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This article contains a theoretical overview of the physical properties of antiferromagnetic Mott insulators in spatial dimensions greater than one. Many such materials have been experimentally studied in the past decade and a half, and we…

Strongly Correlated Electrons · Physics 2009-11-10 Subir Sachdev

The two-layer square lattice quantum antiferromagnet with spins 1/2 shows a magnetic order-disorder transition at a critical ratio of the interplane to intraplane couplings. We investigate the dynamics of a single hole in a bilayer…

Strongly Correlated Electrons · Physics 2009-10-31 Matthias Vojta , Klaus W. Becker

We studied the effect of inserting 0.5 nm-thick spacer layers (Ti, V, Cr, Mo, W) at the Pt/Co interface on the spin-orbit torques, Hall effect, magnetoresistance, saturation magnetization, and magnetic anisotropy. We find that the…

Mesoscale and Nanoscale Physics · Physics 2020-02-07 Can Onur Avci , Geoffrey S. D. Beach , Pietro Gambardella

Layered perovskite iridates realize a rare class of Mott insulators that are predicted to be strongly spin-orbit coupled analogues of the parent state of cuprate high-temperature superconductors. Recent discoveries of pseudogap, magnetic…

Strongly Correlated Electrons · Physics 2017-04-25 H. Chu , L. Zhao , A. de la Torre , T. Hogan , S. D. Wilson , D. Hsieh

The concept of swapping the two most important spin interactions -- exchange and spin-orbit coupling -- is proposed based on two-dimensional multilayer van der Waals heterostructures. Specifically, we show by performing realistic ab initio…

Mesoscale and Nanoscale Physics · Physics 2020-11-05 Klaus Zollner , Martin Gmitra , Jaroslav Fabian

We address the concomitant metal-insulator transition (MIT) and antiferromagnetic ordering in the novel pyrochlore iridate Eu2Ir2O7 by combining x-ray absorption spectroscopy, x-ray and neutron diffractions and density functional theory…

Spin-orbit-torque (SOT) induced magnetization switching in Co/Pt/Co trilayer, with two Co layers exhibiting magnetization easy axes orthogonal to each other is investigated. Pt layer is used as a source of spin-polarized current as it is…

We investigate magnetic excitations in iridium insulators with pentavalent Ir$^{5+}$ ($5d^4$) ions with strong spin-orbit coupling. We obtain a microscopic model based on the local Ir$^{5+}$ multiplets involving $J=0$ (singlet), $J=1$…

Strongly Correlated Electrons · Physics 2019-01-28 Beom Hyun Kim , Dmitry V. Efremov , Jeroen van den Brink

We investigate the properties of CuVOF$_4$(H$_2$O)$_6$$\cdot$H$_2$O, in which two different spin species, Cu(II) and V(IV), form antiferromagnetic spin-1/2 dimers with weak interdimer coupling provided via hydrogen bonding. Using…

Magnetic control of correlated spin systems is central to the development of next-generation spin-based technologies. Rare-earth orthoferrites provide an interesting platform in which exchange coupling between rare-earth 4f and…

Transition metal oxides, in particular, 3d or 4d perovskites have provided diverse emergent physics that originates from the coupling of various degrees of freedom such as spin, lattice, charge, orbital, and also disorder. 5d perovskites…

Strongly Correlated Electrons · Physics 2016-04-19 Abhijit Biswas , Ki-Seok Kim , Yoon Hee Jeong

We investigate the interplay of spin-orbit coupling, electronic correlations, and lattice distortions in the $5d^1$ double perovskite Ba$_2$MgReO$_6$. Combining density-functional theory (DFT) and dynamical mean-field theory (DMFT), we…

Strongly Correlated Electrons · Physics 2023-12-18 Maximilian E. Merkel , Aria Mansouri Tehrani , Claude Ederer

$5d$ iridium oxides are of huge interest due to the potential for new quantum states driven by strong spin-orbit coupling. The strontium iridate Sr$_2$IrO$_4$ is particularly in the spotlight because of the so-called $j_\text{eff}=1/2$…

Engineering magnetic anisotropy in two-dimensional systems has enormous scientific and technological implications. The uniaxial anisotropy universally exhibited by two-dimensional magnets has only two stable spin directions, demanding 180…

Quantum magnets with spin $J=2$, which arise in spin-orbit coupled Mott insulators, can potentially display multipolar orders. We carry out an exact diagonalization study of a simple octahedral crystal field Hamiltonian for two electrons,…

Strongly Correlated Electrons · Physics 2020-04-17 Sreekar Voleti , Dalini D. Maharaj , Bruce D. Gaulin , Graeme Luke , Arun Paramekanti

We have studied the electronic structure of BaCoO$_3$ using soft x-ray absorption spectroscopy at the Co-$L_{2,3}$ and O-$K$ edges, magnetic circular dichroism at the Co-$L_{2,3}$ edges, as well as valence band hard x-ray photoelectron…

Correlated materials with competing spin-orbit and crystal-field interactions can host composite spin-orbital magnons that are highly susceptible to structural and electronic perturbations, enabling the control of magnetic dynamics beyond…

The superfluid-Mott insulator transition of spin-2 boson atoms with repulsive interaction in an optical lattice in a magnetic field is presented. By using the mean field theory, Mott ground states and phase diagrams of superfluid-Mott…

Soft Condensed Matter · Physics 2009-11-10 Shuo Jin , Jing-Min Hou , Bing-Hao Xie , Li-Jun Tian , Mo-Lin Ge

We investigated the magnetic properties of the ilmenite-type iridate CdIrO$_3$ with a honeycomb lattice formed by Ir$^{4+}$ ions prepared via a solid-state metathesis. The magnetization measurements with using the powder sample reveal a…

Strongly Correlated Electrons · Physics 2020-04-20 Yuya Haraguchi , Hiroko Aruga Katori

We demonstrate that magnetic $3d$ impurities with $S=3/2$ spins and no orbital degree of freedom induce changes of spin-orbital order in a $4d^4$ Mott insulator with $S=1$ spins. Impurities act either as spin defects which decouple from the…

Strongly Correlated Electrons · Physics 2016-03-02 Wojciech Brzezicki , Mario Cuoco , Andrzej M. Oleś