode fiber undergoes a series of complex nonlinear…

We propose and characterize experimentally a new source of optical frequency combs for performing multi-heterodyne spectrometry. This comb modality is based on a frequency shifting loop seeded with a CW monochromatic laser. The comb lines…

Optics · Physics 2018-07-04 V. Duran , C. Schnebelin , H. Guillet De Chatellus

With the advent of laser frequency combs, coherent light sources that offer equally-spaced sharp lines over a broad spectral bandwidth have become available. One decade after revolutionizing optical frequency metrology, frequency combs hold…

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