English

Spin dynamics and unconventional Coulomb phase in Nd$_2$Zr$_2$O$_7$

Strongly Correlated Electrons 2021-07-22 v2 Materials Science

Abstract

We investigate the temperature dependence of the spin dynamics in the pyrochlore magnet Nd2_2Zr2_2O7_7 by neutron scattering experiments. At low temperature, this material undergoes a transition towards an "all in - all out" antiferromagnetic phase and the spin dynamics encompass a dispersion-less mode, characterized by a dynamical spin ice structure factor. Unexpectedly, this mode is found to survive above TN300T_{\rm N} \approx 300 mK. Concomitantly, elastic correlations of the spin ice type develop. These are the signatures of a peculiar correlated paramagnetic phase which can be considered as a new example of Coulomb phase. Our observations near TNT_{\rm N} do not reproduce the signatures expected for a Higgs transition, but show reminiscent features of the "all in - all out" order superimposed on a Coulomb phase.

Keywords

Cite

@article{arxiv.2101.09049,
  title  = {Spin dynamics and unconventional Coulomb phase in Nd$_2$Zr$_2$O$_7$},
  author = {M. Léger and E. Lhotel and M. Ciomaga Hatnean and J. Ollivier and A. R. Wildes and S. Raymond and E. Ressouche and G. Balakrishnan and S. Petit},
  journal= {arXiv preprint arXiv:2101.09049},
  year   = {2021}
}

Comments

6 pages + 9 pages supp. mat