Related papers: Raman-induced Kerr-effect dual-comb spectroscopy
The THz Kerr effect measures the birefringence induced in an otherwise isotropic material by a strong THz pulse driving the Raman-active excitations of the systems. Here we provide experimental evidence of a sizable Kerr response in…
The broadband, coherent nature of narrow-linewidth fiber frequency combs is exploited to measure the full complex spectrum of a molecular gas through multi-heterodyne spectroscopy. We measure the absorption and phase shift experienced by…
Dual-comb spectroscopy can provide broad spectral bandwidth and high spectral resolution in a short acquisition time, enabling time-resolved measurements. Specifically, spectroscopy in the mid-infrared wavelength range is of particular…
We analyse Raman-induced self-frequency shift in two-component solitons supported by both quadratic and cubic nonlinearities. Treating Raman terms as a perturbation, we derive expressions for soliton velocity and frequency shifts of the…
Unveiling and controlling the coherent evolution of low energy states is a key to attain light driven new functionalities of materials. Here we investigate the coherent evolution of non-equilibrium photon-phonon Raman interactions in the…
Multidimensional coherent optical spectroscopy is one of the most powerful tools for investigating complex quantum mechanical systems. While it was conceived decades ago in magnetic resonance spectroscopy using micro- and radio-waves, it…
Two--magnon Raman scattering is a useful tool to verify recent suggestions concerning the value of the interplanar exchange constant in antiferromagnetic two--layer systems, such as $YBa_2Cu_3O_{6+x}$. We present a theory for Raman…
We demonstrate a new technique for the experimental measurement of the spectral coherence of microresonator optical frequency combs. Specifically, we use a spectral interference method, typically used in the context of supercontinuum…
Micro-ring resonators (MRRs) "trap" incoming light, and therefore, have been shown to achieve extremely high local intensities of light. Thus, they can be used to facilitate highly non-linear optical signals. By embedding materials that…
Frequency combs based on terahertz quantum cascade lasers feature broadband coverage and high output powers in a compact package, making them an attractive option for broadband spectroscopy. Here, we demonstrate the first multi-heterodyne…
A fieldable dual-comb spectrometer is described based on a "bootstrapped" frequency referencing scheme in which short-term optical phase coherence between combs is attained by referencing each to a free-running diode laser, whilst high…
Two frequency combs can be used to measure the full complex response of a sample in a configuration which can be alternatively viewed as the equivalent of a dispersive Fourier transform spectrometer, infrared time domain spectrometer, or a…
Hyperspectral imaging is a technique that allows for the creation of multi-color images. At terahertz wavelengths, it has emerged as a prominent tool for a number of applications, ranging from non-ionizing cancer diagnosis and…
We describe a detector that measures the mutual coherence of two optical fields directly using quantum interference, free from photon noise of the individual irradiances. Our approach utilizes Raman transition in an atomic system where the…
We propose a novel femtosecond stimulated Raman spectroscopy (FSRS) technique that combines entangled photons with interference detection to select matter pathways and enhance the resolution. Following photo excitation by an actinic pump,…
Mid-infrared (mid-IR) spectroscopy offers unparalleled sensitivity for the detection of trace gases, solids and liquids, which is based on the existence of strong telltale vibrational bands in this part of the spectrum. It was shown more…
We demonstrate low-frequency interferometric impulsive stimulated Raman scattering (ISRS) imaging with high robustness to distortions by optical scattering. ISRS is a pump-probe coherent Raman spectroscopy that can capture Raman vibrational…
Nonstationary molecular states which contain electronic coherences can be impulsively created and manipulated by using recently-developed ultrashort optical and X-ray pulses via photoexcitation, photoionization and Auger processes. We…
Detector nonlinearity is an important factor limiting the maximal power and hence the signal-to-noise ratio (SNR) in dual-comb interferometry. To increase the SNR without overwhelming averaging time, specific experimental conditions must be…
Frequency comb spectroscopy has significantly advanced molecular spectroscopy across scientific research and diverse applications. Among its key performance metrics especially for time-resolved studies, sensitivity and measurement speed are…