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By many-body quantum-chemical calculations, we investigate the role of two structural effects - local ligand distortions and the anisotropic Cd-ion coordination - on the magnetic state of Cd2Os2O7, a spin S=3/2 pyrochlore. We find that…

Strongly Correlated Electrons · Physics 2013-03-28 Nikolay A. Bogdanov , Rémi Maurice , Ioannis Rousochatzakis , Jeroen van den Brink , Liviu Hozoi

The magnetic properties of the pyrochlore iridate material Eu$_2$Ir$_2$O$_7$ (5$d^5$) have been studied based on the first principle calculations, where the crystal field splitting $\Delta$, spin-orbit coupling (SOC) $\lambda$ and Coulomb…

Strongly Correlated Electrons · Physics 2017-11-08 Yilin Wang , Hongming Weng , Liang Fu , Xi Dai

We report measurements performed on a polycrystalline sample of the pyrochlore compound Nd2Sn2O7. It undergoes a second order magnetic phase transition at Tc ~ 0.91 K to a noncoplanar all-in-all-out magnetic structure of the Nd3+ magnetic…

Strongly Correlated Electrons · Physics 2015-11-04 A. Bertin , P. Dalmas de Reotier , B. Fak , C. Marin , A. Yaouanc , A. Forget , D. Sheptyakov , B. Frick , C. Ritter , A. Amato , C. Baines , P. J. C. King

We determined the magnetic structure of CuCr$_2$O$_4$ using neutron diffraction and irreducible representation analysis. The measurements identified a new phase between 155 K and 125 K as nearly collinear magnetic ordering in the Cr…

Strongly Correlated Electrons · Physics 2018-03-20 K. Tomiyasu , S. Lee , H. Ishibashi , Y. Takahashi , T. Kawamata , Y. Koike , T. Nojima , S. Torii , T. Kamiyama

We investigated the piezomagnetic effect in pyrochlore-type oxides Y$_2$Ir$_2$O$_7$ and Cd$_2$Os$_2$O$_7$, which show a non-coplanar magnetic structure called the all-in/all-out antiferromagnetic order at low temperatures. The…

Strongly Correlated Electrons · Physics 2025-05-19 Hiroki Nanjo , Yoshinori Imai , Takuya Aoyama , Junichi Yamaura , Kenya Ohgushi

The influence of spin-orbit coupling (SOC) on the physical properties of the 5d2 system Sr2MgOsO6 is probed via a combination of magnetometry, specific heat measurements, elastic and inelastic neutron scattering, and density functional…

Magnetism of ruthernium pyrochlore oxides A2Ru2O7 (A = Hg, Cd, Ca), whose electronic properties within a localized ion picture are characterized by non-degenerate t2g orbitals (Ru5+, 4d3) and thereby subject to geometrical frustration, has…

Strongly Correlated Electrons · Physics 2015-03-17 M. Miyazaki , R. Kadono , K. H. Satoh , M. Hiraishi , S. Takeshita , A. Koda , A. Yamamoto , H. Takagi

Sr$_{3}$ZnIrO$_{6}$ is an effective spin one-half Mott insulating iridate belonging to a family of magnets which includes a number of quasi-one dimensional systems as well as materials exhibiting three dimensional order. Here we present the…

Strongly Correlated Electrons · Physics 2020-05-19 P. A. McClarty , A. D. Hillier , D. T. Adroja D. D. Khalyavin , S. Rayaprol , P. Manuel , W. Kockelmann , E. V. Sampathkumaran

The Co2V2O7 is recently reported to exhibit amazing magnetic field-induced magnetization plateaus and ferroelectricity, but its magnetic ground state remains ambiguous due to its structural complexity. Magnetometry measurements, and…

Strongly Correlated Electrons · Physics 2019-10-23 W. H. Ji , Y. C. Sun , C. M. N. Kumar , C. Li , S. Nandi , W. T. Jin , Y. Su , X. Sun , Y. Lee , B. Harmon , L. Ke , Z. W. Ouyang , Y. Xiao , Th. Brueckel

We investigate the temperature dependence of the spin dynamics in the pyrochlore magnet Nd$_2$Zr$_2$O$_7$ by neutron scattering experiments. At low temperature, this material undergoes a transition towards an "all in - all out"…

Strongly Correlated Electrons · Physics 2021-07-22 M. Léger , E. Lhotel , M. Ciomaga Hatnean , J. Ollivier , A. R. Wildes , S. Raymond , E. Ressouche , G. Balakrishnan , S. Petit

Neutron scattering has been used to study the magnetic order and spin dynamics of the colossal magnetoresistive pyrochlore Tl_2Mn_2O_7. On cooling from the paramagnetic state, magnetic correlations develop and appear to diverge at T_C (123…

Strongly Correlated Electrons · Physics 2009-10-31 J. W. Lynn , L. Vasiliu-Doloc , M. A. Subramanian

We report on the muon spin rotation/relaxation study of a pyrochlore oxide, Cd2Os2O7, which exhibits a metal-insulator (MI) transition at T_{MI}~225 K without structural phase transition. It reveals strong spin fluctuation (>10^8/s) below…

Strongly Correlated Electrons · Physics 2009-11-13 A. Koda , R. Kadono , K. Ohishi , S. R. Saha , W. Higemoto , S. Yonezawa , Y. Muraoka , Z. Hiroi

The subtle interplay between spin-orbit coupling, exchange interactions, and cation ordering can lead to exotic magnetic states in transition-metal ions. We report a comprehensive study of the Re-based (5$d^1$) ordered double perovskite…

Magnetic systems with spins sitting on a lattice of corner sharing regular tetrahedra have been particularly prolific for the discovery of new magnetic states for the last two decades. The pyrochlore compounds have offered the playground…

Strongly Correlated Electrons · Physics 2017-10-05 P. Dalmas de Reotier , C. Marin , A. Yaouanc , C. Ritter , A. Maisuradze , B. Roessli , A. Bertin , P. J. Baker , A. Amato

Collinear and non-collinear spin structures of wurtzite phase CoO often appearing in nano-sized samples are investigated using first-principles density functional theory calculations. We examined the total energy of several different spin…

Materials Science · Physics 2013-06-03 Myung Joon Han , Heung-Sik Kim , Dong Geun Kim , Jaejun Yu

Cd2Os2O7 shows a peculiar metal-insulator transition at 227 K with magnetic ordering in a frustrated pyrochlore lattice, but its magnetic structure in the ordered state and the transition origin are yet uncovered. We observed a commensurate…

Strongly Correlated Electrons · Physics 2012-06-20 J. Yamaura , K. Ohgushi , H. Ohsumi , T. Hasegawa , I. Yamauchi , K. Sugimoto , S. Takeshita , A. Tokuda , M. Takata , M. Udagawa , M. Takigawa , H. Harima , T. Arima , Z. Hiroi

A supposedly nonmagnetic 5d$^1$ double perosvkite oxide is investigated by a combination of spectroscopic and theoretical methods, namely resonant inelastic X-ray scattering, X-ray absorption spectroscopy, magnetic circular dichroism, and…

The recent discovery of Spin-ice is a spectacular example of non-coplanar spin arrangements that can arise in the pyrochlore A2B2O7 structure. We present magnetic and thermodynamic studies on the metallic-ferromagnet pyrochlore Sm2Mo2O7.…

Strongly Correlated Electrons · Physics 2009-11-13 Surjeet Singh , R. Suryanarayanan , R. Tackett , G. Lawes , A. K. Sood , P. Berthet , A. Revcolevschi

Here, using density functional theory and density matrix renormalization group methods, we investigate the electronic and magnetic properties of RuOCl$_2$ and OsOCl$_2$ with $d^4$ electronic configurations. Different from a previous study…

Strongly Correlated Electrons · Physics 2022-05-16 Yang Zhang , Ling-Fang Lin , Adriana Moreo , Thomas A. Maier , Gonzalo Alvarez , Elbio Dagotto

We report neutron scattering experiments which reveal a large spin gap in the magnetic excitation spectrum of weakly-monoclinic double perovskite Sr2ScOsO6. The spin gap is demonstrative of appreciable spin-orbit-induced anisotropy, despite…

Strongly Correlated Electrons · Physics 2016-07-06 A. E. Taylor , R. Morrow , R. S. Fishman , S. Calder , A. I. Kolesnikov , M. D. Lumsden , P. M. Woodward , A. D. Christianson
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