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The magnetic structure of the mixed antiferromagnet NdMn$_{0.8}$Fe$_{0.2}$O$_3$ was resolved. Neutron powder diffraction data definitively resolve the Mn-sublattice with a magnetic propagation vector ${\bf k} = (000)$ and with the magnetic…

We investigate the effect of alloying at the 3d transition metal site of a rare-earth-transition metal oxide, by considering NdFe0.5Cr0.5O3 alloy with two equal and random distribution of 3d ions, Cr and Fe, interacting with an early 4f…

The structural, magnetic, and electronic properties of NdFe$_{0.5}$Mn$_{0.5}$O$_3$ have been studied in detail using bulk magnetization, neutron/x-ray diffraction and first principles density functional theory calculations. The material…

Strongly Correlated Electrons · Physics 2017-10-25 Ankita Singh , A. Jain , Avijeet Ray , B. Padmanabhan , S. M. Yusuf , T. Maitra , V. K. Malik

The structural and magnetic phase transitions have been studied on NdFeAsO single crystals by neutron and x-ray diffraction complemented by resistivity and specific heat measurements. Two low-temperature phase transitions have been observed…

The magnetic structure of the "nonmetallic metal" FeCrAs, a compound with the characters of both metals and insulators, was examined as a function of temperature using single-crystal neutron diffraction. The magnetic propagation vector was…

Strongly Correlated Electrons · Physics 2019-11-21 W. T. Jin , M. Meven , H. Deng , Y. Su , W. Wu , S. R. Julian , Young-june Kim

We investigated the magnetic phase diagram of single crystals of SrNdFeO$_{4}$ by measuring the magnetic properties, the specific heat and the dielectric permittivity. The system has two magnetically active ions, Fe$^{3+}$ and Nd$^{3+}$.…

Materials Science · Physics 2015-06-05 J. M. Hwang , E. S. Choi , H. D. Zhou , Y. Xin , J. Lu , P. Schlottmann

We investigated the low energy excitations in the parent compound NdFeAsO of the Fe-pnictide superconductor in the $\mu$eV range by a back scattering neutron spectrometer. The energy scans on a powder NdFeAsO sample revealed inelastic peaks…

Strongly Correlated Electrons · Physics 2012-07-03 T. Chatterji , G. N. Iles , B. Frick , A. Marcinkova , J. -W. G. Bos

Neutron and synchrotron resonant X-ray magnetic scattering (RXMS) complemented by heat capacity and resistivity measurements reveal the evolution of the magnetic structures of Fe and Ce sublattices in single crystal CeFeAsO. The RXMS of…

The magnetic structures and the magnetic phase transitions in the Mn-doped orthoferrite TbFeO$_3$ studied using neutron powder diffraction are reported. Magnetic phase transitions are identified at $T^\mathrm{Fe/Mn}_N \approx$ 295~K where a…

Strongly Correlated Electrons · Physics 2016-02-17 Harikrishnan S. Nair , Tapan Chatterji , C. M. N. Kumar , T. Hansen , Hariharan Nhalil , Suja Elizabeth , A. M. Strydom

A combination of synchrotron X-ray, neutron powder diffraction, magnetization, heat capacity and electrical resistivity measurements reveals that NdMnAsO is an antiferromagnetic semiconductor with large Neel temperature (TN = 359(2) K). At…

Superconductivity · Physics 2010-12-01 A. Marcinkova , T. C. Hansen , C. Curfs , S. Margadonna , J. W. G. Bos

The spin reorientation (SR) phenomenon of the square-lattice antiferromagnets RMnAsO (R = Ce, Nd) was investigated by analyzing the spin exchange interactions between the rare-earth and transition-metal ions (R3+ and Mn2+, respectively) on…

Strongly Correlated Electrons · Physics 2012-05-30 Changhoon Lee , Erjun Kan , Hongjun Xiang , Reinhard K. Kremer , Seung-Hun Lee , Zenji Hiroi , Myung-Hwan Whangbo

Structure and magnetic properties of high-quality polycrystlline CeMnAsO, a parent compound of the "1111"-type oxypnictides, have been investigated using neutron powder diffraction and magnetization measurements. We find that CeMnAsO…

Strongly Correlated Electrons · Physics 2015-02-24 Qiang Zhang , Wei Tian , Spencer G. Peterson , Kevin W. Dennis , David Vaknin

Spin reorientation transitions and other related magnetic phenomena, which owe their origin to the complex interplay between multiple magnetic sublattices, have long attracted scientific attention both from the perspective of fundamental…

Materials Science · Physics 2021-10-07 Hena Das , Alejandro F. Rébola , Tanusri Saha-Dasgupta

The magnetic structures adopted by the Fe and Sm sublattices in SmFeAsO have been investigated using element specific x-ray resonant and non-resonant magnetic scattering techniques. Between 110 and 5 K, the Sm and Fe moments are aligned…

We report a polarised neutron study of the magnetic structures and phase trasitions in \gdc\ in low magnetic fields. These experiments have been complemented by integrated intensity measurements with unpolarised neutrons in zero field.…

Strongly Correlated Electrons · Physics 2012-07-03 P. J. Brown , T. Chatterji

We report the magnetic field dependence of resistivity ($\rho$) and specific heat ($C$) for the non-superconducting PrFeAsO compound. Our study shows a hitherto unobserved anomaly at $T_{SR}$ in the resistivity and specific heat data which…

Strongly Correlated Electrons · Physics 2011-12-15 D. Bhoi , P. Mandal , P. Choudhury , S. Pandya , V. Ganesan

Using complementary polarized and unpolarized single-crystal neutron diffraction, we have investigated the temperature-dependent magnetic structures of Eu$_{0.5}$Ca$_{0.5}$Fe$_{2}$As$_{2}$. Upon 50 \% dilution of the Eu sites with isovalent…

Strongly Correlated Electrons · Physics 2019-04-11 W. T. Jin , M. Meven , A. P. Sazonov , S. Demirdis , Y. Su , Y. Xiao , Z. Bukowski , S. Nandi , Th. Brückel

We report the experimental observation of spin reorientation in the double perovskite Ho$_2$FeCoO$_6$. The magnetic phase transitions in this compound are characterized and studied through magnetization and specific heat, and the magnetic…

In the metallic magnet Nb$_{1-y}$Fe$_{2+y}$, the low temperature threshold of ferromagnetism can be investigated by varying the Fe excess $y$ within a narrow homogeneity range. We use elastic neutron scattering to track the evolution of…

Neutron diffraction and muon spin relaxation measurements are used to obtain a detailed phase diagram of Pr(Fe,Ru)AsO. The isoelectronic substitution of Ru for Fe acts effectively as spin dilution, suppressing both the structural and…

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