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Related papers: Dynamical Heterogeneity in a Highly Supercooled Li…

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Recently a new approach to the determination of dynamic correlation lengths, {\xi}, for supercooled liquids, based on the properties of the slow (picosecond) vibrational dynamics, was carried out [L. Hong, V.N. Novikov, and A.P. Sokolov,…

Soft Condensed Matter · Physics 2015-05-30 D. Fragiadakis , R. Casalini , C. M. Roland

The dynamics of supercooled liquids slow down and become increasingly heterogeneous as they are cooled. Recently, local structural variables identified using machine learning, such as "softness", have emerged as predictors of local…

Soft Condensed Matter · Physics 2024-06-11 Sean A. Ridout , Andrea J. Liu

As approaching the glass transition, particle motion in liquids becomes highly heterogeneous and regions with virtually no mobility coexist with liquid-like domains. This complex dynamics is believed to be responsible for different…

Soft Condensed Matter · Physics 2018-03-28 F. Puosi , N. Jakse , A. Pasturel

It is known that a finite-size homogeneous granular fluid develops an hydrodynamic-like instability when dissipation crosses a threshold value. This instability is analyzed in terms of modified hydrodynamic equations: first, a source term…

Statistical Mechanics · Physics 2009-10-31 R. Soto , M. Mareschal , M. Malek Mansour

We investigate dynamical heterogeneities in the collective relaxation of a concentrated microgel system, for which the packing fraction can be conveniently varied by changing the temperature. The packing fraction dependent mechanical…

Soft Condensed Matter · Physics 2011-05-31 David A. Sessoms , Irmgard Bischofberger , Luca Cipelletti , Véronique Trappe

Shear viscosity plays a fundamental role in fluid dynamics from heavy-ion collisions to biological processes. Still, its microscopic mechanisms at the individual particle kinetic level remain a subject of ongoing research, specially in…

Soft Condensed Matter · Physics 2025-11-21 Dong Huang , Shaoyu Lu , Chen Liang , Matteo Baggioli , Yan Feng

Supercooled liquids display dynamics that are inherently heterogeneous in space. This essentially means that at temperatures below the melting point, particle dynamics in certain regions of the liquid can be orders of magnitude faster than…

Soft Condensed Matter · Physics 2021-01-04 Dipanwita Ghoshal , Ashwin Joy

Interest in the dynamical arrest leading to a fluid --> solid transition in thermal and athermal systems has led to questions about the nature of these transitions. These jamming transitions may be dependent on the influence of extended…

Soft Condensed Matter · Physics 2007-05-23 Allison Ferguson , Bulbul Chakraborty

Dynamic heterogeneity as one of the most important properties in supercooled liquids has been found for several decades. However, its structural origin remains open for many systems. Here, we propose a new structural parameter to…

Disordered Systems and Neural Networks · Physics 2015-10-16 S. P. Pan , S. D. Feng , J. W. Qiao , W. M. Wang , J. Y. Qin

We use time-resolved dynamic light scattering to investigate the slow dynamics of a colloidal gel. The final decay of the average intensity autocorrelation function is well described by $g\_2(q,\tau)-1 \sim…

Soft Condensed Matter · Physics 2007-05-23 Agnes Duri , Luca Cipelletti

The dynamical heterogeneity in supercooled liquids measured by a molecular dynamics simulation has been quantified on the basis of the multifractal formalism. The singularity spectrum becomes broader as the glass transition is approached.…

Statistical Mechanics · Physics 2009-11-07 W. Sakikawa , O. Narikiyo

Many amorphous glassy materials exhibit complex spatio-temporal mechanical response and rheology, characterized by an intermittent stress-strain response and a fluctuating velocity profile. Under quasistatic and athermal deformation…

Soft Condensed Matter · Physics 2010-02-01 Michel Tsamados

We examined dynamic heterogeneity in a model tetrahedral network glass-forming liquid. We used four-point correlation functions to extract dynamic correlation lengths xi_4^a(t) and susceptibilities chi_4^a(t) corresponding to structural…

Soft Condensed Matter · Physics 2016-01-20 Hannah Staley , Elijah Flenner , Grzegorz Szamel

We numerically investigate the dynamic heterogeneity and its length scale found in the coarse-grained ionic liquid model systems. In our ionic liquid model systems, cations are modeled as dimers with positive charge, while anions are…

Soft Condensed Matter · Physics 2016-03-10 Soree Kim , Sang-Won Park , YounJoon Jung

Recent experiments and computer simulations show that supercooled liquids around the glass transition temperature are "dynamically heterogeneous" [1]. Such heterogeneity is expected from the random first order transition theory of the glass…

Disordered Systems and Neural Networks · Physics 2009-10-31 Xiaoyu Xia , Peter G. Wolynes

In a recent study by some of us, we have proposed a new measure of the structure of a liquid, the softness of the mean-field caging potential, and shown that it can describe the temperature dependence of the dynamics. In this work, we put…

Soft Condensed Matter · Physics 2022-04-27 Mohit Sharma , Manoj Kumar Nandi , Sarika Maitra Bhattacharyya

We solve numerically the equations of nonlinear fluctuating hydrodynamics (NFH) for the supercooled liquid. The time correlation of the density fluctuations in equilibrium obtained here shows quantitative agreement with molecular…

Soft Condensed Matter · Physics 2008-10-02 Bhaskar Sen Gupta , Shankar P. Das , Jean-Louis Barrat

In this work we develop a theoretical framework for the localization of flow in the steadily flowing regime of sheared disordered solids with inertial dynamics on a microscopic scale. To this aim we perform rheology studies at fixed shear…

Soft Condensed Matter · Physics 2018-12-11 Vishwas V Vasisht , Magali Le Goff , Kirsten Martens , Jean-Louis Barrat

We perform molecular dynamics simulations to characterize the occurrence of inhomogeneous shear flows in soft jammed materials. We use rough walls to impose a simple shear flow and study the athermal motion of jammed assemblies of soft…

Soft Condensed Matter · Physics 2012-02-23 Pinaki Chaudhuri , Ludovic Berthier , Lydéric Bocquet

Using molecular dynamics simulations of a binary Lennard-Jones model of glass-forming liquids, we examine how the decay of the normalized neighbor-persistence function $C_{\rm B}(t)$, which decays from unity at short times to zero at long…

Soft Condensed Matter · Physics 2025-02-04 Katrianna S. Sarkar , Kevin A. Interiano-Alberto , Jack F. Douglas , Robert S. Hoy