English

Tuning the magnetic and structural phase transitions of PrFeAsO via Fe/Ru spin dilution

Superconductivity 2015-06-22 v1

Abstract

Neutron diffraction and muon spin relaxation measurements are used to obtain a detailed phase diagram of Pr(Fe,Ru)AsO. The isoelectronic substitution of Ru for Fe acts effectively as spin dilution, suppressing both the structural and magnetic phase transitions. The temperature of the tetragonal-orthorhombic structural phase transition decreases gradually as a function of x. Slightly below the transition temperature coherent precessions of the muon spin are observed corresponding to static magnetism, possibly reflecting a significant magneto-elastic coupling in the FeAs layers. Short range order in both the Fe and Pr moments persists for higher levels of x. The static magnetic moments disappear at a concentration coincident with that expected for percolation of the J1-J2 square lattice model.

Keywords

Cite

@article{arxiv.1407.4067,
  title  = {Tuning the magnetic and structural phase transitions of PrFeAsO via Fe/Ru spin dilution},
  author = {Yuen Yiu and Pietro Bonfà and Samuele Sanna and Roberto De Renzi and Pietro Carretta and Michael A. McGuire and Ashfia Huq and Stephen E. Nagler},
  journal= {arXiv preprint arXiv:1407.4067},
  year   = {2015}
}