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We report a high-field electron spin resonance study in the sub-THz frequency domain of a single crystal of Sr$_2$IrO$_4$ that has been recently proposed as a prototypical spin-orbital Mott insulator. In the antiferromagnetically (AFM)…

Strongly Correlated Electrons · Physics 2015-06-18 S. Bahr , A. Alfonsov , G. Jackeli , G. Khaliullin , A. Matsumoto , T. Takayama , H. Takagi , B. Büchner , V. Kataev

Dielectric and magnetic phenomena in spin and charge frustrated system RFe2O4 (R is a rare-earth metal ion) are studied. An electronic model for charge, spin and orbital degrees in a pair of triangular-lattice planes is derived. We analyze…

Strongly Correlated Electrons · Physics 2009-11-13 Makoto Naka , Aya Nagano , Sumio Ishihara

We show that the magnetic response of atomically thin materials with Dirac spectrum and spin-orbit interactions can exhibit strong dependence on electron-electron interactions. While graphene itself has a very small spin-orbit coupling,…

Mesoscale and Nanoscale Physics · Physics 2020-07-24 Sanghita Sengupta , Madalina I. Furis , Oleg P. Sushkov , Valeri N. Kotov

Using {\it ab initio} methods, we investigate the modification of the magnetic properties of the $m=2$ member of the strontium iridates Ruddlesden-Popper series Sr$_{m+1}$Ir$_{m}$O$_{3m+1}$, bilayer Sr$_3$Ir$_2$O$_7$, induced by epitaxial…

Materials Science · Physics 2017-01-20 Bongjae Kim , Peitao Liu , Cesare Franchini

Spin-reorientation phase transitions that involve the rotation of a crystal$'$s magnetization have been well characterized in distorted-perovskite oxides such as the orthoferrites. In these systems spin reorientation occurs due to competing…

Strongly Correlated Electrons · Physics 2020-06-29 A. M. Vibhakar , D. D. Khalyavin , P. Manuel , J. Liu , A. A. Belik , R. D. Johnson

We present an anti-ferromagnetically ordered ground state of Na$_{2}$IrO$_{3}$ based on density-functional-theory calculations including both spin-orbit coupling and on-site Coulomb interaction $U$. We show that the splitting of $e_{g}'$…

Strongly Correlated Electrons · Physics 2009-07-07 Hosub Jin , Heungsik Kim , Hogyun Jeong , Choong H. Kim , Jaejun Yu

Motivated by the recent experimental developments in van der Waals heterostructures, we investigate the emergent magnetism in Mott insulator - semimetal moir\'e superlattices by deriving effective spin models and exploring their phase…

Strongly Correlated Electrons · Physics 2024-11-05 M. A. Keskiner , Pouyan Ghaemi , M. Ö. Oktel , Onur Erten

The electronic and magnetic structure, including the Heisenberg model exchange interaction parameters, was explored for the recently proposed novel cuprate Cu$_2$F$_5$. Using the DFT+U calculation, it is shown that the compound is formed by…

Strongly Correlated Electrons · Physics 2021-08-11 Dmitry M. Korotin , Dmitry Y. Novoselov , Vladimir I. Anisimov , Artem R. Oganov

The competition between fractionalized spin-liquid states and magnetically ordered phases is an important paradigm in frustrated magnetism. Spin-orbit coupled Mott insulators with Ising-like magnetic anisotropies, such as Kitaev materials,…

Strongly Correlated Electrons · Physics 2022-12-08 G. Shankar , Chien-Hung Lin , Joseph Maciejko

We present a detailed first principles study on the magnetic structure of an Fe monolayer on different surfaces of 5d transition metals. We use the spin-cluster expansion technique to obtain parameters of a spin model, and predict the…

Materials Science · Physics 2014-05-06 E. Simon , K. Palotás , B. Ujfalussy , A. Deák , G. M. Stocks , L. Szunyogh

In two-dimensional van der Waals magnetic materials, the interplay between magnetism and electron correlation can give rise to new ground states and lead to novel transport and optical properties. A fundamental question in these materials…

We find using LSDA+U band structure calculations that the novel one-dimensional cobaltate Ca$_3$Co$_2$O$_6$ is not a ferromagnetic half-metal but a Mott insulator. Both the octahedral and the trigonal Co ions are formally trivalent, with…

Strongly Correlated Electrons · Physics 2007-05-23 Hua Wu , M. W. Haverkort , Z. Hu , D. I. Khomskii , L. H. Tjeng

The electron's kinetic energy plays a pivotal role in magnetism. While virtual electron hopping promotes antiferromagnetism in an insulator, the real process usually favors ferromagnetism. But in kinetically frustrated systems, such as hole…

Strongly Correlated Electrons · Physics 2023-07-25 Zui Tao , Wenjin Zhao , Bowen Shen , Patrick Knüppel , Kenji Watanabe , Takashi Taniguchi , Jie Shan , Kin Fai Mak

We report an unusual, non-monotonous dependence of the exchange bias on the thickness of the ferromagnetic layer in a ferromagnet/antiferromagnet bilayer system. We show that in epitaxial CoO/Fe(110) bilayers, the evolution of the Fe…

Mesoscale and Nanoscale Physics · Physics 2017-09-29 M. Ślęzak , T. Ślęzak , P. Dróżdż , B. Matlak , K. Matlak , J. Korecki

We explore the spin superfluid transport in exchange interaction dominated three-sublattice antiferromagnets. The system in the long-wavelength regime is described by an $SO(3)$ invariant field theory. Additional corrections from…

Mesoscale and Nanoscale Physics · Physics 2021-03-03 Bo Li , Alexey A. Kovalev

As a hallmark of electronic correlation, spin-charge interplay underlies many emergent phenomena in doped Mott insulators, such as high-temperature superconductivity, whereas the half-filled parent state is usually electronically frozen…

We have carried out Raman spectroscopy experiments to investigate two-magnon excitations in epitaxial thin films of the quasi-two-dimensional antiferromagnetic Mott insulator Sr$_2$IrO$_4$ under in-plane misfit strain. With in-plane biaxial…

Strongly Correlated Electrons · Physics 2019-10-08 A. Seo , P. P. Stavropoulos , H. -H. Kim , K. Fürsich , M. Souri , J. G. Connell , H. Gretarsson , M. Minola , H. Y. Kee , B. Keimer

We employ density functional theory plus dynamical mean field theory and identify the physical origin of why two layers of SrVO$_3$ on a SrTiO$_3$ substrate are insulating: the thin film geometry lifts the orbital degeneracy which in turn…

The novel electronic state of the canted antiferromagnetic (AFM) insulator, strontium iridate (Sr2IrO4) has been well described by the spin-orbit-entangled isospin Jeff = 1/2, but the role of isospin in transport phenomena remains poorly…

Strongly Correlated Electrons · Physics 2019-05-03 Nara Lee , Eunjung Ko , Hwan Young Choi , Yun Jeong Hong , Muhammad Nauman , Woun Kang , Hyoung Joon Choi , Young Jai Choi , Younjung Jo

Moir\'e heterostructures of transition metal dichalcogenides exhibit Mott-insulating behaviour both at half-filling as well as at fractional fillings, where electronic degrees of freedom form self-organized Wigner crystal states. An open…

Strongly Correlated Electrons · Physics 2024-01-31 Urban F. P. Seifert , Leon Balents