Related papers: Raman-induced Kerr-effect dual-comb spectroscopy
Excited-state vibrational dynamics in molecules can be studied by an electronically off-resonant Raman process induced by a probe pulse with variable delay with respect to an actinic pulse. We establish the connection between several…
We report on resonance Raman spectroscopy measurements with excitation photon energy down to 1.16 eV on graphene, to study how low-energy carriers interact with lattice vibrations. Thanks to the excitation energy close to the Dirac point at…
Different from the Kerr effect,stimulated Raman scattering (SRS) is a delayed response to molecular vibrations in materials. In microcavities, when driven in an anomalous group velocity dispersion (GVD) regime, SRS typically leads to…
Plasmon-enhanced Raman scattering (PERS) becomes nonlinear when phonon pumping and phonon-stimulated scattering come into play. It is fundamental to the understanding of PERS and its photobleaching behavior. By quantization of the molecular…
The Raman scattering spectra from magnetic excitations in an antiferromagnetic spin-1/2 two leg ladder is investigated for weak and strong interladder coupling. In the first case, a cusp in the Raman intensityis obtained at a frequency…
We present a new type of dual optical frequency comb source capable of scaling applications to high measurement speeds while combining high average power, ultra-low noise operation, and a compact setup. Our approach is based on a…
We simulate a third-order nonlinear signal in a pump-probe spectroscopy from the interference between first- and second-order wavepackets (WPs), as well as from a state-to-state transition for Stokes and coherent anti-Stokes pathways in the…
We experimentally demonstrate four-wave-mixing spectroscopy using frequency combs. The experiment uses a geometry where excitation pulses and four-wave-mixing signals generated by a sample co-propagate. We separate them in the radio…
This paper presents a novel approach to dual-frequency comb generation utilizing a single fiber Fabry-Perot resonator, advancing the implementation of these sources in fiber-based systems. Dual-comb applications such as spectroscopy,…
We radically simplify coherently averaged dual-comb spectroscopy by introducing a real-time self-correction system: a radio frequency system-on-chip computes each incoming dual-comb interferogram's phase, frequency, and arrival time;…
Optical frequency combs [1-8] have resulted in significant advances in optical frequency metrology and found wide application to precise physical measurements [1-4, 9] and molecular fingerprinting [8]. A direct analogue of frequency combs…
Rapid and large scanning of a dissipative Kerr-microresonator soliton comb with the characterization of all comb modes along with the separation of the comb modes is imperative for the emerging applications of the frequency-scanned soliton…
We report on an Er-doped fiber (EDF)-laser-based dual-comb system that allows us to perform triggerless asynchronous optical sampling (ASOPS) pump-probe measurements of ultrafast demagnetization and spin precession in magnetic materials.…
In a uniform microresonator, the generation of a broadband Kerr frequency comb is triggered by Turing patterns. Here, we study a distinctly different route to initiate the Kerr frequency comb by Faraday ripples. Momentum conservation is…
We present a quantum-mechanical model that describes fiber-based frequency conversion by four-wave-mixing Bragg scattering in the presence of Raman interactions. In the case of continuous-wave pumps we find closed-form expressions for the…
One of the most widely used chiroptical spectroscopic methods for studying chiral molecules is Raman optical activity; however, the chiral Raman optical activity signal is extremely weak. Here, we theoretically examine enhanced chiral…
We present a flexible and efficient ultrafast time-resolved spontaneous Raman spectroscopy setup to study collective excitation and quasi-particle dynamics in quantum matter. The setup has a broad energy tuning range extending from the…
To date there are extensive studies of optical nonlinearities in whispering gallery resonators (WGRs) in the near and mid-infrared wavelengths. Pushing this research into the visible region is equally valuable. Here, we demonstrate a Kerr…
A two-phonon system with lowest-order coupling of form $Q_RQ_{IR}^2$ is studied by perturbation method, and analytic results for both phonon displacements and frequencies are obtained. The frequency renormalization of infrared (IR) active…
Using an enhanced optically heterodyned optical Kerr effect method and a theoretical description of the interactions between an optical beam, a single layer of graphene, and its substrate, we provide experimental answers to questions raised…