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We present a comprehensive characterization of cold molecular beams from a cryogenic buffer-gas cell, providing an insight into the physics of buffer-gas cooling. Cold molecular beams are extracted from a cryogenic cell by electrostatic…
A novel, computationally designed, class of triangular-shape organic molecules with an inverted singlet-triplet (IST) energy gap is investigated with the aid of ab initio methods of electronic structure theory. The considered molecular…
Photon upconverters are anti Stokes emitters capable of generating photons with higher energy than those absorbed. This behavior can be achieved through different mechanisms, which are extensively studied for applications in imaging,…
We propose a laser cooling concept for the translational motion of molecules which does not require repeated spontaneous emission by each molecule. The cooling works by repetition of three main steps: velocity selection of a narrow momentum…
This theoretical paper investigates the formation of ground state molecules from ultracold cesium atoms in a two-color scheme. Following previous work on photoassociation with chirped picosecond pulses [Luc-Koenig et al., Phys. Rev. A {\bf…
We report coherent association of atoms into a single weakly bound NaCs molecule in an optical tweezer through an optical Raman transition. The Raman technique uses a deeply bound electronic excited intermediate state to achieve a large…
We present a new method for the generation of rotationally and vibrationally state-selected, translationally cold molecular ions in ion traps. Our technique is based on the state-selective threshold photoionization of neutral molecules…
We propose an alternative method to laser cooling. Our approach utilizes the extreme brightness of a supersonic atomic beam, and the adiabatic atomic coilgun to slow atoms in the beam or to bring them to rest. We show how internal-state…
In this paper we propose an alternative scheme to generate a supersinglet state of three three-level atoms via a single-mode of a cavity QED based on the two-photon transitions described by the 'full microscopical Hamiltonian approach'. In…
We propose cascaded spontaneous four-wave mixing (SFWM) in microring resonators as a scalable and efficient approach for directly generating non-Gaussian states of light. Focusing on the well-understood "low-gain" regime, we demonstrate…
We employ semiclassical theoretical analysis to study laser cooling of free atoms using three-level cascade transitions, where the upper transition is much weaker than the lower one. This represents an alternate cooling scheme, particularly…
A ray of photons, emitted from a laser source, is in a coherent state, where macroscopic number of photons are degenerate in the same quantum state. The coherent state has degrees of freedom for spin and orbital angular momentum, which…
Singlet fission is a photoconversion process that generates a doubly excited, maximally spin entangled pair state. This state has applications to quantum information and computing that are only beginning to be realized. In this article, we…
We present a method for producing three-dimensional Bose-Einstein condensates using only laser cooling. The phase transition to condensation is crossed with $2.5 {\times} 10^{4}$ $^{87}\mathrm{Rb}$ atoms at a temperature of $T_{\mathrm{c}}…
One possibility for the creation of ultracold, high-phase-space-density quantum gases of molecules in the rovibrational ground state relies on first associating weakly-bound molecules from quantum-degenerate atomic gases on a Feshbach…
Laser cooling of single atoms in optical tweezers is a prerequisite for neutral atom quantum computing and simulation. Resolved sideband cooling comprises a well-established method for efficient motional ground-state preparation, but…
We demonstrate 3D microwave projection sideband cooling of trapped, neutral atoms. The technique employs state-dependent potentials that enable microwave photons to drive vibration-number reducing transitions. The particular cooling…
We propose a highly efficient and fast method of translational cooling for high-angular-momentum atoms. Optical pumping and stimulated transitions, combined with magnetic forces, can be used to compress phase-space density, and the…
CeRuSn exhibits an extraordinary room temperature structure at 300~K with coexistence of two types of Ce ions, namely trivalent Ce$^{3+}$ and intermediate valent Ce$^{(4-\delta)+}$, in a metallic environment. The ordered arrangement of…
We present a generic theory of primary photoexcitations in low band gap donor-acceptor conjugated copolymers. Because of the combined effects of strong electron correlations and broken symmetry, there is considerable mixing between a…