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The dimensionality of the electronic and magnetic structure of a given material is generally predetermined by its crystal structure. Here, using elastic and inelastic neutron scattering combined with magnetization measurements, we find…

The relation between crystal symmetries, electron correlations, and electronic structure steers the formation of a large array of unconventional phases of matter, including magneto-electric loop currents and chiral magnetism. Detection of…

We report low-temperature powder X-ray and neutron diffraction studies on breathing pyrochlore magnets Cu$M$Cr$_{4}$S$_{8}$ ($M$ = Al, Ga), which undergo a magnetic transition at $T_{\rm N} \approx$ 21 and 31 K for {$M$ = Al and Ga,…

Materials Science · Physics 2024-05-09 Masaki Gen , Taro Nakajima , Hiraku Saito , Yusuke Tokunaga , Taka-hisa Arima

The role of spin-orbit coupling and Hund's rule coupling on magnetic ordering, anisotropy, and excitations are investigated within a minimal three-orbital model for the $5d^3$ compound $\rm Na Os O_3$. Asymmetry between the magnetic moments…

Strongly Correlated Electrons · Physics 2019-03-12 Avinash Singh , Shubhajyoti Mohapatra , Churna Bhandari , Sashi Satpathy

Spin-orbit interaction established itself as a major role player for emergent phenomena in modern condensed matter including a topological insulator, spin liquid and spin-dependent transports. However, its function is rather limited to…

Strongly Correlated Electrons · Physics 2022-02-16 Hiroki Nakai , Chisa Hotta

The singlet ground state magnetism in pyrochlore osmates Y$_2$Os$_2$O$_7$ and Ho$_2$Os$_2$O$_7$ is studied by DC and AC susceptibility, specific heat, and neutron powder diffraction measurements. Despite the expected non-magnetic singlet in…

Strongly Correlated Electrons · Physics 2016-05-04 Z. Y. Zhao , S. Calder , A. A. Aczel , M. A. McGuire , B. C. Sales , D. G. Mandrus , G. Chen , N. Trivedi , H. D. Zhou , J. -Q. Yan

Using density functional theory and LDA+U method, we investigate magnetic and electronic structure of Y$_{2}$Ir$_{2}$O$_{7}$ and rare-earth based pyrochlore iridates. Our study reveals that the ground state is a non-collinear magnetic…

Materials Science · Physics 2010-03-18 Xiangang Wan , Jinming Dong , Sergey Y. Savrasov

The influence of the spin-orbit coupling on the magnetic structure of deposited transition metal nanostructure systems has been studied by fully relativistic electronic structure calculations. The interplay of exchange coupling and magnetic…

Materials Science · Physics 2009-02-20 S. Mankovsky , S. Bornemann , J. Minár , S. Polesya , H. Ebert , J. B. Staunton , A. I. Lichtenstein

$\gamma$-triclinic and $\alpha$-monoclinic polymorphs of CoV$_{2}$O$_{6}$ are two of the few known transition metal ion based materials that display stepped $1/3$ magnetization plateaus at low temperatures. Neutron diffraction [M. Markkula…

Strongly Correlated Electrons · Physics 2015-12-23 F. Wallington , A. M. Arevalo-Lopez , J. W. Taylor , J. R. Stewart , V. Garcia-Sakai , J. P. Attfield , C. Stock

In this work we study the interplay between the crystal structure and magnetism of the pyroarsenate \alpha-Cu_2As_2O_7 by means of magnetization, heat capacity, electron spin resonance and nuclear magnetic resonance measurements as well as…

The consequences of nonmagnetic-ion dilution for the pyrochlore family Y$_{2}$($M_{1-x}N_{x}$)$_{2}$O$_{7}$ ($M$ = magnetic ion, $N$ = nonmagnetic ion) have been investigated. As a first step, we experimentally examine the magnetic…

Strongly Correlated Electrons · Physics 2017-10-04 L. Shen , C. Greaves , R. Riyat , T. C. Hansen , E. Blackburn

Density functional calculations are performed to study the magnetic order of the severely distorted square planar cupric oxide (CuO) and local spin disorder in it in the presence of the transition metal impurities M (= Cr, Mn, Fe, Co and…

Strongly Correlated Electrons · Physics 2017-04-05 B. G. Ganga , P. N. Santhosh , B. R. K. Nanda

Pyrochlore iridates A2Ir2O7 (A = rare earth elements, Y or Bi) hold great promise for realizing novel electronic and magnetic states owing to the interplay of spin-orbit coupling, electron correlation and geometrical frustration. A…

Strongly Correlated Electrons · Physics 2017-10-04 W. C. Yang , W. K. Zhu , H. D. Zhou , L. Ling , E. S. Choi , M. Lee , Y. Losovyj , Chi-Ken Lu , S. X. Zhang

Anisotropic multiferroic properties of SrMnGe2O6 pyroxene single crystals were systematically investigated by means of magnetization, heat capacity, pyroelectric current measurement and elastic and inelastic neutron scattering experiments.…

Characterizing the anisotropic structure in noncollinear antiferromagnets is essential for antiferromagnetic spintronics. In this work, we provide a microscopic theory linking the anisotropy effects induced by the rigid-body rotation of…

Materials Science · Physics 2025-07-15 Zheng Liu , Yang Gao , Qian Niu

Metal-insulator transitions in pyrochlore iridates (A2Ir2O7) are believed to occur due to subtle interplay of spin-orbit coupling, geometric frustration, and electron interactions. In particular, the nature of magnetic ordering of iridium…

Strongly Correlated Electrons · Physics 2014-07-29 Eric Kin-Ho Lee , Subhro Bhattacharjee , Yong Baek Kim

Nd2Hf2O7, belonging to the family of geometrically frustrated cubic rare earth pyrochlore oxides, was recently identified to order antiferromagnetically below T_N = 0.55 K with an all-in/all-out arrangement of Nd3+ moments, however with a…

Strongly Correlated Electrons · Physics 2017-12-15 V. K. Anand , D. L. Abernathy , D. T. Adroja , A. D. Hillier , P. K. Biswas , B. Lake

We report the low temperature magnetic properties of Nd$^{3+}$ pyrochlore $\rm Nd_2ScNbO_7$. Susceptibility and magnetization show an easy-axis moment, and heat capacity reveals a phase transition to long range order at $T_N=371(2)$ mK with…

Strongly Correlated Electrons · Physics 2022-08-11 A. Scheie , M. Sanders , Yiming Qiu , T. R. Prisk , R. J. Cava , C. Broholm

Within the past 20 years or so, there has occurred an explosion of interest in the magnetic behavior of pyrochlore oxides of the type $A_{2}^{3+}$$B_{2}^{4+}$O$_{7}$ where $A$ is a rare-earth ion and $B$ is usually a transition metal. Both…

Disordered Systems and Neural Networks · Physics 2010-01-26 Jason S. Gardner , Michel J. P. Gingras , John E. Greedan

We investigate the magnetic order in single crystalline EuCd$_2$Sb$_2$ thin films using a combined theoretical and experimental approach. Resonant elastic x-ray scattering experiments reveal a sharp magnetic peak at $q = (0, 0,…