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Alkali superoxides differ from conventional transition metal magnets, exhibit magnetism from partially occupied oxygen molecular $\pi^*$-orbitals. Among them, CsO$_2$ stands out for its potential to exhibit novel quantum collective…

Strongly Correlated Electrons · Physics 2024-11-12 Ryota Ono , Ravi Kaushik , Sergey Artyukhin , Martin Jansen , Igor Solovyev , Russell A. Ewings

We present synchrotron x-ray diffraction, neutron powder diffraction and time-of-flight inelastic neutron scattering measurements on the rare earth pyrochlore oxide Nd2Zr2O7 to study the ordered state magnetic structure and cystal field…

Strongly Correlated Electrons · Physics 2016-01-20 J. Xu , V. K. Anand , A. K. Bera , M. Frontzek , D. L. Abernathy , N. Casati , K. Siemensmeyer , B. Lake

In 3d-electron magnetic systems, the magnetic structures that transform each other by spin rotation have very close degenerate energies due to small spin-orbit coupling and can be easily controlled by chemical substitution and external…

Materials Science · Physics 2025-11-20 Vu Thi Ngoc Huyen , Yuki Yanagi , Michi-To Suzuki

Pyrochlores offer an ideal playground to investigate the magnetic ground state of frustrated magnetic systems. In this class of materials, competition between various magnetic interactions remains frustrated and prevents an ordered magnetic…

Strongly Correlated Electrons · Physics 2022-10-06 Karan Singh , Dheeraj Ranaut , G. Sharma , K. Mukherjee

The spin dynamics in the geometrically frustrated pyrochlore antiferromagnet $\rm Gd_2Sn_2O_7$ is studied by means of the electron spin resonance. In the ordered phase ($T_N = 1$ K), we have detected three gapped resonance modes. Their…

Strongly Correlated Electrons · Physics 2013-05-29 S. S. Sosin , L. A. Prozorova , P. Bonville , M. E. Zhitomirsky

The presence of spin-orbit coupling drives the anomalous magnetotransport at oxide interfaces and forms the basis for numerous intriguing properties of these 2D electron systems, such as topologically protected phases or anti-localization.…

Strongly Correlated Electrons · Physics 2018-02-28 Patrick Seiler , Jone Zabaleta , Robin Wanke , Jochen Mannhart , Thilo Kopp , Daniel Braak

We present a muon spin relaxation study on the Ising pyrochlore Nd$_2$Zr$_2$O$_7$ which develops an "all-in-all-out" magnetic order below 0.4~K. At 20~mK far below the ordering transition temperature, the zero-field muon spin relaxation…

Materials Science · Physics 2016-09-07 J. Xu , C. Balz , C. Baines , H. Luetkens , B. Lake

LiOsO$_3$ is the first experimentally confirmed polar metal with ferroelectric-like distortion. One puzzling experimental fact is its paramagnetic state down to very low temperature with negligible magnetic moment, which is anomalous…

Materials Science · Physics 2018-11-20 Y. Zhang , J. J. Gong , C. F. Li , L. Lin , Z. B. Yan , Shuai Dong , J. -M. Liu

The electronic ground state of Ca3LiOsO6 was recently considered within an intermediate coupling regime that revealed J=3/2 spin-orbit entangled magnetic moments. Through inelastic neutron scattering and density functional theory we…

Strongly Correlated Electrons · Physics 2017-11-29 S. Calder , D. J. Singh , V. O. Garlea , M. D. Lumsden , Y. G. Shi , K. Yamaura , A. D. Christianson

Er2Ti2O7 is believed to be a realization of an XY antiferromagnet on a frustrated lattice of corner-sharing regular tetrahedra. It is presented as an example of the order-by-disorder mechanism in which fluctuations lift the degeneracy of…

Strongly Correlated Electrons · Physics 2012-09-28 P. Dalmas de Reotier , A. Yaouanc , Y. Chapuis , S. H. Curnoe , B. Grenier , E. Ressouche , C. Marin , J. Lago , C. Baines , S. R. Giblin

The insulating pyrochlore compound Nd2Sn2O7 has been shown to undergo a second order magnetic phase transition at Tc ~ 0.91 K to a noncoplanar all-in--all-out magnetic structure of the Nd3+ magnetic moments. An anomalously slow paramagnetic…

Strongly Correlated Electrons · Physics 2017-05-04 P. Dalmas de Reotier , A. Yaouanc , A. Maisuradze , A. Bertin , P. J. Baker , A. D. Hillier , A. Forget

We report the observation of magnetic domains in the exotic, antiferromagnetically ordered all-in-all-out state of Nd$_2$Zr$_2$O$_7$, induced by spin canting. The all-in-all-out state can be realized by Ising-like spins on a pyrochlore…

Strongly Correlated Electrons · Physics 2017-05-16 L. Opherden , J. Hornung , T. Herrmannsdörfer , J. Xu , A. T. M. N. Islam , B. Lake , J. Wosnitza

The pyrochlore oxides $A_2B_2$O$_7$ exhibit a complex interplay between geometrical frustration, electronic correlations, and spin-orbit coupling, due to the lattice structure and active charge, spin, and orbital degrees of freedom.…

Strongly Correlated Electrons · Physics 2019-06-07 Hiroshi Shinaoka , Yukitoshi Motome , Takashi Miyake , Shoji Ishibashi , Philipp Werner

Rare-earth pyrochlores are known to exhibit exotic magnetic phenomena. We report a study of crystal growth and characterizations of a new rare-earth compound Er$_2$AlSbO$_7$, in which Al$^{3+}$ and Sb$^{5+}$ ions share the same positions…

The family of magnetic rare-earth pyrochlore oxides R2M2O7 plays host to a diverse array of exotic phenomena, driven by the interplay between geometrical frustration and spin-orbit interaction, which leads to anisotropy in both magnetic…

Strongly Correlated Electrons · Physics 2017-03-21 Han Yan , Owen Benton , Ludovic D. C. Jaubert , Nic Shannon

Neutron inelastic scattering and diffraction techniques have been used to study the MnV2O4 spinel system. Our measurements show the existence of two transitions to long-range ordered ferrimagnetic states; the first collinear and the second…

Strongly Correlated Electrons · Physics 2009-11-13 V. O. Garlea , R. Jin , D. Mandrus , B. Roessli , Q. Huang , M. Miller , A. J. Schultz , S. E. Nagler

We study the prototype 5d pyrochlore iridate Y2Ir2O7 from first principles using the local density approximation and dynamical mean-field theory (LDA+DMFT). We map out the phase diagram in the space of temperature, onsite Coulomb repulsion…

Strongly Correlated Electrons · Physics 2015-10-14 Hiroshi Shinaoka , Shintaro Hoshino , Matthias Troyer , Philipp Werner

The search for new quantum phases, especially in frustrated magnets, is central to modern condensed matter physics. One of the most promising places to look is in rare-earth pyrochlore magnets with highly-anisotropic exchange interactions,…

Strongly Correlated Electrons · Physics 2017-03-29 Han Yan , Owen Benton , Ludovic D. C. Jaubert , Nic Shannon

We present AC and DC magnetometry, heat capacity, muon spin relaxation ($\mu$SR) and resonant inelastic X-ray scattering (RIXS) studies of the pyrochlore osmate Y$_2$Os$_2$O$_7$. We observe a non-zero effective moment governed by…

We report a detailed investigation of the magnetic order in 192 stable magnetic two-dimensional materials from the Computational 2D Materials Database having one magnetic atom in the unit cell. The calculations are based on a systematic…

Materials Science · Physics 2024-08-09 Joachim Sødequist , Thomas Olsen