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Related papers: Oriented rotational wave-packet dynamics studies v…

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We show that circularly polarized femtosecond laser pulses produce field-free alignment in linear and planar molecules. We study the rotational wavepacket evolution of O$_2$ and benzene created by circularly polarized light. For benzene, we…

Chemical Physics · Physics 2014-06-06 C T L Smeenk , P B Corkum

Research of the nonlinear optical characteristics of transition metal dichalcogenides in the presence of photoactive particles, plasmonic nanocavities, waveguides, and metamaterials is still in its early stages. This investigation delves…

Coherent, optically dressed media composed of two-level molecular systems without inversion symmetry are considered as all-optically tunable sources of coherent radiation in the microwave domain. A theoretical model and a numerical toolbox…

Quantum Physics · Physics 2020-12-08 Piotr Gładysz , Piotr Wcisło , Karolina Słowik

Quantum emitters inside optical cavities can create not only fixed photon number states but also photon number wave packets, which are states with a finite photon number distribution that oscillates in time. These states emerge when the…

Quantum Physics · Physics 2025-09-04 Luca Nimmesgern , Moritz Cygorek , Doris E. Reiter , Vollrath Martin Axt

We report measurements and theoretical simulations of high-order harmonic generation (HHG) in aligned N$_2$ molecules using a 1200-nm intense laser field when the generating pulse is perpendicular to the aligning one. With increasing laser…

An all-optical measurement of high-order fractional molecular echoes is demonstrated by using high-order harmonic generation (HHG). Excited by a pair of time-delayed short laser pulses, the signatures of full and high order fractional (1/2…

Chemical Physics · Physics 2019-10-23 Baoning Wang , Lixin He , Yanqing He , Yinfu Zhang , Renzhi Shao , Pengfei Lan , Peixiang Lu

As an attractive degree of freedom in electromagnetic (EM) waves, the orbital angular momentum (OAM) enables infinite communication channels for both classical and quantum communications. The exploration of OAM generation inspires various…

Optics · Physics 2018-08-21 Menglin L. N. Chen , Li Jun Jiang , Wei E. I. Sha

The extreme nonlinear optical process of high-harmonic generation (HHG) makes it possible to map the properties of a laser beam onto a radiating electron wavefunction, and in turn, onto the emitted x-ray light. Bright HHG beams typically…

Control of molecular rotations by laser fields is an active area of research focusing on the alignment/orientation of otherwise isotropic molecular samples. Oriented molecules are useful in many applications, such as molecular orbital…

Chemical Physics · Physics 2020-07-03 Long Xu , Ilia Tutunnikov , Erez Gershnabel , Yehiam Prior , Ilya Sh. Averbukh

High-harmonic generation in two-colour ($\omega-2\omega$) counter-rotating circularly polarised laser fields opens the path to generate isolated attosecond pulses and attosecond pulse trains with controlled ellipticity. The generated…

The generation of high harmonics is a strongly nonlinear effect that allows to probe properties of the target and to study electron dynamics in matter. It has been investigated in many different kinds of targets, including molecular gases,…

Quantum Physics · Physics 2026-05-06 Lina Bielke , Samuel Schöpa , Falk-Erik Wiechmann , Franziska Fennel , Dieter Bauer

It is shown that highly localized solitons can be created in lower dimensional Bose-Einstein condensates (BEC), trapped in a regular harmonic trap, by temporally varying the trap frequency. A BEC trapped in such a trap can be effectively…

Other Condensed Matter · Physics 2009-09-29 S. Sree Ranjani , P. K. Panigrahi , A. K. Kapoor

We investigate the alignment-dependent high-order harmonic spectrum generated from nonadiabatically aligned molecules around the first half rotational revival. It is found that the evolution of the molecular alignment is encoded in the…

Atomic Physics · Physics 2014-03-13 Meiyan Qin , Xiaosong Zhu , Yang Li , Qingbin Zhang , Pengfei Lan , Peixiang Lu

The physics of high harmonics has led to the generation of attosecond pulses and to trains of attosecond pulses. Measurements that confirm the pulse duration are all performed in the far field. All pulse duration measurements tacitly assume…

Optics · Physics 2012-06-15 E. Frumker , G. G. Paulus , H. Niikura , A. Naumov , D. M. Villeneuve , P. B. Corkum

We report the enhancement of individual harmonics generated at a relativistic ultra-steep plasma vacuum interface. Simulations show the harmonic emission to be due to the coupled action of two high velocity oscillations -- at the…

We demonstrate a new high-order harmonic generation mechanism reaching the `water window' spectral region in experiments with multi-terawatt femtosecond lasers irradiating gas jets. A few hundred harmonic orders are resolved, giving uJ/sr…

The use of tunable pre-pulse is a common technique to enhance the high-order harmonic generation from surface plasma. The shape and dynamic of the electron density, the degree of ionization and its rate, and the plasma heating are…

In our recent study [Commun. Phys. 3, 92 (2020)], we have developed an approach for energy-scaling of high-order harmonic generation in water-window region under neutral-medium condition. More specifically, we obtained nanojoule-class…

We present what is probably the simplest classical system featuring the echo phenomenon - a collection of randomly oriented free rotors with dispersed rotational velocities. Following excitation by a pair of time-delayed impulsive kicks,…

Applying time-dependent local density approximation (TDLDA), we study the high-order harmonic generation (HHG) of ethylene subjected to the one-color ($\omega=2.72$ eV) and the two-color ($\omega_1=2.72$ eV and $\omega_2=5.44$ eV)…

Atomic and Molecular Clusters · Physics 2009-03-31 Z. P. Wang , P. M. Dinh , P. -G. Reinhard , E. Suraud , F. S. Zhang