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The magnetic ground states of $R_2$Ru$_2$O$_7$ and $A_2$Ru$_2$O$_7$ with $R=$ Pr, Gd, Ho, and Er, as well as $A=$ Ca, Cd are predicted devising a combination of the cluster-multipole (CMP) theory and spin-density-functional theory (SDFT).…

Strongly Correlated Electrons · Physics 2022-02-22 Marie-Therese Huebsch , Yuske Nomura , Shiro Sakai , Ryotaro Arita

By systematic first-principles calculations, we study the electronic structure and magnetic property of SrCrO$_3$. Our results suggest that SrCrO$_3$ is a weakly correlated antiferromagnetic (AF) metal, a very rare situation in…

Materials Science · Physics 2010-07-20 Guangtao Wang , Zhi Li , C. Q. Jin , Zhong Fang

Spin wave excitations and stability of the ($\pi,0$) ordered magnetic state are investigated in a minimal two-band itinerant-electron model for iron pnictides. Presence of hopping anisotropy generates a strong ferro-orbital order in the…

Strongly Correlated Electrons · Physics 2015-07-07 Sayandip Ghosh , Avinash Singh

Materials with strongly correlated electrons exhibit physical properties that are often difficult to predict as they result from the interactions of large numbers of electrons combined with several quantum degrees of freedom. The layered…

Transition metal oxides of the $4d$ and $5d$ block have recently become the targets of materials discovery, largely due to their strong spin-orbit coupling that can generate exotic magnetic and electronic states. Here we report the high…

Recent developments have led to an explosion of activity on skyrmions in three-dimensional (3D) chiral magnets. Experiments have directly probed these topological spin textures, revealed their nontrivial properties, and led to suggestions…

Strongly Correlated Electrons · Physics 2014-09-11 Sumilan Banerjee , James Rowland , Onur Erten , Mohit Randeria

First principles density functional calculations within the local spin density approximation (LSDA) and the generalized gradient approximation (GGA) are reported for pyrochlore Cd$_2$Os$_2$O$_7$ and Cd$_{2}$Re$_{2}$O$_7$. The transition…

Condensed Matter · Physics 2009-11-07 D. J. Singh , P. Blaha , K. Schwarz , J. O. Sofo

We study the $S=1/2$ pyrochlore Heisenberg antiferromagnet in a magnetic field. Using large scale density-matrix renormalization group (DMRG) calculations for clusters up to $128$ spins, we find indications for a finite triplet gap, causing…

Strongly Correlated Electrons · Physics 2022-09-14 Imre Hagymási , Robin Schäfer , Roderich Moessner , David J. Luitz

Pyrochlore magnets are candidates for spin-ice behavior. We present theoretical simulations of relevance for the pyrochlore family R2Ti2O7 (R= rare earth) supported by magnetothermal measurements on selected systems. By considering long…

Statistical Mechanics · Physics 2009-10-31 R. Siddharthan , B. S. Shastry , A. P. Ramirez , A. Hayashi , R. J. Cava , S. Rosenkranz

Research efforts on the low temperature magnetic order and electronic properties of U$_3$O$_8$ have been inconclusive so far. Reinterpreting neutron scattering results, we use group representation theory to show that the ground state…

Strongly Correlated Electrons · Physics 2023-01-24 Rolando Saniz , Gianguido Baldinozzi , Ine Arts , Gregory Leinders , Dirk Lamoen , Marc Verwerft

Pyrochlore oxides possessing "all-in-all-out" spin ordering have attracted burgeoning interest as a rich ground of emergent states. This ordering has two distinct types of magnetic domains (all-in-all-out or all-out-all-in) with broken…

Materials Science · Physics 2016-03-09 T. C. Fujita , M. Uchida , Y. Kozuka , W. Sano , A. Tsukazaki , T. Arima , M. Kawasaki

Neutron scattering and magnetization measurements have been performed on the stuffed pyrochlore system Tb2+xTi2-2xNbxO7. We find that despite the introduction of chemical disorder and increasingly antiferromagnetic interactions, a spin…

Strongly Correlated Electrons · Physics 2010-02-25 B. G. Ueland , J. S. Gardner , A. J. Williams , M. L. Dahlberg , J. G. Kim , Y. Qiu , J. R. D. Copley , P. Schiffer , R. J. Cava

Recent neutron scattering measurements on the spinel CdCr2O4 revealed a rare example of helical magnetic order in geometrically frustrated pyrochlore antiferromagnet. The spin spiral characterized by an incommensurate wavevector Q = 2pi (0,…

Strongly Correlated Electrons · Physics 2013-02-19 Eunsong Choi , Gia-Wei Chern , Natalia Perkins

We present the results of a muon-spin relaxation (muSR) investigation into magnetic ordering in several families of layered quasi-two-dimensional molecular antiferromagnets based on transition metal ions such as S=1/2 Cu2+ bridged with…

We report a resonant inelastic X-ray scattering study on a single crystal of a non-stoichiometric pyrochlore iridate Tb$_{2+x}$Ir$_{2-x}$O$_{7-y}$ ($x \simeq 0.25$) that magnetically orders at $T_{\rm{N}}\simeq 50$ K. We find that the…

Strongly Correlated Electrons · Physics 2024-09-18 Q. Faure , A. Toschi , J. R. Soh , E. Lhotel , B. Detlefs , D. Prabhakaran , D. F. McMorrow , C. J. Sahle

The manganese pnictide CaMn$_2$Bi$_2$, with Mn atoms arranged in a puckered honeycomb structure, exhibits narrow-gap antiferromagnetism, and it is currently a promising candidate for the study of complex electronic and magnetic phenomena,…

We address the concomitant metal-insulator transition (MIT) and antiferromagnetic ordering in the novel pyrochlore iridate Eu2Ir2O7 by combining x-ray absorption spectroscopy, x-ray and neutron diffractions and density functional theory…

The spin-chain compounds, Ca3CuIrO6 and Ca3CuRhO6, crystallizing in a K4CdCl6-derived monoclinic structure, are investigated by ac and dc magnetization, isothermal remnant magnetization as well as heat capacity measurements. The results…

Strongly Correlated Electrons · Physics 2009-11-10 S. Rayaprol , E. V. Sampathkumaran

The spin-liquid phase of two highly frustrated pyrochlore magnets Gd2Ti2O7 and Gd2Sn2O7 is probed using electron spin resonance in the temperature range 1.3 - 30 K. The deviation of the absorption line from the paramagnetic position \nu…

Strongly Correlated Electrons · Physics 2013-05-29 S. S. Sosin , L. A. Prozorova , A. I. Smirnov , P. Bonville , G. Jasmin - Le Bras , O. A. Petrenko

Examples of materials where an "order by disorder" mechanism is at play to select a particular ground state are scarce. It has recently been proposed, however, that the antiferromagnetic XY pyrochlore Er2Ti2O7, reveals a most convincing…

Strongly Correlated Electrons · Physics 2015-06-23 S. Petit , J. Robert , S. Guitteny , P. Bonville , C. Decorse , J. Ollivier , H. Mutka , M. J. P. Gingras , I. Mirebeau