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We studied the high-order harmonic generation (HHG) from 2D solid materials in circularly and bichromatic circularly polarized laser fields numerically by simulating the dynamics of single-active-electron processes in 2D periodic…

The harmonic emission from cluster nanoplasmas subject to short, intense infrared laser pulses is analyzed by means of particle-in-cell simulations. A pronounced resonant enhancement of the low-order harmonic yields is found when the Mie…

Plasma Physics · Physics 2009-11-13 M. Kundu , S. V. Popruzhenko , D. Bauer

We develop a numerical scheme to investigate the high-order harmonic generation (HHG) in intense laser-matter interactions. Tracing the time evolution of every electronic laser-field-free state, we "observe" the HHG in a time-integrated…

Atomic Physics · Physics 2008-11-14 Y. J. Chen , J. Liu , Bambi Hu

We present theoretical results on the high-harmonic generation (HHG) in bulk diamond induced by intense laser pulse of wavelength 800 nm and duration 15 fs. For laser intensity in the range $1 \le I \le 50 $ TW/cm$^2$ above bandgap…

Atomic Physics · Physics 2018-02-23 Tzveta Apostolova , Boyan Obreshkov

We predict high-order harmonics in which the polarization within the spectral bandwidth of each harmonic varies continuously and significantly. For example, the interaction of counter-rotating circularly-polarized bichromatic drivers having…

Optics · Physics 2014-10-24 Avner Fleischer , Ofer Kfir , Pavel Sidorenko , Oren Cohen

Asymmetric molecules look different when viewed from one side or the other. This difference influences the electronic structure of the valence electrons, thereby giving stereo sensitivity to chemistry and biology. We show that attosecond…

We study the generation of terahertz radiation from atoms and molecules driven by an ultrashort fundamental laser and its second harmonic field by solving time-dependent Schr\"odinger equation (TDSE). The comparisons between one-, two-, and…

We study nonlinear optical response of Landau quantized graphene to an intense electromagnetic wave. In particular, we consider high harmonic generation process. It is shown that one can achieve efficient generation of high harmonics with…

Mesoscale and Nanoscale Physics · Physics 2017-05-24 H. K. Avetissian , A. G. Ghazaryan , G. F. Mkrtchian , Kh. V. Sedrakian

Present photoionization experiments cannot measure molecular frame photoelectron angular distributions (MFPAD) from the outermost valence electrons of molecules. We show that details of the MFPAD can be retrieved with high-order harmonics…

Atomic Physics · Physics 2009-05-24 Anh-Thu Le , R. R. Lucchese , M. T. Lee , C. D. Lin

It is demonstrated by single-atom simulations that X-ray signals in the 3.4 to 4 keV region from an 8 micron laser driven high harmonic generation can be increased by more than two orders of magnitude when a single-cycle pulse centered at…

Atomic Physics · Physics 2019-04-24 Zenghu Chang

We study high order harmonics generation (HHG) in crystalline silicon and diamond subjected to near and mid-infrared laser pulses. We employ time-dependent density functional theory and solve the time-dependent Kohn-Sham equation in the…

Materials Science · Physics 2022-08-31 David Freeman , Shunsuke Yamada , Atsushi Yamada , Kazuhiro Yabana , Anatoli Kheifets

We studied the high-harmonic generation by the interaction of sub-cycle laser pulses with the He atom. The sub-cycle pulses are modeled using the complex source vector beam model, which is an exact solution to Maxwell's equations and…

Using a quantum mechanical three-step model we present numerical calculations on the high-harmonic generation from four polyatomic molecules. Ethylene (C$_2$H$_4$) serves as an example where orbital symmetry directly affects the harmonic…

Atomic Physics · Physics 2007-10-20 C. B. Madsen , L. B. Madsen

We report the observation of macroscopic field-free orientation, i.e. more than 73 % of CO molecules pointing in the same direction. This is achieved through an all-optical scheme operating at high particle densities ($>10^{17}$cm$^{-3}$)…

Chemical Physics · Physics 2014-07-09 P. M. Kraus , D. Baykusheva , H. J. Wörner

We derive a simple theory for high-order harmonic generation due to pumping a noninteracting metal with a large amplitude oscillating electric field. The model assumes that the radiated light field arises from the acceleration of electrons…

Optics · Physics 2015-01-12 J. K. Freericks , A. Y. Liu , A. F. Kemper , T. P. Devereaux

We present the generation of high order harmonics in crystalline silicon subjected to intense near-infrared 30fs laser pulse. The harmonic spectrum extends from the near infrared to the extreme ultraviolet spectral region. Depending on the…

Atomic Physics · Physics 2020-08-10 Boyan Obreshkov , Tzveta Apostolova

We present a generic approach for treating the effect of nuclear motion in the high-order harmonic generation from polyatomic molecules. Our procedure relies on a separation of nuclear and electron dynamics where we account for the…

Atomic Physics · Physics 2010-04-21 C. B. Madsen , M. Abu-samha , L. B. Madsen

We theoretically consider the phenomenon of field-free long-lasting orientation of symmetric-top molecules ionized by two-color laser pulses. The anisotropic ionization produces a significant long-lasting orientation of the surviving…

Chemical Physics · Physics 2023-03-08 Long Xu , Ilia Tutunnikov , Yehiam Prior , Ilya Sh. Averbukh

We demonstrate coherent hard electromagnetic radiation generation from reflection by the electron density singularity formed at the relativistic bow wave in laser plasma via particle-in-cell simulations. Wake and bow waves driven by an…

High-order harmonic generation by a bicircular field, which consists of two coplanar counter-rotating circularly polarized fields of frequency $r\omega$ and $s\omega$ ($r$ and $s$ are integers), is investigated for a polyatomic molecule.…

Atomic Physics · Physics 2016-10-05 Senad Odžak , Elvedin Hasović , Dejan B. Milošević
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