English

Ultra-small moment incommensurate spin density wave order masking a ferromagnetic quantum critical point in NbFe$_2$

Strongly Correlated Electrons 2019-12-18 v2

Abstract

In the metallic magnet Nb1y_{1-y}Fe2+y_{2+y}, the low temperature threshold of ferromagnetism can be investigated by varying the Fe excess yy within a narrow homogeneity range. We use elastic neutron scattering to track the evolution of magnetic order from Fe-rich, ferromagnetic Nb0.981_{0.981}Fe2.019_{2.019} to approximately stoichiometric NbFe2_2, in which we can, for the first time, characterise a long-wavelength spin density wave state burying a ferromagnetic quantum critical point. The associated ordering wavevector qSDW=\mathbf{q}_{\rm SDW}=(0,0,lSDWl_{\rm SDW}) is found to depend significantly on yy and TT, staying finite but decreasing as the ferromagnetic state is approached. The phase diagram follows a two order-parameter Landau theory, for which all the coefficients can now be determined. Our findings suggest that the emergence of SDW order cannot be attributed to band structure effects alone. They indicate a common microscopic origin of both types of magnetic order and provide strong constraints on related theoretical scenarios based on, e.g., quantum order by disorder.

Keywords

Cite

@article{arxiv.1704.08379,
  title  = {Ultra-small moment incommensurate spin density wave order masking a ferromagnetic quantum critical point in NbFe$_2$},
  author = {P. G. Niklowitz and M. Hirschberger and M. Lucas and P. Cermak and A. Schneidewind and E. Faulhaber and J. -M. Mignot and W. J. Duncan and A. Neubauer and C. Pfleiderer and F. M. Grosche},
  journal= {arXiv preprint arXiv:1704.08379},
  year   = {2019}
}

Comments

Addition of absolute magnetic moment estimates and of a two order-parameter Landau model analysis