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Non-classical multi-photon and number states attracts many people because of their wide applications in fundamental quantum mechanics tests, quantum metrology and quantum computation, therefore it is a longstanding aim to generate such…

Quantum Physics · Physics 2015-01-13 Dong-Sheng Ding , Wei Zhang , Shuai Shi , Zhi-Yuan Zhou , Yan Li , Bao-Sen Shi , Guang-Can Guo

Cooling the rotation and the vibration of molecules by broadband light sources was possible for trapped molecular ions or ultracold molecules. Because of a low power spectral density, the cooling timescale has never fell below than a few…

Atomic Physics · Physics 2018-06-06 A. Cournol , P. Pillet , H. Lignier , D. Comparat

Subradiance, i.e. the cooperative inhibition of spontaneous emission by destructive interatomic interference, can be realized in a cold atomic sample confined in a ring cavity and lightened by a two-frequency laser. The atoms, scattering…

Other Condensed Matter · Physics 2015-05-13 M. M. Cola , D. Bigerni , N. Piovella

We present a new theoretical scheme for laser cooling of rare earth doped solids with optical super-radiance (SR), which is the coherent, sharply directed spontaneous emission of photons by a system of laser excited rare earth ions in the…

Optics · Physics 2015-05-19 Galina Nemova , Raman Kashyap

A novel atom-molecule conversion technique has been investigated. Ultracold 85Rb atoms sitting in a DC magnetic field near the 155G Feshbach resonance are associated by applying a small sinusoidal oscillation to the magnetic field. There is…

Other Condensed Matter · Physics 2009-11-11 S. T. Thompson , E. Hodby , C. E. Wieman

Singlet exciton fission has the potential to increase the efficiency of crystalline silicon solar cells beyond the conventional single junction limit. Perhaps the largest obstacle to achieving this enhancement is uncertainty about energy…

The formation of ultracold metastable RbCs molecules is observed in a double species magneto-optical trap through photoassociation below the ^85Rb(5S_1/2)+^133Cs(6P_3/2) dissociation limit followed by spontaneous emission. The molecules are…

Atomic Physics · Physics 2015-06-03 N. Bouloufa-Maafa , M. Aymar , O. Dulieu , C. Gabbanini

Laser cooling is theoretically investigated in a cascade three-level scheme, where the excited state of a laser-driven transition is coupled by a second laser to a top, more stable level, as for alkali-earth atoms. The second laser action…

Quantum Physics · Physics 2013-05-29 Giovanna Morigi , Ennio Arimondo

Charge transfer multiplet (CTM) theory is a computationally undemanding and highly mature method for simulating the soft X-ray spectra of first-row transition metal complexes. However, CTM theory has seldom been applied to the simulation of…

Chemical Physics · Physics 2018-03-06 Kaili Zhang , Gregory S. Girolami , Josh Vura-Weis

We perform magnetically-assisted Sisyphus laser cooling of the triatomic free radical strontium monohydroxide (SrOH). This is achieved with principal optical cycling in the rotationally closed $P\left(N"=1\right)$ branch of either the…

We consider two-color heteronuclear photoassociation of atoms into dipolar molecules in the J=1 electro-vibrational ground state, where a free-ground laser couples atoms directly to the ground state and a free-bound laser couples the atoms…

Quantum Gases · Physics 2009-11-19 Matt Mackie , Catherine DeBrosse

The continuous pumping of atoms into a Bose-Einstein condensate via spontaneous emission from a thermal reservoir is analyzed. We consider the case of atoms with a three-level $\Lambda$ scheme, in which one of the atomic transitions has a…

Quantum Physics · Physics 2009-11-06 L. Santos , F. Floegel , T. Pfau , M. Lewenstein

We propose a method that enables efficient frequency conversion of quantum information based on recently demonstrated strong parametric coupling between two single-photon pulses propagating in a slow-light atomic medium at different group…

Quantum Physics · Physics 2015-05-14 A. Gogyan , Yu. Malakyan

Chemical reactions typically proceed via stochastic encounters between reactants. Going beyond this paradigm, we combine exactly two atoms into a single, controlled reaction. The experimental apparatus traps two individual laser-cooled…

Atomic Physics · Physics 2018-04-25 L. R. Liu , J. D. Hood , Y. Yu , J. T. Zhang , N. R. Hutzler , T. Rosenband , K. -K. Ni

The majority of molecules proposed for laser cooling and trapping experiments have $\Sigma$-type ground states. Specifically, $^2\Sigma$ states have cycling transitions analogous to D1-lines in alkali-metal atoms while $^1\Sigma$ states…

Atomic Physics · Physics 2024-09-04 J. R. Daniel , J. C. Shaw , C. Wang , L. -R. Liu , B. K. Kendrick , B. Hemmerling , D. J. McCarron

The paper investigates cold molecules formation in the photoassociation of two cold atoms by a strong laser pulse applied at short interatomic distances, which lead to a molecular dynamics taking place in the light-induced (adiabatic)…

Quantum Physics · Physics 2009-07-23 M. Vatasescu

We demonstrate a new spectroscopic method for studying electronic transitions in molecules with extremely broad range of angular momentum. We employ an optical centrifuge to create narrow rotational wave packets in the ground electronic…

Chemical Physics · Physics 2017-09-13 Aleksey Korobenko , Alexander A. Milner , John W. Hepburn , Valery Milner

We investigated transition strengths from ultracold weakly bound 41K87Rb molecules produced via the photoassociation of laser-cooled atoms. An accurate potential energy curve of the excited state (3)1Sigma+ was constructed by carrying out…

Atomic Physics · Physics 2015-05-20 K. Aikawa , D. Akamatsu , M. Hayashi , J. Kobayashi , M. Ueda , S. Inouye

We demonstrate Doppler-free saturated absorption spectroscopy of cold molecular radicals formed by laser ablation inside a cryogenic buffer gas cell. By lowering the temperature, congested regions of the spectrum can be simplified, and by…

We report cooling of a single neutral atom to its three-dimensional vibrational ground state in an optical tweezer. After employing Raman sideband cooling for tens of milliseconds, we measure via sideband spectroscopy a three-dimensional…

Atomic Physics · Physics 2012-11-30 Adam M. Kaufman , Brian J. Lester , Cindy A. Regal