Related papers: Triplet-singlet conversion by broadband optical pu…
We present a magnetically enhanced laser cooling scheme applicable to multi-level type-II transitions and further diatomic molecules with adiabatic transfer. An angled magnetic field is introduced to not only remix the dark states, but also…
Exploring inelastic and reactive collisions on the quantum level is a main goal of the developing field of ultracold chemistry. We present first experimental studies of inelastic collisions of metastable ultracold triplet molecules in the…
It is shown theoretically how to directly obtain the energy distribution of a weakly interacting gas of bosons confined in an optical lattice in the tight-binding limit. This is accomplished by adding a linear potential to a suitably…
We show that ordered monolayers of organic molecules stabilized by hydrogen bonding on the surface of exfoliated few-layer hexagonal boron nitride (hBN) flakes may be incorporated into van der Waals heterostructures with integral few-layer…
While conventional lasers are based on gain media with three or four real levels, unconventional lasers including virtual levels and two-photon processes offer new opportunities. We study lasing that involves a two-photon process through a…
Multiphoton states are needed for quantum communication and computation. Multiphoton states are significantly more difficult to generate than one- and two-photon states because two individual down-conversion processes must be cascaded. Only…
Molecular spin systems based on photoexcited triplet pairs formed via singlet fission (SF) are attractive as carriers of quantum information because of their potentially pure and controllable spin polarization, but developing systems that…
Third-order parametric down-conversion (TOPDC) describes a class of nonlinear interactions in which a pump photon is converted into a photon triplet. This process can occur spontaneously, or it can be stimulated by seeding fields. In the…
Cadmium is laser-cooled and trapped with excitations to triplet states with UVA light, first using only the $67\,$kHz wide $326\,$nm intercombination line and subsequently, for large loading rates, the $25\,$MHz wide $361\,$nm…
Laser-cooled atoms coupled to nanophotonic structures constitute a powerful research platform for the exploration of new regimes of light-matter interaction. While the initialization of the atomic internal degrees of freedom in these…
At ambient temperatures, CeRuSn exhibits an extraordinary structure with a coexistence of two types of Ce ions in a metallic environment, namely trivalent Ce3+ and intermediate valent Ce(4-x)+. Charge ordering produces a doubling of the…
We present a method for creating a quantum degenerate gas of metastable alkaline-earth atoms. This has yet to be achieved due to inelastic collisions that limit evaporative cooling in the metastable states. Quantum degenerate samples…
Singlet fission, a spin-allowed energy transfer process generating two triplet excitons from one singlet exciton, has the potential to dramatically increase the efficiency of organic solar cells. However, the dynamical mechanism of this…
We present an X-ray based stimulated Raman approach to control the preparation of optically dark electronic states in generic molecular systems. Leveraging on the unique properties of core-level excited states, we demonstrate that optically…
We present a generalization of the diagrammatic pump-probe approach to coherent backscattering (CBS) of intense laser light for atoms with degenerate energy levels. We employ this approach for a characterization of the double scattering…
A conditioned unitary transformation ($90^o$ polarization rotation) is performed at single-photon level. The transformation is realized by rotating polarization for one of the photons of a polarization-entangled biphoton state (signal…
Polaritons, mixed light-matter quasiparticles, undergo a transition to a condensed, macroscopically coherent state at low temperatures or high densities. Recent experiments show that coupling light to organic molecules inside a microcavity…
The ability to efficiently produce and manipulate nonclassical states of light is a critical requirement for the development of quantum optical technologies. In recent years, experiments have demonstrated that cascaded spontaneous…
We probe the dynamics of dissociating CS$_2$ molecules across the entire reaction pathway upon excitation. Photoelectron spectroscopy measurements using laboratory-generated femtosecond extreme ultraviolet pulses monitor the competing…
We report the first observation of an optical transition from a ground trion state T to excited trion state T* in (6,5) single-wall carbon nanotubes non-covalently doped with hydrochloric acid. The position of such an excited trion level T*…